IP Library Granted Patent US 8,445,568
Granted Patent B2
US 8,445,568 · App. 12/237,410 · Granted May 21, 2013

Flame retardant thermoplastic composition and articles formed therefrom

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Quick Facts
Patent No.
US 8,445,568
App. No.
12/237,410
Granted
May 21, 2013
Kind
B2
Abstract

A thermoplastic composition can comprise: polycarbonate, aromatic sulphone sulphonate, aromatic sulphonate, and brominated polycarbonate. In an embodiment, when the composition is formed into a 3 mm thick extruded sheet, the sheet can have a smoke density of less than 200 at an exposure period of 240 seconds in accordance with the smoke density test as set forth in ASTM E662-06, and a burn length of less than 150 mm, a drip flame time of less than 3 seconds, and an overall flame time of less than 15 seconds in accordance with the flammability test as set forth in 14 C.F.R. 25.853, Appendix F, Part I(a)(1)(ii).

Claims (56)

1. A thermoplastic resin composition, comprising:

a transparent polycarbonate resin;

an aromatic sulphonate;

an aromatic sulphone sulphonate different from the aromatic sulphonate; and

a brominated polycarbonate resin;

wherein the composition, when in the form of a 3 mm thick extruded sheet, is transparent and has a smoke density of less than 200 at an exposure period of 240 seconds in accordance with the smoke density test as set forth in ASTM E662-06, and a burn length of less than 150 mm, a drip flame time of less than 3 seconds, and an overall flame time of less than 15 seconds in accordance with the flammability test as set forth in 14 C.F.R. 25.853, Appendix F, Part I(a)(1)(ii); and

wherein the composition, when in the form of a 5 mm thick extruded sheet, has a haze of 0% to 6% as measured in accordance with ASTM D1003-00, Procedure A, illuminant C.

2. The composition of claim 1 , wherein the aromatic sulphone sulphonate is present in an amount of 0.01 wt % to 0.6 wt %, based on the total weight of the composition.

3. The composition of claim 2 , wherein the aromatic sulphone sulphonate is present in an amount of 0.1 wt % to 0.4 wt %, based on the total weight of the composition.

4. The composition of claim 1 , wherein the aromatic sulphonate is present in an amount of 0.01 wt % to 0.1 wt %, based on the total weight of the composition.

5. The composition of claim 4 , wherein the aromatic sulphonate is present in an amount of 0.02 wt % to 0.06 wt %, based on the total weight of the composition.

6. The composition of claim 1 , wherein the brominated polycarbonate comprises 24 wt % to 28 wt % bromine, based on the total weight of the brominated polycarbonate.

7. The composition of claim 6 , wherein the brominated polycarbonate is present in an amount of 1 wt % to 10 wt %, based on the total weight of the composition.

8. The composition of claim 7 , wherein the brominated polycarbonate is present in an amount of 2 wt % to 8 wt %, based on the total weight of the polycarbonate resin.

9. The composition of claim 1 , wherein the aromatic sulphone sulphonate comprises an alkali metal diphenyl sulphone sulphonate and the aromatic sulphonate comprises an alkali metal salt of toluene sulfonic acid.

10. The composition of claim 1 , wherein the aromatic sulphonate comprises a sodium salt of toluene sulfonic acid.

11. The composition of claim 1 , wherein the aromatic sulphone sulphonate comprises potassium diphenyl sulphone sulphonate.

12. A thermoplastic composition, comprising:

0.01 wt % to 0.1 wt % sodium toluene sulphonic acid;

0.01 wt % to 0.6 wt % potassium diphenyl sulphon-3-sulphonate;

a brominated polycarbonate resin, in an amount such that the composition comprises 0.26 wt % to 2.6 wt % bromine; and

a polycarbonate resin;

wherein when the composition is formed into a 3 mm thick extruded sheet, the sheet has a smoke density of less than 200 at an exposure period of 240 seconds in accordance with the smoke density test as set forth in ASTM E662-06, and a burn length of less than 150 mm, a drip flame time of less than 3 seconds, and an overall flame time of less than 15 seconds in accordance with the flammability test as set forth in 14 C.F.R. 25.853, Appendix F, Part I(a)(1)(ii);

wherein the thermoplastic composition, when in the form of a 5 mm thick extruded sheet, has a haze of 0% to 6% as measured in accordance with ASTM D1003-00, Procedure A, illuminant C.

13. A sheet comprising:

a transparent thermoplastic composition, comprising:

0.01 wt % to 0.1 wt % aromatic sulphonate;

0.01 wt % to 0.6 wt % aromatic sulphone sulphonate;

a brominated polycarbonate resin, in an amount such that the composition comprises 0.26 wt % to 2.6 wt % bromine; and

a polycarbonate resin;

wherein the thermoplastic composition is in the form of a transparent sheet;

wherein when the composition is formed into a 3 mm thick extruded sheet, the sheet has a smoke density of less than 200 at an exposure period of 240 seconds in accordance with the smoke density test as set forth in ASTM E662-06, and a burn length of less than 150 mm, a drip flame time of less than 3 seconds, and an overall flame time of less than 15 seconds in accordance with the flammability test as set forth in 14 C.F.R. 25.853, Appendix F, Part I(a)(1)(ii); and

wherein the composition, when in the form of a 5 mm thick extruded sheet, has a haze of 0% to 6% as measured in accordance with ASTM D1003-00, Procedure A, illuminant C.

14. The sheet of claim 13 , wherein the aromatic sulphone sulphonate comprises potassium diphenyl sulphone sulphonate in an amount of 0.1 wt % to 0.4 wt %, and the aromatic sulphonate comprises a sodium salt of toluene sulfonic acid in an amount of 0.01 wt % to 0.1 wt %, based on the total weight of the composition.

15. The sheet of claim 13 , wherein the aromatic sulphonate is present in an amount of 0.02 wt % to 0.06 wt % based on the total weight of the composition, and the composition comprises 0.52 wt % to 2.08 wt % bromine.

16. An aircraft interior component comprising the sheet of claim 13 .

17. The sheet of claim 13 , wherein the sheet has a haze level of less than or equal to 4% as measured in accordance with ASTM D1003-00, Procedure A, illuminant C.

18. A sheet comprising:

transparent thermoplastic resin composition, comprising:

a polycarbonate resin;

an aromatic sulphonate;

an aromatic sulphone sulphonate; and

a brominated polycarbonate resin;

wherein when the composition is formed into a 3 mm thick extruded sheet, the sheet has a smoke density of less than 200 at an exposure period of 240 seconds in accordance with the smoke density test as set forth in ASTM E662-06, and a burn length of less than 150 mm, a drip flame time of less than 3 seconds, and an overall flame time of less than 15 seconds in accordance with the flammability test as set forth in 14 C.F.R. 25.853, Appendix F, Part I(a)(1)(ii); and

wherein the composition, when in the form of a 5 mm thick extruded sheet, has a haze of 0% to 6% as measured in accordance with ASTM D1003-00, Procedure A, illuminant C.

19. The sheet of claim 18 , wherein the sheet has a haze level of less than or equal to 4% as measured in accordance with ASTM D1003-00, Procedure A, illuminant C.

20. The sheet of claim 18 , wherein the aromatic sulphone sulphonate comprises potassium diphenyl sulphone sulphonate and the aromatic sulphonate comprises a sodium salt of toluene sulfonic acid.

21. The composition of claim 1 , wherein, the haze is less than or equal to 4%.

22. The composition of claim 21 , wherein the haze is 0.5% to 4%.

23. The sheet of claim 18 , wherein the haze is less than or equal to 4%.

24. The composition of claim 1 , wherein, when in the form of a 5.0 mm sheet, has a transparency of greater than or equal to 60%, as measured in accordance with ASTM D1003-00, Procedure A, illuminant C.

25. The composition of claim 24 , wherein the transparency is greater than or equal to 75%.

26. The composition of claim 24 , wherein the transparency is greater than or equal to 90%.

27. The composition of claim 1 , wherein the aromatic sulphonate comprises a sodium salt of toluene sulfonic acid in an amount of 0.02 wt % to 0.06wt %, the aromatic sulphone sulphonate comprises potassium diphenyl sulphone sulphonate in an amount of 0.1 wt % to 0.4wt %, and 0.25wt % to 2.5 wt % bromine, all based on the total weight of the composition.

28. The composition of claim 1 , wherein the aromatic sulphonate comprises a sodium salt of toluene sulfonic acid in an amount of 0.01 wt % to 0.1wt %, the aromatic sulphone sulphonate comprises potassium diphenyl sulphone sulphonate in an amount of 0.lwt % to 0.4wt %, and 0.25wt % to 2.5wt % bromine, all based on the total weight of the composition.

29. The composition of claim 1 , wherein the composition comprises 1.04 to 1.56 wt % bromine.

Assignments (4)
CHANGE OF NAME Recorded Jun 6, 2016
From: SABIC INNOVATIVE PLASTICS IP B.V.
To: SABIC GLOBAL TECHNOLOGIES B.V.
Reel/Frame 038883/0816 →
RELEASE OF SECURITY INTEREST Recorded Mar 17, 2014
From: CITIBANK, N.A.
To: SABIC INNOVATIVE PLASTICS IP B.V.
Reel/Frame 032459/0798 →
SECURITY AGREEMENT Recorded Jun 18, 2009
From: SABIC INNOVATIVE PLASTICS IP B.V.
To: CITIBANK, N.A., AS COLLATERAL AGENT
Reel/Frame 022843/0918 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Sep 29, 2008
From: KARREMANS, ARJAN; MAAS, CHRISTIANUS JOHANNES JACOBUS; VAN DEN BOGERD, JOSHUA ARIE; VOLKERS, ANDRIES ADRIAAN
To: SABIC INNOVATIVE PLASTICS IP B.V.
Reel/Frame 021600/0113 →