IP Library Granted Patent US 8,409,595
Granted Patent B2
US 8,409,595 · App. 12/568,763 · Granted Apr 2, 2013

Method for decreasing sebum production

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Quick Facts
Patent No.
US 8,409,595
App. No.
12/568,763
Granted
Apr 2, 2013
Kind
B2
Abstract

The present invention is directed to the topical application of the malonamide ACAT inhibitors described by Formula I. Other aspects of the invention are directed to topical formulations of these diamides, their use to treat sebaceous gland disorders and their use to alleviate oily skin.

Claims (71)

1. A method for alleviating oily skin comprising administering to a patient in need thereof, an effective amount of a compound of the formula:

in which R 1 and R 2 are each independently C 1-6 alkyl;

X is CH 2 ;

R 3 is C 1-6 alkyl or pyridyl;

p is 1;

R 4 is selected from the group consisting of C 1-6 alkyl, C 1-6 alkoxy, and SR 7 ;

R 7 is C 1-6 alkyl;

or a pharmaceutically acceptable salt thereof.

2. A method for decreasing sebum secretion comprising administering to a patient in need thereof, an effective amount of a compound of the formula:

in which R 1 and R 2 are each independently C 1-6 alkyl;

X is CH 2 ;

R 3 is C 1-6 aiki or pyridyl;

p is 1;

R 4 is selected from the group consisting of C 1-6 alkyl, C 1-6 alkoxy, and SR 7 ;

R 7 is C 1-6 alkyl;

or a pharmaceutically acceptable salt thereof.

3. A method for decreasing sebum secretion comprising administering to a patient in need thereof, an effective amount of a compound of the formula:

in which R 3 is C 1-6 alkyl or pyridyl;

R 4 is selected from the group consisting of C 1-6 alkyl, C 1-6 alkoxy, and SR 7 ;

R 7 is C 1-6 alkyl;

or a pharmaceutically acceptable salt thereof.

4. A method according to claim 3 in which said compound is selected from the group consisting of N′-[2,6-bis(1-niethylethyl)phenyl]-N-(1-methylethyl)-N-([4-(methylthio)phenyl]methyl]- propanediamide or pharmaceutically acceptable salt thereof, and N-[2,6-bis(1- methylethyl)pheny]-]β-[[(4-methoxyphenyl)meth)](2-pyridinyl)amino]-]β-oxo-propanamide, or pharmaceutically acceptable salt thereof.

5. A method for treating acne comprising administering to a patient in need thereof, an effective amount of a compound of the formula:

in which R 1 and R 2 are each independently C 1-6 alkyl;

X is CH 2 ;

R 3 is C 1-6 alkyl or pyridyl;

p is 1;

R 4 is selected from the group consisting of C 1-6 alkyl, C 1-6 alkoxy, and SR 7 ;

R 7 is C 1-6 alkyl;

or a pharmaceutically acceptable salt thereof.

6. A method according to claim 5 in which said compound is selected from the group consisting of N′-[2,6-bis(1-methylethyl)phenyl]-N-(1-methylethyl)-N-[[4(methylthio)phenyl]methyl]-propanediamide or pharmaceutically acceptable salt thereof, and N-[2,6-bis(1-methylethyl)phenyl]-]β-[[(4-methoxyphenyl)methyl](2-pyridinyl)amino]-]β-oxo-propanamide or pharmaceutically acceptable salt thereof.

7. An article of manufacture comprising a compound of the formula

in which R 1 and R 2 are each independently C 1-6 alkyl;

X is CH 2 ;

R 3 is C 1-6 alkyl or pyridyl;

p is 1;

R 4 is selected from the group consisting of C 1-6 alkyl, C 1-6 alkoxy, and SR 7 ;

R 7 is C 1-6 alkyl;

or a pharmaceutically acceptable salt thereof, packaged for retail distribution, which advises a consumer how to utilize the compound to alleviate a condition selected from the group consisting of acne, oily skin, and seborrheic dermatitis.

8. The article according to claim 7 in which said compound is N-Benzyl-N′-(2,6-diisopropyl-phenyl)-N-isopropyl-malonamide or a pharmaceutically acceptable salt thereof.

9. A method for alleviating oily skin comprising administering to a patient in need thereof, an effective amount of a compound of the formula:

in which R 3 is C 1-6 alkyl or pyridyl;

R 4 is selected from the group consisting of C 1-6 alkyl, C 1-6 alkoxy, and SR 7 ;

R 7 is C 1-6 alkyl;

or a pharmaceutically acceptable salt thereof.

10. A method according to claim 9 , wherein said compound is selected from the group consisting of N′-[2,6-bis(1-methylethyl)phenyl]-N-(1-methylethyl)-N-[[4-(methylthio)phenyl]methyl]-propanediamide or pharmaceutically acceptable salt thereof, and N-[2,6-bis(1-methylethyl)phenyl]-]β-[[(4-methoxyphenyl)methyl](2-pyridinyl)amino]-]β-oxo-propanamide or pharmaceutically acceptable salt thereof.

11. A method for treating acne comprising administering to a patient in need thereof an effective amount of a compound of the formula:

in which R 3 is C 1-6 alkyl or pyridyi;

R 4 is selected from the group consisting of C 1-6 alkyl, C 1-6 alkoxy, and SR 7 ;

R 7 is C 1-6 alkyl;

or a pharmaceutically acceptable salt thereof.

12. A method for treating seborrheic dermatitis comprising administering to a patient in need thereof an effective amount of a compound of the formula:

in which R 1 and R 2 are each independently C 1-6 alkyl;

X is CH 2 ;

R 3 is C 1-6 alkyl or pyridyl;

p is 1;

R 4 is selected from the group consisting of C 1-6 alkyl, C 1-6 alkoxy, and SR 7 ;

R 7 is C 1-6 alkyl;

or a pharmaceutically acceptable salt thereof.

13. A method for treating seborrheic dermatitis comprising administering to a patient in need thereof, an effective amount of a compound of the formula:

in which R 3 is C 1-6 alkyl or pyridyl;

R 4 is selected from the group consisting of C 1-6 alkyl, C 1-6 alkoxy, and SR 7 ;

R 7 is C 1-6 alkyl;

or a pharmaceutically acceptable salt thereof.

14. A method according to claim 13 , wherein said compound is selected from the group consisting of: N-benzyl-N′-(2,6-diisopropyl-phenyl)-N-isopropyl-malonamide, N′-[2,6-bis(1 -methylethyl)phenyl]-N-(1 -methylethyl)-N-[[4-(methylthio)phenyl]methyl]-propanediamide or pharmaceutically acceptable salt thereof, and N-[2,6-bis(1-methylethyl)phenyl]-]β-[[(4-methoxyphenyl)methyl](2-pyridinyl)amino]-]β-oxo-propanamide or pharmaceutically acceptable salt thereof.

15. An article of manufacture comprision a compound of the formula

in which R 3 is C 1-6 alkyl or pyridyl;

R 4 is selected from the group consisting of C 1-6 alkyl, C 1-6 alkoxy, and SR 7 ;

R 7 is C 1-6 alkyl;

or a pharmaceutically acceptable salt thereof, packaged for retail distribution, which advises a consumer how to utilize the compound to alleviate a condition selected from the group consistion of acne, oily skin, and seborrheic dermatits.

16. The article according to claim 14 , wherein said compound is Selected from the group consistion of: N′-[2,6-bis(1-methylethyl)phenyl]-N-(1-methylethyl)-N-[[4-(methylthio)phenyl]methyl]-propanediamide or pharmaceutically acceptable salt thereof, and N-[2,6-bis(1-methylethyl)phenyl]-]β-[[(4-methoxyphenyl)methyl](2-pyridinyl)amino]-]β-oxo-propanamide or pharmaceutically acceptable salt thereof.

Assignments (8)
RELEASE OF SECURITY INTEREST Recorded Apr 8, 2025
From: BARCLAYS BANK PLC, AS COLLATERAL AGENT
To: SOLTA MEDICAL, INC.; PRECISION DERMATOLOGY, INC.; BAUSCH HEALTH IRELAND LIMITED (F/K/A/ VALEANT PHARMACEUTICALS IRELAND LIMITED); SALIX PHARMACEUTICALS, INC.; SALIX PHARMACEUTICALS, LTD; SANTARUS, INC.; MEDICIS PHARMACEUTICAL CORPORATION; HUMAX PHARMACEUTICAL S.A.; SOLTA MEDICAL IRELAND LIMITED; BAUSCH & LOMB MEXICO, S.A. DE C.V.; BAUSCH+LOMB OPS B.V.; BAUSCH HEALTH AMERICAS, INC.; BAUSCH HEALTH COMPANIES INC.; BAUSCH HEALTH HOLDCO LIMITED; BAUSCH HEALTH MAGYARORSZAG KFT (A/K/A BAUSCH HEALTH HUNGARY LLC); BAUSCH HEALTH POLAND SPOLKA Z OGRANICZONA ODPOWIEDZIALNOSCIA (F/K/A VALEANT PHARMA POLAND SPOLKA Z OGRANICZONA ODPOWIEDZIALNOSCIA); BAUSCH HEALTH US, LLC; BAUSCH HEALTH, CANADA INC. / SANTE BAUSCH, CANADA INC.; ICN POLFA RZESZOW SPOLKA AKCYJNA (A/K/A ICN POLFA RZESZOW S.A.); ORAPHARMA, INC.; PRZEDSIEBIORSTWO FARMACEUTYCZNE JELFA SPOLKA AKCYJNA (A/K/A PRZEDSIEBIORSTWO FARMACEUTYCZNE JELFA S.A.); SOLTA MEDICAL DUTCH HOLDINGS B.V.; V-BAC HOLDING CORP.; VRX HOLDCO LLC; 1261229 B.C. LTD.; 1530065 B.C. LTD.
Reel/Frame 070778/0199 →
NOTICE OF SUCCESSION OF AGENCY Recorded Jan 9, 2015
From: GOLDMAN SACHS LENDING PARTNERS, LLC
To: BARCLAYS BANK PLC, AS SUCCESSOR AGENT
Reel/Frame 034749/0689 →
RELEASE OF SECURITY INTEREST Recorded Jan 10, 2014
From: GOLDMAN SACHS LENDING PARTNERS LLC
To: MEDICIS PHARMACEUTICAL CORPORATION
Reel/Frame 031944/0190 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Sep 25, 2013
From: MEDICIS PHARMACEUTICAL CORPORATION
To: THESAN PHARMACEUTICALS, INC.
Reel/Frame 031280/0766 →
SECURITY AGREEMENT Recorded Apr 24, 2013
From: MEDICIS PHARMACEUTICAL CORPORATION
To: GOLDMAN SACHS LENDING PARTNERS LLC
Reel/Frame 030281/0433 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Dec 13, 2011
From: GRACEWAY PHARMACEUTICALS, LLC
To: MEDICIS PHARMACEUTICAL CORPORATION
Reel/Frame 027370/0813 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded May 18, 2010
From: KOSTLAN, CATHERINE R.; RAHEJA, RAJ NEIL; TUGNAIT, MEERA; WADE, KIMBERLY
To: WARNER-LAMBERT COMPANY LLC
Reel/Frame 024399/0682 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded May 18, 2010
From: PFIZER INC.; WARNER LAMBERT LLC
To: GRACEWAY PHARMACEUTICALS LLC
Reel/Frame 024399/0812 →