IP Library Granted Patent US 9,109,153
Granted Patent B2
US 9,109,153 · App. 12/545,747 · Granted Aug 18, 2015

Method for manufacturing a nanoparticle, method for manufacturing a light-emitting element having the nanoparticle, and method for manufacturing a display substrate having the nanoparticle

Inventors: Jung-Han Shin (Yongin-si, KR); Jae-Byung Park (Seongnam-si, KR); Hae-Il Park (Seoul, KR); Jin-Seob Byun (Seoul, KR); Hyoung-Joo Kim (Uiwang-si, KR); Sung-Jee Kim (Pohang-si, KR); Sahid Hussain (Pohang-si, KR); Ji-Won Bang (Pohang-si, KR)
Assignees: SAMSUNG DISPLAY CO., LTD.; POSTECH ACADEMY INDUSTRY FOUNDATION
C09K11/02B82Y30/00C01B19/007C01B25/087C01G3/00C01G5/00C01G7/00C01G9/08C01G11/02C01G15/00C01G55/00C09K11/565C09K11/703C09K11/883H05B33/14C01P2002/84C01P2004/03C01P2004/64C01P2004/84
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Quick Facts
Patent No.
US 9,109,153
App. No.
12/545,747
Granted
Aug 18, 2015
Kind
B2
Abstract

In a method for manufacturing a nanoparticle, a precursor (e.g., transition metal complex) mixed with polyethylene glycol (PEG) is thermally decomposed. A nanoparticle is formed from the thermal decomposition. PEG is cost effective and less toxic than chemicals that are conventionally used for nanoparticle production, so that costs for manufacturing the nanoparticle may be decreased. Further, PEG may be reused to produce more nanoparticles.

Claims (41)

1. A method for manufacturing a nanoparticle, the method comprising:

mixing a precursor with polyethylene glycol (PEG) to form a first mixture,

wherein the precursor comprises a first transition metal complex comprising a first transition metal that forms a core of the nanoparticle;

thermally decomposing the first mixture to form the core of the nanoparticle in the PEG;

after thermal decomposition, mixing a hydrophobic solution having a higher hydrophobicity than the PEG into the PEG containing the nanoparticle to dissolve the nanoparticle into the hydrophobic solution and to precipitate the PEG to solid-state PEG;

separating the solid-state PEG from the hydrophobic solution including the dissolved nanoparticle;

heating the solid-state PEG to transform solid-state PEG into liquid-state PEG; and

reusing the liquid-state PEG to manufacture another nanoparticle.

2. The method of claim 1 , wherein the first mixture is thermally decomposed by agitation at a temperature in a range of about 100° C. to about 300° C.

3. The method of claim 1 , wherein the first mixture is collected via transforming a phase of solid-state PEG.

4. The method of claim 1 , wherein the hydrophobic solution comprises one of hexane, chloroform, and cyclohexane.

5. The method of claim 1 , wherein the nanoparticle comprises one of indium phosphide (InP) and cadmium selenide (CdSe).

6. The method of claim 1 , further comprising forming an outer layer on the nanoparticle using a second transition metal complex,

wherein forming the outer layer comprises:

mixing the second transition metal complex with the first mixture after thermal decomposition to form a second mixture; and

thermally decomposing the second mixture.

7. The method of claim 6 , further comprising:

mixing the thermally decomposed second mixture including the nanoparticle with the outer layer with a hydrophobic solution having a higher hydrophobicity than the PEG; and

separating solid-state PEG from the nanoparticle with the outer layer by precipitating the solid-state PEG in the hydrophobic solution.

8. The method of claim 7 , wherein the first mixture is collected via transforming a phase of solid-state PEG.

9. The method of claim 6 , wherein the outer layer comprises zinc sulfide (ZnS).

10. The method of claim 1 , wherein the nanoparticle comprises at least one of transition metal oxide, transition metal sulfide, transition metal selenide, transition metal telluride, transition metal nitride, transition metal phosphide, and transition metal arsenide.

11. The method of claim 10 , wherein the transition metal comprises at least one of zinc (Zn), cadmium (Cd), mercury (Hg), gallium (Ga), indium (In), tin (Sn), lead (Pb), and copper (Cu).

12. A method for manufacturing a light-emitting element, the method comprising:

thermally decomposing a first mixture including a precursor mixed with PEG to form a nanoparticle, wherein the precursor comprises a first transition metal complex comprising a first transition metal that forms a core of a nanoparticle;

forming a first electrode layer on a substrate;

forming a light-emitting layer having the nanoparticle on the first electrode layer; and

forming a second electrode layer on the light-emitting layer,

after thermal decomposition, mixing a hydrophobic solution having a higher hydrophobicity than the PEG into the PEG containing the nanoparticle to dissolve the nanoparticle into the hydrophobic solution and to precipitate the PEG to solid-state PEG;

separating solid-state PEG from the hydrophobic solution including the nanoparticle;

heating the solid-state PEG to transform solid-state PEG into liquid-state PEG; and

reusing the liquid-state PEG to manufacture another nanoparticle.

13. The method of claim 12 , wherein the first mixture is collected via transforming a phase of solid-state PEG.

14. A method for manufacturing a display substrate, the method comprising:

thermally decomposing a first mixture including a precursor mixed with PEG to form a nanoparticle, wherein the precursor comprises a first transition metal complex comprising a first transition metal that forms a core of the nanoparticle;

forming a color layer disposing the nanoparticle in a pixel area of a substrate,

after thermal decomposition, mixing a hydrophobic solution having a higher hydrophobicity than PEG into the PEG containing the nanoparticle to dissolve the nanoparticle into the hydrophobic solution and to precipitate the PEG to solid-state PEG;

separating solid-state PEG from hydrophobic solution including the nanoparticle;

heating the solid-state PEG to transform solid-state PEG into liquid-state PEG; and

reusing the liquid-state PEG to manufacture another nanoparticle.

15. The method of claim 14 , wherein the first mixture is collected via transforming the phase of solid-state PEG.

Assignments (3)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Sep 20, 2012
From: SAMSUNG ELECTRONICS CO., LTD.
To: SAMSUNG DISPLAY CO., LTD.
Reel/Frame 028992/0001 →
CORRECTIVE ASSIGNMENT TO CORRECT THE ASSIGNEE PREVIOUSLY RECORDED ON REEL 023132 FRAME 0132. ASSIGNOR(S) HEREBY CONFIRMS THE CORRECT CO-ASSIGNEES ARE SAMSUNG ELECTRONICS CO., LTD. AND POSTECH ACADEMY INDUSTRY FOUNDATION. Recorded Mar 7, 2012
From: SHIN, JUNG-HAN; PARK, JAE-BYUNG; PARK, HAE-IL; BYUN, JIN-SEOB; KIM, HYOUNG-JOO; KIM, SUNG-JEE; BANG, JI-WON; SAHID, HUSSAIN
To: SAMSUNG ELECTRONICS CO., LTD.; POSTECH ACADEMY INDUSTRY FOUNDATION
Reel/Frame 027840/0590 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Aug 21, 2009
From: SHIN, JUNG-HAN; PARK, JAE-BYUNG; PARK, HAE-IL; BYUN, JIN-SEOB; KIM, HYOUNG-JOO; KIM, SUNG-JEE; BANG, JI-WON; SAHID, HUSSAIN
To: SAMSUNG ELECTRONICS CO., LTD.
Reel/Frame 023132/0132 →
Continuity (1)
Related Publication 20100129529A1 · May 27, 2010