IP Library Granted Patent US 9,012,037
Granted Patent B2
US 9,012,037 · App. 12/129,729 · Granted Apr 21, 2015

Hole transport materials

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Quick Facts
Patent No.
US 9,012,037
App. No.
12/129,729
Granted
Apr 21, 2015
Kind
B2
Abstract

There is provided a hole transport compound having Formula I or Formula II: Ar 1 is the same or different at each occurrence and can be phenylene, naphthylene, or binaphthylene. Ar 2 is the same or different at each occurrence and can be phenyl, biphenyl, terphenyl, naphthyl, or binaphthyl. m and n are the same or different and are an integer greater than 0. T is the same or different at each occurrence and is a conjugated moiety including at least one triarylamino group. The T moiety is connected in a non-planar configuration.

Claims (42)

1. A liquid processable hole transport compound having Formula I or Formula II:

wherein:

Ar 1 is the same or different at each occurrence and is selected from the group consisting of phenylene, naphthylene, and binaphthylene;

Ar 2 is the same or different at each occurrence and is selected from the group consisting of phenyl, biphenyl, terphenyl, naphthyl, and binaphthyl;

m and n are the same or different and each is an integer greater than 0; and

T is the same or different at each occurrence and is a conjugated moiety including at least one triarylamino group, wherein the moiety is connected in a non-planar configuration;

wherein the compound comprises at least one set of adjacent aryl groups selected from one of the following:

where R represents an alkyl, aryl, alkoxy, or aryloxy group and the dashed line represents a possible point of attachment,

further comprising at least two sets of adjacent naphthyl groups.

2. A liquid processable hole transport compound having Formula I or Formula II:

wherein:

Ar 1 is the same or different at each occurrence and is selected from the group consisting of phenylene, naphthylene, and binaphthylene;

Ar 2 is the same or different at each occurrence and is selected from the group consisting of phenyl, biphenyl, terphenyl, naphthyl, and binaphthyl;

m and n are the same or different and each is an integer greater than 0; and

T is the same or different at each occurrence and is a conjugated moiety including at least one triarylamino group, wherein the moiety is connected in a non-planar configuration;

wherein the compound comprises at least one set of adjacent aryl groups selected from one of the following:

where R represents an alkyl, aryl, alkoxy, or aryloxy group and the dashed line represents a possible point of attachment.

3. An organic electronic device comprising a first electrical contact layer, a second electrical contact layer and an active layer there between, wherein the active layer comprises a liquid processable hole transport material having Formula I or Formula II:

wherein:

Ar 1 is the same or different at each occurrence and is selected from the group consisting of phenylene, naphthylene, and binaphthylene;

Ar 2 is the same or different at each occurrence and is selected from the group consisting of phenyl, biphenyl, terphenyl, naphthyl, and binaphthyl;

m and n are the same or different and are an integer greater than 0; and

T is the same or different at each occurrence and is a conjugated moiety including at least one triarylamino group, wherein the moiety is connected in a non-planar configuration;

wherein the compound comprises at least one set of adjacent aryl groups selected from one of the following:

where R represents an alkyl, aryl, alkoxy, or aryloxy group and the dashed line represents a possible point of attachment.

4. The compound of claim 2 , wherein T has Formula III:

wherein:

Ar 3 is the same or different at each occurrence and is selected from the group consisting of phenylene, naphthylene, and binaphthylene;

Ar 4 is selected from the group consisting of phenylene, biphenylene, naphthylene, and binaphthylene; and

Ar 5 is the same or different at each occurrence and is selected from the group consisting of phenyl, biphenyl, terphenyl, naphthyl, and binaphthyl.

5. The compound of claim 4 , wherein Ar 3 has at least one substituent selected from the group consisting of alkyl and alkoxy.

6. The compound of claim 1 , wherein T has Formula III:

wherein:

Ar 3 is the same or different at each occurrence and is selected from the group consisting of phenylene, naphthylene, and binaphthylene;

Ar 4 is selected from the group consisting of phenylene, biphenylene, naphthylene, and binaphthylene; and

Ar 5 is the same or different at each occurrence and is selected from the group consisting of phenyl, biphenyl, terphenyl, naphthyl, and binaphthyl.

7. The compound of claim 6 , wherein Ar 3 has at least one substituent selected from the group consisting of alkyl and alkoxy.

8. The device of claim 3 , wherein the active layer is a hole transport layer.

9. The device of claim 3 , wherein the active layer is a photoactive layer and further comprises a photoactive material.

10. The device of claim 9 , wherein the hole transport material functions as a host material for the photoactive material.

11. The device of claim 10 , wherein the ratio of host material to photoactive material is in the range of from 5:1 to 20:1.

12. The device of claim 11 , wherein the ratio of host material to photoactive material is in the range of from 10:1 to 15:1.

Assignments (2)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Aug 22, 2019
From: E. I. DU PONT DE NEMOURS AND COMPANY
To: LG CHEM, LTD.
Reel/Frame 050150/0482 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Aug 20, 2008
From: JOHANSSON, GARY A.; LECLOUX, DANIEL DAVID; SMITH, ERIC MAURICE
To: E. I. DU PONT DE NEMOURS AND COMPANY
Reel/Frame 021414/0344 →