IP Library Granted Patent US 12669441
Granted Patent B2
US 12669441 · App. 18/137,053 · Granted Jun 30, 2026

Methods and kits for rapid, colormetric beryllium detection

Inventors: Melissa Ensor Freiderich (Oak Ridge, TN); Jesse D. Bush (Oak Ridge, TN); Courtney R. Huntley (Oak Ridge, TN)
Assignee: Consolidated Nuclear Security, LLC
G01N21/78G01N2001/028G01N21/293
View Patent ↗
Loading inventors, assignments & file history…
Monitor This Case
Get email alerts when status or documents change.
Order Certified Copies
Most orders are placed with the USPTO same day — all within 24 business hours.
Order via The Patent Place →
Pre-filled with this patent's details
Quick Facts
Patent No.
US 12669441
App. No.
18/137,053
Granted
Jun 30, 2026
Kind
B2
Abstract

Disclosed herein are methods and kits employing a colorimetric test wherein the presence of beryllium is indicated by a visible color change. Advantageously, according to embodiments, when the dye containing substrate contacts beryllium, the color change occurs almost instantly, allowing for rapid, near-real-time detection of beryllium without the use of complex instrumentation.

Claims (44)

1 . A method for rapidly detecting beryllium, the method comprising:

providing a substrate saturated with a dye solution including at least one of Chrome Azurol S (CAS) or Eriochrome Cyanine R (ECR) to form a saturated substrate;

contacting an aqueous solution suspected of containing beryllium with the saturated substrate, wherein the saturated substrate is dry prior to contact with the aqueous solution; and

detecting a visible color change on the saturated substrate following contact with the aqueous solution on a condition that beryllium is present in the aqueous solution at a concentration above a lower limit of detection of 002 microgram, the visible color change occurring in less than about 1 minute.

2 . The method of claim 1 , further comprising:

determining numerical values descriptive of the color change via a colorimeter; and

quantifying an amount of beryllium detected based at least in part on the numerical values.

3 . The method of claim 1 , wherein:

the substrate is at least one of a cotton swatch, a filter paper, a filter felt, a cotton swab, a quilted cotton square or a fabric.

4 . The method of claim 1 , further comprising:

storing the dried substrate for greater than 10 days prior to contacting the aqueous solution.

5 . The method of claim 1 , wherein:

the dye solution includes at least one of ethylenediaminetetraacetic acid (EDTA) or Gum Arabic.

6 . The method of claim 5 , wherein:

the dye solution includes at least one of a surfactant or a buffer.

7 . A method for rapidly detecting beryllium, the method comprising:

providing a substrate saturated with a dye solution including at least one of Chrome Azurol S (CAS) or Eriochrome Cyanine R (ECR) to form a saturated substrate;

wiping a solid surface suspected of containing beryllium thereon with the saturated substrate, wherein the saturated substrate is dry prior to the wiping of the solid surface; and

spraying the saturated substrate, following the wiping, with at least one of water, a dilute acid solution or an ammonium bifluoride solution to dissolve the beryllium and obtain a visible color change on the saturated substrate in less than about 1 minute on a condition that beryllium is present at a concentration above a lower limit of detection of 0.002 microgram.

8 . The method of claim 7 , further comprising:

determining numerical values descriptive of the color change via a colorimeter; and

quantifying an amount of beryllium present based at least in part on the numerical values.

9 . The method of claim 7 , wherein:

the substrate is at least one of a cotton swatch, a filter paper, a filter felt, a cotton swab, a quilted cotton square or a fabric.

10 . The method of claim 7 , wherein:

the substrate has been stored for greater than 10 days prior to the wiping.

11 . The method of claim 7 , wherein:

the dye solution includes ethylenediaminetetraacetic acid (EDTA) and Gum Arabic.

12 . The method of claim 11 , wherein:

the dye solution includes at least one of a surfactant or a buffer.

13 . A kit configured to rapidly detect beryllium, the kit comprising:

a dye solution including at least one of Chrome Azurol S (CAS) or Eriochrome Cyanine R (ECR), the dye solution configured to provide a visible color change in less than about 1 minute in the presence of beryllium at a concentration of at least 0.002 microgram; and

a substrate configured to receive a portion of the dye solution to form a saturated substrate, the saturated substrate being configured to, when dry, contact a target location suspected of containing beryllium to place the dye solution in contact with the suspected beryllium.

14 . The kit of claim 13 , further comprising:

a colorimeter configured to quantify an amount of beryllium present via numerical values for the color change.

15 . The kit of claim 13 , wherein:

the substrate is at least one of a cotton swatch, a filter paper, a filter felt, a cotton swab, a quilted cotton square or a fabric.

16 . The kit of claim 13 , wherein:

the saturated substrate is dried; and

the dried saturated substrate is configured to be stored for at least 10 days prior to use.

17 . The kit of claim 13 , wherein:

the dye solution includes ethylenediaminetetraacetic acid (EDTA) and Gum Arabic.

18 . The kit of claim 13 , wherein:

the dye solution includes at least one of a surfactant or a buffer.