IP Library Granted Patent US 12698402
Granted Patent B2
US 12698402 · App. 18/183,641 · Granted Aug 4, 2026

Curable composition, three-dimensional object producing method, three-dimensional object producing apparatus, and artificial tooth object

Inventors: Hiroyuki Naito (Tokyo, JP); Yuki Shingai (Kanagawa, JP); Noriaki Okada (Kanagawa, JP)
Assignee: Ricoh Company, Ltd.
C09D4/06A61C13/0013A61C13/08B33Y70/00C09D7/62C09D7/67C09D7/68C09D135/02C09D175/14B33Y10/00B33Y30/00
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Quick Facts
Patent No.
US 12698402
App. No.
18/183,641
Granted
Aug 4, 2026
Kind
B2
Abstract

A curable composition containing a radical-polymerizable monomer and a hard solid component having a volume average particle diameter of 10 nm or greater and 1,000 nm or less is provided. The content of the hard solid component is 3% by volume or greater and 40% by volume or less. The difference (n 1 −n 2 ) between the refractive index (n 1 ) of a cured product of any other component than the hard solid component and the refractive index (n 2 ) of the hard solid component is 0.04 or greater.

Claims (46)

1 . A curable composition, comprising:

a radical-polymerizable monomer; and

a hard solid component having a volume average particle diameter of 10 nm or greater and 1,000 nm or less,

wherein a content of the hard solid component is 3% by volume or greater and 40% by volume or less,

an absolute value (|n 1 −n 2 |) of a difference between a refractive index (n 1 ) of a cured product of any other component than the hard solid component and a refractive index (n 2 ) of the hard solid component is 0.04 or greater, and

a viscosity of the curable composition at 25° C. is 1,000 mPa·s or lower.

2 . The curable composition according to claim 1 ,

wherein the difference between the refractive indices is 0.05 or greater.

3 . The curable composition according to claim 2 ,

wherein the difference between the refractive indices is 0.07 or greater.

4 . The curable composition according to claim 1 ,

wherein the hard solid component is silica that is surface-modified with a silane coupling agent.

5 . The curable composition according to claim 4 ,

wherein the silane coupling agent contains an unsaturated double bond.

6 . The curable composition according to claim 1 ,

wherein the content of the hard solid component is 5% by volume or greater and 30% by volume or less relative to a whole amount of the curable composition.

7 . The curable composition according to claim 1 ,

wherein the volume average particle diameter of the hard solid component is 100 nm or greater and 500 nm or less.

8 . The curable composition according to claim 7 ,

wherein the volume average particle diameter of the hard solid component is 180 nm or greater and 500 nm or less.

9 . The curable composition according to claim 1 ,

wherein the radical-polymerizable monomer contains a (meth)acrylic-based monomer.

10 . The curable composition according to claim 1 , further comprising:

a polymerization initiator,

wherein a content of the polymerization initiator is 0.1% by mass or greater and 10.0% by mass or less relative to a whole amount of the curable composition.

11 . The curable composition according to claim 1 , further comprising:

a radical-polymerizable oligomer.

12 . The curable composition according to claim 11 ,

wherein the radical-polymerizable oligomer contains a urethane group.

13 . The curable composition according to claim 11 ,

wherein a content of the radical-polymerizable oligomer is 1.0% by mass or greater and 40.0% by mass or less relative to a whole amount of the curable composition.

14 . A three-dimensional object producing method, comprising:

discharging the curable composition according to claim 1 by an inkjet method; and

curing the curable composition discharged, by irradiation with active energy rays,

wherein the three-dimensional object producing method includes repeating the discharging and the curing in order.

15 . A three-dimensional object producing apparatus, comprising:

a storage container storing the curable composition according to claim 1 ;

a discharging unit configured to discharge the curable composition by an inkjet method; and

a curing unit configured to cure the curable composition discharged, by irradiation with active energy rays.

16 . An artificial tooth object, comprising:

a hard solid component having a volume average particle diameter of 10 nm or greater and 1,000 nm or less,

wherein a content of the hard solid component is 3% by volume or greater and 40% by volume or less,

an absolute value (|n 1 −n 2 |) of a difference between a refractive index (n 1 ) of a cured product of any other component than the hard solid component and a refractive index (n 2 ) of the hard solid component is 0.04 or greater,

the hard solid component is spherical particles, and 50% by number of primary particles of the spherical particles are distributed separately from one another, and

a total light transmittance through the artificial tooth object having an average thickness of 1 mm is 30% or lower, and

said artificial tooth object is obtained by irradiating the curable composition according to claim 1 , with active energy rays or heating.