IP Library Granted Patent US 7,659,327
Granted Patent B2
US 7,659,327 · App. 11/500,019 · Granted Feb 9, 2010

Coated microspheres and their use

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Quick Facts
Patent No.
US 7,659,327
App. No.
11/500,019
Granted
Feb 9, 2010
Kind
B2
Abstract

The invention relates to microspheres coated with a phenolic novolak resin, a process for preparing them, and their use in making foundry shapes, e.g. molds, cores, sleeves, pouring cups, etc., which are used in casting metal parts.

Claims (15)

1. A process for preparing a foundry shape comprising:

(a) filling a tool, which is heated before and/or after filling the tooling, with microspheres coated with a phenolic novolak resin prepared by a process comprising:

(i) mixing a phenolic novolak resin with a refractory comprising heated microspheres;

(ii) adding a catalytically effective amount of hexamethylene tetramine to said mixture; and

(iii) allowing the mixture of (ii) to cure,

(b) curing the coated microspheres to form a cured foundry shape;

(c) removing the cured foundry shape from the tooling.

2. The process of claim 1 wherein the tool is heated to a temperature of 205° C. to 250° C.

3. The process of claim 1 where the uncured portion of the coated microspheres is removed before removing the foundry shape from the tooling.

4. The process of claim 1 wherein the phenolic novolak resin is mixed with salicylic acid before mixing the phenolic novolak resin with the micro spheres.

5. The process of claim 4 wherein the amount of hexamethylene tetramine is from 10 to 25 weight percent based upon the weight of the resin.

6. The process of claim 5 wherein the amount of microspheres is from 10 to 100 percent by volume based upon the volume of the refractory.

7. The process of claim 6 wherein the microspheres are hollow aluminosilicate microspheres.

8. The process of claim 7 wherein in the temperature of the heated microspheres is from 200° C. to 300° C.

9. The process of claim 8 wherein other refractories, selected from the group consisting of silica sand, chromite sand, zircon sand, and mixtures thereof, are used in addition to the microspheres.

Assignments (8)
RELEASE OF SECURITY INTEREST Recorded Nov 4, 2024
From: GLAS TRUST CORPORATION LIMITED
To: ASK CHEMICALS LLC
Reel/Frame 069292/0617 →
CONVERSATION Recorded Mar 30, 2023
From: ASK CHEMICALS L.P.
To: ASK CHEMICALS LLC
Reel/Frame 063196/0385 →
SECURITY INTEREST Recorded Jun 23, 2017
From: ASK CHEMICALS L.P.
To: HSBC CORPORATE TRUSTEE COMPANY (UK) LIMITED, AS SECURITY AGENT
Reel/Frame 042962/0520 →
RELEASE OF SECURITY INTEREST Recorded May 18, 2017
From: INVESTEC BANK, PLC, AS SECURITY AGENT
To: ASK CHEMICALS LP
Reel/Frame 042498/0029 →
SECURITY AGREEMENT SUPPLEMENT Recorded Oct 9, 2014
From: ASK CHEMICALS LP
To: INVESTEC BANK PLC, AS SECURITY AGENT
Reel/Frame 033944/0454 →
CORRECTIVE ASSIGNMENT TO REMOVE PATENT NUMBER 6763859 PREVIOUSLY RECORDED AT REEL: 025622 FRAME: 0222. ASSIGNOR(S) HEREBY CONFIRMS THE ASSIGNMENT. Recorded May 30, 2014
From: ASHLAND LICENSING AND INTELLECTUAL PROPERTY LLC
To: ASK CHEMICALS L.P.
Reel/Frame 033063/0840 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jan 12, 2011
From: ASHLAND LICENSING AND INTELLECTUAL PROPERTY LLC
To: ASK CHEMICALS L.P.
Reel/Frame 025622/0222 →
PARTIAL RELEASE OF PATENT SECURITY AGREEMENT Recorded Dec 2, 2010
From: BANK OF AMERICA, N.A., AS COLLATERAL AGENT
To: ASHLAND LICENSING AND INTELLECTUAL PROPERTY LLC
Reel/Frame 025437/0375 →