IP Library Granted Patent US 12713881
Granted Patent B2
US 12713881 · App. 17/882,840 · Granted Aug 18, 2026

Photoresist having strengthening material

Inventors: Yuan Chih Lo (Hsinchu City, TW); Shi-Cheng Wang (Tainan City, TW); Cheng-Han Wu (Taichung City, TW); Ching-Yu Chang (Yilang County, TW)
Assignee: TAIWAN SEMICONDUCTOR MANUFACTURING COMPANY, LTD.
H10P76/2041G03F7/16G03F7/2002H10P50/71
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Quick Facts
Patent No.
US 12713881
App. No.
17/882,840
Granted
Aug 18, 2026
Kind
B2
Abstract

A method of manufacturing a semiconductor device includes forming a photoresist layer over a substrate, exposing the photoresist layer to an EUV radiation, developing the photoresist layer to form a patterned photoresist, forming a coating layer on the patterned photoresist, and after forming the coating layer on the patterned photoresist, etching the substrate using a combination of the coating layer and the patterned photoresist as an etching mask.

Claims (40)

1 . A method of manufacturing a semiconductor device, comprising:

forming a photoresist layer over a substrate;

exposing the photoresist layer to an EUV radiation;

developing the photoresist layer to form a patterned photoresist;

forming a coating layer on the patterned photoresist and being in direct contact with the patterned photoresist, wherein the coating layer comprises a plurality of separated portions embedded in the patterned photoresist, the separated portions consist essentially of one or more metal oxides; and

after forming the coating layer on the patterned photoresist, etching the substrate primarily using a combination of the coating layer and the patterned photoresist as an etching mask.

2 . The method of claim 1 , wherein the coating layer covers a surface of the patterned photoresist.

3 . The method of claim 1 , wherein the coating layer fills pores in the patterned photoresist.

4 . The method of claim 1 , further comprising:

during or after forming the coating layer on the patterned photoresist, exposing the combination of the coating layer and the patterned photoresist to an extreme ultra violet (EUV) radiation, a deep ultraviolet (DUV) radiation, an ultraviolet (UV) radiation, or a visible light.

5 . The method of claim 1 , further comprising:

during or after forming the coating layer on the patterned photoresist, baking the combination of the coating layer and the patterned photoresist.

6 . The method of claim 1 , further comprising:

during or after forming the coating layer on the patterned photoresist, performing a liquid treatment on the combination of the coating layer and the patterned photoresist.

7 . The method of claim 1 , wherein forming the coating layer on the patterned photoresist is performed using a solution-coating method, a sol-gel process, a chemical vapor deposition (CVD) process, a physical vapor deposition (PVD) process, or an atomic layer deposition (ALD) process.

8 . The method of claim 1 , wherein the coating layer is in a gaseous state at room temperature.

9 . The method of claim 1 , wherein the coating layer is made of a solution prepared by dissolving a chemical compound in an organic solvent or water.

10 . The method of claim 1 , wherein at least one of the separated portions comprise a wavy profile when viewed from a cross-sectional view.

11 . The method of claim 1 , wherein forming the photoresist layer over the substrate comprises forming the photoresist layer comprises a wavy profile when viewed from a cross-sectional view.

12 . A method, comprising:

forming a target layer on a substrate;

forming a patterned mask over the target layer, wherein the patterned mask is made of:

a metal-oxide based photoresist including a plurality of pores; and

a fill material filling into the plurality of pores of the metal-oxide based photoresist and being in direct contact with the metal-oxide based photoresist, wherein the fill material comprises separated portions inside the metal-oxide based photoresist,

the separated portions consist essentially of one or more metal oxides;

etching the target layer primarily using the patterned mask as an etch mask; and

removing the patterned mask.

13 . The method of claim 12 , wherein the fill material comprises the metal oxides including R a Sn b O c R′ d X e , R a Ti b O c R′ d X e , R a Zr b O c R′ d X e , R a Hf b O c R′ d X e , R a Zn b O c R′ d X e , R a Al b O c R′ d X e or R a Cu b O c R′ d X e , R is a mono-dentate organic ligand or a multi-dentate organic ligand consisting of a branched, unbranched, or cyclic alkyl, alkene, alkyne, ketone, amide, carboxylic acid, aromatic ring, or a derivative thereof, substituted with a halogen group, R′ is an organic ligand consisting of a branched, unbranched, or cyclic alkyl, alkene, alkyne, ketone, amide, carboxylic acid, aromatic ring, or a derivative thereof, substituted with a halogen group or an H atom, X is a halide or a carboxylic anion, and a sum of a, c, d and e equals to a multiplied value obtained by multiplying b and an oxidation number of a metal of the metal oxides.

14 . The method of claim 12 , wherein the fill material has molecules having a size smaller than each of the pores of the plurality of pores of the metal-oxide based photoresist.

15 . The method of claim 12 , wherein the separated portions include a multilayer structure.

16 . A method, comprising:

forming a photoresist layer on a substrate;

patterning the photoresist layer into a patterned photoresist;

forming a photoresist-strengthening material on the patterned photoresist and being in direct contact with the patterned photoresist, wherein the photoresist-strengthening material comprises separated portions inside the photoresist layer, the separated portions consist essentially of one or more organometallic compounds;

performing a hardening treatment to harden the photoresist-strengthening material; and

after performing the hardening treatment, etching the substrate primarily using a combination of the hardened photoresist-strengthening material and the patterned photoresist as an etching mask.

17 . The method of claim 16 , wherein the hardening treatment comprises baking the photoresist-strengthening material formed on the patterned photoresist.

18 . The method of claim 16 , wherein the hardening treatment comprises performing a liquid treatment on the photoresist-strengthening material formed on the patterned photoresist.

19 . The method of claim 16 , wherein the photoresist-strengthening material is the organometallic compounds including R a Sn b X c , R a Ti b X c , R a Zr b X c , R a Hf b X c , R a Zn b X c , R a Al b X c or R a Cu b X c , R is a mono-dentate organic ligand or a multi-dentate organic ligand consisting of a branched, unbranched, or cyclic alkyl, alkene, alkyne, ketone, amide, carboxylic acid, aromatic ring, or a derivative thereof, substituted with a halogen group, X is an organic ligand consisting of a branched, unbranched, cyclic alkyl, alkene, alkyne, ketone, amide, carboxylic acid, aromatic ring, or a derivative thereof, substituted with a halogen group, an NR′ 2 , a halide, an SW, or an OR′, R′ consists of a branched, unbranched, or cyclic alkyl, alkene, alkyne, ketone, amide, carboxylic acid, aromatic ring, or a derivative thereof, substituted with a halogen group or an H atom, and a sum of a and c is equal to a multiplied value obtained by multiplying b and an oxidation number of a metal of the organometallic compounds.

20 . The method of claim 16 , wherein the substrate comprises a semiconductor wafer, and forming the photoresist layer on the substrate comprises forming the photoresist layer in direct contact with the semiconductor wafer.