IP Library Granted Patent US 8,083,874
Granted Patent B2
US 8,083,874 · App. 11/115,159 · Granted Dec 27, 2011

Method for producing low thermal expansion Ni-base superalloy

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Quick Facts
Patent No.
US 8,083,874
App. No.
11/115,159
Granted
Dec 27, 2011
Kind
B2
Abstract

A method for producing a low thermal expansion Ni-base superalloy including the steps of subjecting the alloy to a solution heat treatment under the condition of at a temperature of 1000 to 1200° C. and subjecting the alloy to either a carbide stabilizing treatment for making aggregated carbides on grain boundaries and stabilizing the carbides under the conditions of at a temperature of not less than 850° C. and less than 1000° C. and for 1 to 50 hours, or a carbide stabilizing treatment for making aggregated carbides on grain boundaries and stabilizing the carbides by cooling from the temperature in the solution heat treatment to 850° C. at a cooling rate of 100° C. or less per hour. The method also including the steps of subjecting the alloy to a first aging treatment for precipitating y′ phase under the conditions of at a temperature of 720 to 900° C. and for 1 to 50 hours, and subjecting the alloy to a second aging treatment for precipitating A 2 B phase under the conditions of at a temperature of 550 to 700° C. and for 5 to 100 hours.

Claims (70)

1. A method for producing a forged low thermal expansion Ni-base superalloy with a high creep fracture strength, the superalloy comprising a nickel containing γ′ phase, a nickel containing A 2 B phase and, as a matrix, an austenite phase wherein Ni is the main component and Mo, W and Re are solid-solved therein, and a carbide phase in the form of aggregated carbides on grain boundaries, said method comprising:

preparing an alloy comprising, by weight %,

C: 0.02 to 0.15%,

Si: 1% or less,

Mn: 1% or less,

Cr: 5 to 20%,

at least one of Mo, W and Re, which satisfy the relationship Mo+½(W+Re): 17 to 27%,

Al: 0.1 to 1.22%,

Ti: 0.1 to 2%,

Nb and Ta, which satisfy the relationship

Nb+Ta/2: 1.5% or less,

Fe: 10% or less,

Co: 5% or less,

B: 0.001 to 0.02%,

Zr: 0.001 to 0.2%,

a remainder of Ni and inevitable components;

subjecting the alloy to a solution heat treatment under the condition of at a temperature of 1000 to 1200° C.;

subjecting the alloy to either a carbide stabilizing treatment to form the aggregated carbides on grain boundaries and to stabilize the aggregated carbides under the conditions of at a temperature of not less than 850° C. and less than 1000° C. and for 1 to 50 hours, or a carbide stabilizing treatment to form the aggregated carbides on grain boundaries to stabilize the aggregated carbides by cooling from the temperature in the solution heat treatment to 850° C. at a cooling rate of 100° C. or less per hour;

subjecting the alloy to a first aging treatment to precipitate the γ′ phase under the conditions of at a temperature of 720 to 900° C. and for 1 to 50 hours; and

subjecting the alloy to a second aging treatment to precipitate the A 2 B phase under the conditions of at a temperature of 550 to 700° C. and for 5 to 100 hours.

2. The method of claim 1 wherein the alloy is subjected to a carbide stabilizing treatment to form the aggregated carbides on grain boundaries and stabilizing the carbides under the conditions of a temperature of not less than 850° C. and less than 1000° C. for 1 to 50 hours, and the solution heat treatment is from 1050° C. to 1150° C.

3. The method of claim 1 wherein the alloy is subjected to a carbide stabilizing treatment to form the aggregated carbides on grain boundaries and stabilizing the carbides by cooling from the temperature in the solution heat treatment to 850° C. at a cooling rate of 100° C. or less per hour, and the solution heat treatment is from 1050° C. to 1150° C.

4. The method of claim 1 wherein the alloy has enhanced creep rupture strength under high temperature.

5. The method of claim 1 wherein the carbon content is from 0.02 to 0.10.

6. The method of claim 1 , wherein the alloy contains Mo.

7. A method for producing a forged low thermal expansion Ni-base superalloy with high creep fracture strength, the superalloy comprising an nickel containing γ′ phase, a nickel containing A 2 B phase and, as a matrix, an austenite phase wherein Ni is the main component and Mo, W and Re are solid-solved therein, and a carbide phase in the form of aggregated carbides on grain boundaries, said method comprising:

preparing an alloy comprising, by weight %,

C: 0.02 to 0.15%,

Si: 1% or less,

Mn: 1% or less,

Cr: 5 to 20%,

at least one of Mo, W and Re, which satisfy the relationship Mo+½(W+Re): 17 to 27%,

Al: 0 to 1.22%,

Ti: 0.1 to 2%,

Nb and Ta, which satisfy the relationship

Nb+Ta/2: 1.5% or less,

Fe: 10% or less,

Co: 5% or less,

B: 0.001 to 0.02%,

Zr: 0.001 to 0.2%,

a remainder of Ni and inevitable components;

subjecting the alloy to a solution heat treatment under the condition of at a temperature of 1000 to 1200° C.;

subjecting the alloy to a carbide stabilizing treatment to form the aggregated carbides on grain boundaries and to stabilize the aggregated carbides under the conditions of at a temperature of not less than 850° C. and less than 1000° C. and for 1 to 50 hours, subjecting the alloy to a first aging treatment to precipitate the γ′ phase under the conditions of at a temperature of 720 to 900° C. and for 1 to 50 hours; and

subjecting the alloy to a second aging treatment to precipitate the A 2 B phase under the conditions of at a temperature of 550 to 700° C. and for 5 to 100 hours.

8. The method of claim 7 , wherein the alloy has enhanced creep rupture strength under high temperature.

9. The method of claim 7 wherein the carbon content is from 0.02 to 0.10.

10. The method of claim 7 , wherein the carbon content is from 0.02 to 0.10.

11. The method of claim 7 , wherein the alloy contains Mo.

12. A method for producing a forged low thermal expansion Ni-base superalloy with high creep fracture strength, the superalloy comprising a nickel containing γ′ phase, a nickel containing A 2 B phase and, as a matrix, an austenite phase wherein Ni is the main component and Mo, W and Re are solid-solved therein, and a carbide phase in the form of aggregated carbides on grain boundaries, said method comprising:

preparing an alloy comprising, by weight %,

C: 0.02 to 0.15%,

Si: 1% or less,

Mn: 1% or less,

Cr: 5 to 20%,

at least one of Mo, W and Re, which satisfy the relationship Mo+½(W+Re): 17 to 27%,

Al: 0.1 to 1.22%,

Ti: 0.1 to 2%,

Nb and Ta, which satisfy the relationship

Nb+Ta/2: 1.5% or less,

Fe: 10% or less,

Co: 5% or less,

B: 0.001 to 0.02%,

Zr: 0.001 to 0.2%,

a remainder of Ni and inevitable components;

subjecting the alloy to a solution heat treatment under the condition of at a temperature of 1000 to 1200° C.;

a carbide stabilizing treatment to form the aggregated carbides on grain boundaries and to stabilize the aggregated carbides by cooling from the temperature in the solution heat treatment to 850° C. at a cooling rate of 100° C. or less per hour,

subjecting the alloy to a first aging treatment to precipitate the γ′ phase under the conditions of at a temperature of 720 to 900° C. and for 1 to 50 hours; and

subjecting the alloy to a second aging treatment to precipitate the A 2 B phase under the conditions of at a temperature of 550 to 700° C. and for 5 to 100 hours.

13. The method of claim 12 , wherein the alloy has enhanced creep rupture strength under high temperature and contains Mo.

14. The method of claim 13 wherein the carbon content is from 0.02 to 0.10.

Assignments (3)
CORRECTIVE ASSIGNMENT TO CORRECT THE REMOVING PATENT APPLICATION NUMBER 11921683 PREVIOUSLY RECORDED AT REEL: 054975 FRAME: 0438. ASSIGNOR(S) HEREBY CONFIRMS THE ASSIGNMENT. Recorded May 26, 2023
From: MITSUBISHI HITACHI POWER SYSTEMS, LTD.
To: MITSUBISHI POWER, LTD.
Reel/Frame 063787/0867 →
CHANGE OF NAME Recorded Jan 13, 2021
From: MITSUBISHI HITACHI POWER SYSTEMS, LTD.
To: MITSUBISHI POWER, LTD.
Reel/Frame 054975/0438 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Feb 26, 2015
From: MITSUBISHI HEAVY INDUSTRIES, LTD.
To: MITSUBISHI HITACHI POWER SYSTEMS, LTD.
Reel/Frame 035101/0029 →