IP Library Granted Patent US 12699054
Granted Patent B2
US 12699054 · App. 18/090,163 · Granted Aug 4, 2026

Stabilized n,n-diethyl-p-phenylenediamine solution and method for detecting chlorine

Inventor: Douglas Royer (Gilbert, IA)
Assignee: HACH COMPANY
G01N21/78G01N33/18
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Quick Facts
Patent No.
US 12699054
App. No.
18/090,163
Granted
Aug 4, 2026
Kind
B2
Abstract

A reagent for chlorine analysis includes N,N-diethyl-p-phenylenediamine (DPD), an inorganic chloride salt at a concentration of 0.5 M or more, and water. Additionally, a method for detecting chlorine in an aqueous sample includes subjecting a test sample to photometry. The test sample includes the aqueous sample; and a DPD reagent that includes DPD, an inorganic chloride salt at a concentration of 0.5 M or more, and water. The reagent and detection method can be used with minimal or no strong acids.

Claims (19)

1 . A reagent for chlorine analysis, the reagent comprising:

N,N-diethyl-p-phenylenediamine (DPD);

an inorganic chloride salt at a concentration of 1.0 M or more; and

water.

2 . The reagent of claim 1 , wherein the reagent is stable for at least 30 days at 20° C.

3 . The reagent of claim 1 , further comprising one or more strong acids at a total concentration of 0.3 M or less.

4 . The reagent of claim 3 , wherein the total concentration of the one or more strong acids in the reagent is 0.2 M or less.

5 . The reagent of claim 3 , wherein the total concentration of the one or more strong acids in the reagent is 0.1 M or less.

6 . The reagent of claim 1 , not comprising any strong acids.

7 . The reagent of claim 1 , wherein the inorganic chloride salt is NaCl or KCl.

8 . The reagent of claim 1 , wherein the inorganic chloride salt is NaCl.

9 . The reagent of claim 1 , wherein the inorganic chloride salt is KCl.

10 . The reagent of claim 1 , wherein the concentration of the inorganic chloride salt in the reagent is 2.0 M or more.

11 . The reagent of claim 1 , wherein the concentration of the inorganic chloride salt in the reagent is 3.0 M or more.

12 . The reagent of claim 3 , wherein a molar ratio of the inorganic chloride salt to the one or more strong acids in the reagent is 30:1 or more.

13 . The reagent of claim 3 , wherein a molar ratio of the inorganic chloride salt to the one or more strong acids in the reagent is 50:1 or more.

14 . The reagent of claim 1 , wherein a concentration of the DPD in the reagent is 20 g/L or more.

15 . The reagent of claim 1 , wherein a molar ratio of the DPD to the inorganic chloride salt in the reagent is in a range of 1:5 to 1:40.

16 . The reagent of claim 3 , wherein a molar ratio of the DPD to the one or more strong acids in the reagent is in a range of 2:1 to 1:5.