IP Library Granted Patent US 12662622
Granted Patent B1
US 12662622 · App. 19/313,193 · Granted Jun 23, 2026

Long term stability of mesoporous nano-capsules of cationic surfactant at high temperature and salinity conditions

Inventor: Ahmed Wasel Alsmaeil (Dhahran, SA)
Assignee: SAUDI ARABIAN OIL COMPANY
C09K8/584
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Quick Facts
Patent No.
US 12662622
App. No.
19/313,193
Granted
Jun 23, 2026
Kind
B1
Abstract

A method for stabilizing mesoporous materials includes providing a suspension including a mesoporous particle, wherein the mesoporous particle includes an encapsulated surfactant; contacting the suspension with a solution including ring-opened GLYMO at a temperature ranging from 40 to 80° C. and at a pH ranging from 8 to 11 to form a surface modified mesoporous particle, and contacting the surface modified mesoporous particle with a zwitterionic surfactant solution to form a stabilized mesoporous material. A wellbore fluid composition includes an aqueous base fluid and the mesoporous materials. A method for treating a hydrocarbon-bearing formation includes introducing into a hydrocarbon-bearing formation a wellbore fluid composition including an aqueous base fluid and mesoporous materials, displacing hydrocarbons from the formation by contacting the hydrocarbons with the wellbore fluid composition, and recovering the hydrocarbons.

Claims (31)

1 . A method for stabilizing mesoporous materials comprising:

providing a suspension comprising a mesoporous particle, wherein the mesoporous particle comprises an encapsulated surfactant;

contacting the suspension with a solution comprising ring-opened 3-(glycidyloxypropyl)trimethoxysilane (GLYMO) at a temperature ranging from 40 to 80° C. and at a pH ranging from 8 to 11 to form a surface modified mesoporous particle; and

contacting the surface modified mesoporous particle with a zwitterionic surfactant solution to form a stabilized mesoporous material.

2 . The method of claim 1 , wherein the contacting the surface modified mesoporous particle with a zwitterionic surfactant solution comprises:

sonicating at a temperature of 40° C.-80° C. for 20 minutes to 1 hour.

3 . The method of claim 1 , wherein the zwitterionic surfactant solution comprises:

a zwitterionic surfactant present at a concentration ranging from 0.01 g/mL to 1 g/mL.

4 . The method of claim 1 , wherein the encapsulated surfactant is a cationic or anionic surfactant.

5 . The method of claim 4 , wherein the cationic surfactant is selected from the group consisting of cetyltrimethylammonium bromide, cetyltrimethylammonium chloride, octadecyltrimethylammonium chloride, hexadecylpyridinium bromide, didodecyldimethylammonium bromide, dioctadecyldimethylammonium bromide, and N,N-dimethyl-N-octadecyl-N-benzylammonium chloride.

6 . The method of claim 1 , wherein the stabilized mesoporous materials have an average particle diameter ranging from 5 nm to 500 nm.

7 . The method of claim 1 , wherein the mesoporous particle is MCM-41.

8 . The method of claim 1 , wherein the zwitterionic surfactant solution comprises cocamidopropyl hydroxysultaine.

9 . The method of claim 1 , wherein the solution comprising the ring-opened GLYMO includes GLYMO at a concentration ranges from 9 to 10 μmol/mL.

10 . A wellbore fluid composition comprising:

an aqueous base fluid, and mesoporous materials comprising an encapsulated surfactant and 3-(glycidyloxypropyl)trimethoxysilane (GLYMO) as a surface functionality;

wherein the mesoporous materials are formed by treating the mesoporous materials with a zwitterionic surfactant.

11 . The wellbore fluid composition of claim 10 , wherein the encapsulated surfactant is a cationic surfactant or an anionic surfactant.

12 . The wellbore fluid composition of claim 11 , wherein the cationic surfactant selected from the group consisting of cetyltrimethylammonium bromide, cetyltrimethylammonium chloride, octadecyltrimethylammonium chloride, hexadecylpyridinium bromide, didodecyldimethylammonium bromide, dioctadecyldimethylammonium bromide, and N,N-dimethyl-N-octadecyl-N-benzylammonium chloride.

13 . The wellbore fluid composition of claim 10 , wherein the zwitterionic surfactant is cocamidopropyl hydroxysultaine.

14 . The wellbore fluid composition of claim 10 , wherein the mesoporous materials have an average particle diameter ranging from 5 nm to 500 nm.

15 . The wellbore fluid composition of claim 10 , wherein the mesoporous material is MCM-41.

16 . A method for treating a hydrocarbon-bearing formation comprising:

introducing into a hydrocarbon-bearing formation a wellbore fluid composition comprising an aqueous base fluid and mesoporous materials, wherein the mesoporous materials comprise an encapsulated cationic surfactant and 3-(glycidyloxypropyl)trimethoxysilane (GLYMO) as a surface functionality;

displacing hydrocarbons from the hydrocarbon-bearing formation by contacting the hydrocarbons with the wellbore fluid composition; and

recovering the hydrocarbons from the hydrocarbon-bearing formation,

wherein the mesoporous materials are formed by treating the mesoporous materials with a zwitterionic surfactant.

17 . The method of claim 16 , wherein the mesoporous material is MCM-41 surface-functionalized by GLYMO.

18 . The method of claim 16 , wherein the mesoporous materials have an average particle diameter ranging from 5 nm to 500 nm.

19 . The method of claim 16 , wherein the zwitterionic surfactant is cocamidopropyl hydroxysultaine.

20 . The method of claim 16 , wherein the encapsulated surfactant is a cationic or anionic surfactant, wherein the cationic surfactant is selected from the group consisting of cetyltrimethylammonium bromide, cetyltrimethylammonium chloride, octadecyltrimethylammonium chloride, hexadecylpyridinium bromide, didodecyldimethylammonium bromide, dioctadecyldimethylammonium bromide, and N,N-dimethyl-N-octadecyl-N-benzylammonium chloride; and the anionic surfactant is selected from the group consisting of sodium dodecyl sulfate, sodium lauryl sulfate, and dioctyl sulfosuccinate sodium.