IP Library Granted Patent US 12692363
Granted Patent B2
US 12692363 · App. 18/196,046 · Granted Jul 28, 2026

Protective material and associated protective wear

Inventors: Kamalesh Sirkar (Bridgewater, NJ); Zafar Iqbal (Morris Plains, NJ); Yufeng Song (Newark, NJ); Gregory Peterson (Bel Air, MD); Cheng Peng (Huntington Beach, CA)
Assignees: New Jersey Institute of Technology; The United States of America, as represented by the Secretary of the Army
C08K3/20C08J5/18C08J2327/18
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Quick Facts
Patent No.
US 12692363
App. No.
18/196,046
Granted
Jul 28, 2026
Kind
B2
Abstract

An example protective material formed from a multilayered laminate is provided. The protective material includes a first layer including a microporous membrane supporting a material. The protective material includes a second layer positioned adjacent to the first layer. The second layer includes porous membrane supporting a bed of a metal organic framework (MOF). The combination of the first and second layers provides a barrier against toxic vapors/gases, while allowing for moisture transmission, resulting in protection and comfort to the user.

Claims (24)

1 . A protective material, comprising:

a first layer including a microporous membrane supporting a cross-linked graphene oxide laminate membrane; and

a second layer positioned adjacent to the first layer, the second layer including a porous membrane defining pores, wherein the pores of the porous membrane are filled with nanocrystals of metal organic frameworks.

2 . The protective material of claim 1 , wherein the first layer and the second layer are secured or bonded to each other along an entire overlapping surface area of the respective first and second layers.

3 . The protective material of claim 1 , wherein the first and second layers are flexible.

4 . The protective material of claim 1 , wherein the first layer is configured as an outermost layer of the protective material and is intended to face a feed gas before the second layer faces the feed gas.

5 . The protective material of claim 1 , wherein the first layer blocks chemical warfare agents for a first period of time, and during a second period of time immediately beyond the first period of time, the first layer allows permeation of chemical warfare agents through the first layer and to the second layer at a chemical warfare agent level that is reduced by a factor of at least 94.7% relative to the chemical warfare agent level blocked by the first layer in the first period of time.

6 . The protective material of claim 5 , wherein the second layer at least one of absorbs or adsorbs the permeated chemical warfare agents for the second period of time.

7 . The protective material of claim 1 , wherein the first layer is impermeable to small gases at zero relative humidity and allows water vapor to pass therethrough.

8 . The protective material of claim 1 , wherein the material of the first layer comprises compressed graphene oxide, wherein contiguous layers are crosslinked.

9 . The protective material of claim 1 , wherein the microporous membrane of the first layer is fabricated from polyethersulfone, polyetheretherketone, polyurethane, crosslinked polyvinyl alcohol, polyether block amide, or surface-treated polyamide.

10 . The protective material of claim 1 , wherein the metal organic frameworks of the second layer are sorptive or reactive nanostructured UiO-66-NH 2 .

11 . The protective material of claim 1 , wherein the microporous membrane is bonded to the cross-linked graphene oxide laminate membrane by glutaraldehyde-based or amine-based crosslinking.

12 . The protective material of claim 1 , wherein the first and second layers allow transmission of moisture therethrough at a rate of at least 1,500 g/m 2 per day at 30° C. and a relative humidity difference of 50%.

13 . The protective material of claim 1 , wherein a combination of the first and second layers is configured to completely block ammonia for about 2,750 minutes.

14 . The protective material of claim 1 , wherein a combination of the first and second layers is configured to completely block sulfur mustard gas for about 1,075 minutes.

15 . The protective material of claim 1 , wherein a combination of the first and second layers is configured to completely block Soman gas and a nerve simulant for about 176 minutes.

16 . The protective material of claim 1 , wherein a combination of the first and second layers is configured to completely block dimethyl methyl phosphonate for about 7 days.

17 . The protective material of claim 1 , wherein the microporous membrane of the first layer is laser treated to include laser-induced graphene, and the first layer is configured as an outermost layer of the protective material such that the laser-induced graphene faces a feed gas before the second layer faces the feed gas.

18 . A protective wear fabricated from the protective material of claim 1 .

19 . A protective packaging for one or more items fabricated from the protective material of claim 1 .

20 . A protective material, comprising:

a first layer including a microporous membrane supporting a MXene laminate; and

a second layer positioned adjacent to the first layer, the second layer including a porous membrane defining pores, wherein the pores of the porous membrane are filled with nanocrystals of metal organic frameworks.