IP Library Granted Patent US 12696903
Granted Patent B1
US 12696903 · App. 19/567,795 · Granted Aug 4, 2026

Eco-friendly insecticidal agent against

Inventors: Nashi Khaled Alqahtani (Hofouf, SA); Hany Mohamed Abd El-Lateef Ahmed (Hofouf, SA); Othman A. Farghaly (Al Baha, SA); Antar A. Abdelhamid (Al Baha, SA)
Assignee: KING FAISAL UNIVERSITY
A01N47/40A01P7/04C07D239/22
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Quick Facts
Patent No.
US 12696903
App. No.
19/567,795
Granted
Aug 4, 2026
Kind
B1
Abstract

Synthesis of ethyl ethyl-4-[2-(4-chlorophenyl)ethenyl]-2-(cyanoimino)-6-oxohexahydropyrimidine-5-carboxylate and its use as an insecticidal agent.

Claims (21)

1 . A compound having the formula I:

2 . An insecticidally acceptable composition comprising an insecticidally effective amount of ethyl-4-[2-(4-chlorophenyl)ethenyl]-2-(cyanoimino)-6-oxohexahydropyrimidine-5-carboxylate compound having the formula I:

and an insecticidally acceptable carrier.

3 . A method of killing insects comprising applying an insecticidally effective amount of the insecticidally acceptable composition of claim 2 to the insects or to a target site of insect infestation.

4 . The method of killing insects of claim 3 , wherein the insects belong to the species Aphis gossypii.

5 . The method of killing insects of claim 4 , wherein the ethyl-4-[2-(4-chlorophenyl)ethenyl]-2-(cyanoimino)-6-oxohexahydropyrimidine-5-carboxylate compound has an LC 50 of about 0.561 ppm against the species Aphis gossypii after 24 hours of treatment.

6 . The method of killing insects of claim 4 , wherein the ethyl-4-[2-(4-chlorophenyl)ethenyl]-2-(cyanoimino)-6-oxohexahydropyrimidine-5-carboxylate compound has an LC 50 of about 0.112 ppm against the species Aphis gossypii after 24 hours of treatment.

7 . The method of killing insects of claim 3 , wherein the ethyl-4-[2-(4-chlorophenyl)ethenyl]-2-(cyanoimino)-6-oxohexahydropyrimidine-5-carboxylate compound is applied to cotton leaves.

8 . The method of killing insects of claim 3 , wherein about 12.5 ppm to about 200 ppm of the insecticidally acceptable composition is applied to the insects or to the target site.

9 . A method of repelling insects comprising applying to a target site of insect infestation an insecticidally effective amount of the insecticidally acceptable composition of claim 2 .

10 . The method of repelling insects of claim 9 , wherein the insects belong to the species Aphis gossypii.

11 . A method of controlling an insect pest, comprising applying to a target site of insect infestation an insecticidally effective amount of the insecticidally acceptable composition of claim 2 .

12 . The method of controlling the insect pest of claim 11 , wherein the insect pest belongs to the species Aphis gossypii.

13 . A method of making an ethyl-4-[2-(4-chlorophenyl)ethenyl]-2-(cyanoimino)-6-oxohexahydropyrimidine-5-carboxylate compound, the method comprising:

combining cyanoguanidine, diethyl malonate, and sodium ethoxide to obtain a reaction mixture;

treating the reaction mixture with 3-(4-chlorophenyl) acrylaldehyde to obtain ethyl-4-[2-(4-chlorophenyl)ethenyl]-2-(cyanoimino)-6-oxohexahydropyrimidine-5-carboxylate.

14 . The method of making the ethyl-4-[2-(4-chlorophenyl)ethenyl]-2-(cyanoimino)-6-oxohexahydropyrimidine-5-carboxylate compound of claim 13 , wherein the diethyl malonate is in ethanol.

15 . The method of making the ethyl-4-[2-(4-chlorophenyl)ethenyl]-2-(cyanoimino)-6-oxohexahydropyrimidine-5-carboxylate compound of claim 14 , wherein a catalytic amount of the sodium ethoxide is added.

16 . The method of making the ethyl-4-[2-(4-chlorophenyl)ethenyl]-2-(cyanoimino)-6-oxohexahydropyrimidine-5-carboxylate compound of claim 14 , wherein the ethyl-4-[2-(4-chlorophenyl)ethenyl]-2-(cyanoimino)-6-oxohexahydropyrimidine-5-carboxylate is obtained in about an 62% yield.

17 . The method of making the ethyl-4-[2-(4-chlorophenyl)ethenyl]-2-(cyanoimino)-6-oxohexahydropyrimidine-5-carboxylate compound of claim 14 , wherein the ethyl-4-[2-(4-chlorophenyl)ethenyl]-2-(cyanoimino)-6-oxohexahydropyrimidine-5-carboxylate has a melting point of at least about 166° C. to about 168° C.

18 . The method of making the ethyl-4-[2-(4-chlorophenyl)ethenyl]-2-(cyanoimino)-6-oxohexahydropyrimidine-5-carboxylate compound of claim 14 , wherein the ethyl-4-[2-(4-chlorophenyl)ethenyl]-2-(cyanoimino)-6-oxohexahydropyrimidine-5-carboxylate is a white solid.