IP Library Granted Patent US 7,247,680
Granted Patent B2
US 7,247,680 · App. 10/466,307 · Granted Jul 24, 2007

High shrink polyethylene films

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Quick Facts
Patent No.
US 7,247,680
App. No.
10/466,307
Granted
Jul 24, 2007
Kind
B2
Abstract

A homogeneous blend of a low density polyethylene with a metallocene-catalysed polyethylene having a density of from 0.906 g/cm 3 and a Dow Rheology Index of at least 5/MI 2 ,MI 2 being the melt index measured according to ASTMD-1238 condition 190° C./2.16 kg and the Dow Rheology Index being determined by a dynamic rheological analysis performed at 190°.

Claims (22)

1. A polyethylene composition comprising a homogenous blend of a low density polyethylene with a metallocene-catalyzed polyethylene having a density of at least 0.906 g/cm 3 and a Dow Rheology Index of at least 5/MI 2 , wherein MI 2 is the melt index measured according to ASTMD-1238 condition 190° C./2.16 kg and the Dow Rheology Index being determined by a dynamic rheological analysis performed at 190°, said metallocene-catalyzed polyethylene being catalyzed with a catalyst system comprising a metallocene component and an activating agent selected from the group consisting of an alumoxane or an aluminum alkyl providing a mole ratio of aluminum to the transition metal of said metallocene component within the range of 50:1-300:1.

2. The composition of claim 1 wherein the metallocene-catalyzed polyethylene has a Dow Rheology Index of at least 10/MI 2 .

3. The composition of claim 1 wherein the metallocene-catalyzed polyethylene has a Dow Rheology Index of at least 20/MI 2 .

4. The composition of claim 1 wherein the metallocene-catalyzed polyethylene has a density of from 0.925 g/cm 3 to less than 0.965 g/cm 3 .

5. The composition of claim 4 wherein the metallocene-catalyzed polyethylene has a Dow Rheology Index of at least 10/MI 2 .

6. The composition of claim 4 wherein the metallocene-catalyzed polyethylene has a Dow Rheology Index of at least 20/MI 2 .

7. The composition of claim 1 wherein the metallocene-catalyzed polyethylene has a density of from 0.906 g/cm 3 to less than 0.925 g/cm 3 .

8. The composition of claim 7 wherein the metallocene-catalyzed polyethylene has a Dow Rheology Index of at least 10/MI 2 .

9. The composition of claim 7 wherein the metallocene-catalyzed polyethylene has a Dow Rheology Index of at least 20/M 2 .

10. A blown film comprising at least one layer formed of a polyethylene composition comprising a homogenous blend of a low density polyethylene with a metallocene-catalyzed polyethylene having a density of at least 0.906 g/cm 3 and a Dow Rheology Index of at least 5/MI 2 , wherein MI 2 is the melt index measured according to ASTMD-1238 condition 190° C./2.16 kg and the Dow Rheology Index being determined by a dynamic rheological analysis performed at 190°, said metallocene-catalyzed polyethylene being catalyzed with a catalyst system comprising a metallocene component and an activating agent selected from the group consisting of an alumoxane or an aluminum alkyl providing a mole ratio of aluminum to the transition metal of said metallocene component within the range of 50:1-300:1.

11. The film of claim 10 wherein said layer is a monolayer blown film.

12. The film of claim 10 wherein said layer comprises at least one layer of a multilayer blown film.

13. A process for the preparation of a blown film, forming said film in a blown film line from a polyethylene composition comprising a homogenous blend of a low density polyethylene with a metallocene-catalyzed polyethylene having a density of at least 0.906 g/cm 3 and a Dow Rheology Index of at least 5/MI 2 , wherein MI 2 is the melt index measured according to ASTMD-1238 condition 190° C./2.16 kg and the Dow Rheology Index being determined by a dynamic rheological analysis performed at 190°, said metallocene-catalyzed polyethylene being catalyzed with a catalyst system comprising a metallocene component and an activating agent selected from the group consisting of an alumoxane or an aluminum alkyl providing a mole ratio of aluminum to the transition metal of said metallocene component within the range of 50:1-300:1, said film being characterized by:

a cohesion force in the transverse direction at room temperature of at least 5% greater than the cohesion force in the transverse direction of a corresponding biaxially-oriented film formed of said low density polyethylene in a pure form; and

a gloss at an angle of 45° of at least 60 and a haze of less than 10% while keeping a good rigidity.

14. A biaxially-oriented film which has been oriented in the machine direction and the transverse direction, formed from a homogenous blend of a polyethylene composition comprising a homogenous blend of a low density polyethylene with a metallocene-catalyzed polyethylene having a density of at least 0.906 g/cm 3 and a Dow Rheology Index of at least 5/MI 2 , wherein MI 2 is the melt index measured according to ASTMD-1238 condition 190° C./2.16 kg and the Dow Rheology Index being determined by a dynamic rheological analysis performed at 190°, said metallocene-catalyzed polyethylene being catalyzed with a catalyst system comprising a metallocene component and an activating agent selected from the group consisting of an alumoxane or an aluminum alkyl providing a mole ratio of aluminum to the transition metal of said metallocene component within the range of 50:1-300:1, said film having a cohesion force in the transverse direction which is greater than the cohesion force in the transverse direction of a corresponding biaxially-oriented film formed of said low density polyethylene in a pure form.

15. The biaxially-oriented film of claim 14 , wherein said film has a cohesion force in the machine direction which is greater than the cohesion force in the machine direction of the corresponding film formed of said low density polyethylene in a pure form.

16. The film of claim 15 , having a gloss at an angle of 45° of at least 60, and a haze which is less than 10%.

17. A blown film comprising at least one layer of the polyethylene composition of claim 4 .

18. The blown film of claim 17 wherein the metallocene catalyzed polyethylene has Dow Rheology Index of at least 10/MI 2 .

19. A biaxially oriented film which has been oriented in the machine direction and the transverse direction, formed from the polyethylene composition of claim 4 wherein said film has a cohesion force in the transverse direction which is greater than the cohesion force in the transverse direction of a corresponding biaxially-oriented film formed of said low density polyethylene in a pure form.

20. THe biaxially-oriented film of calim 19 , wherein said film has a cohesion force in the machine direction which is greater than the cohesion force in the machine direction of the corresponding film formed of said low density polyethylene in a pure form.

Assignments (1)
CHANGE OF NAME Recorded Aug 30, 2005
From: ATOFINA RESEARCH
To: TOTAL PETROCHEMICALS RESEARCH FELUY
Reel/Frame 016470/0203 →