IP Library Granted Patent US 8,398,764
Granted Patent B2
US 8,398,764 · App. 12/634,387 · Granted Mar 19, 2013

Titanium and zirconium mixtures and emulsions for use in preparing gypsum wallboard

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Quick Facts
Patent No.
US 8,398,764
App. No.
12/634,387
Granted
Mar 19, 2013
Kind
B2
Abstract

Provided herein are mixtures, emulsions and other additives for use in manufacturing gypsum wallboard. The mixtures and emulsions may be wax-based emulsions or wax-free mixtures or emulsions, with wax-based emulsions including water, at least one wax, a dispersant which may include sulfur or a sulfur-containing group, and an additive comprising an organic titanium compound or organic zirconium compound. Mixtures may also be prepared including water, a dispersant; and an additive comprising an organic titanium compound or organic zirconium compound. Gypsum slurries may be prepared using such emulsions and mixtures and/or through addition of an organic titanium compound or organic zirconium compound.

Claims (33)

1. A wax emulsion useful for gypsum-based building products, comprising,

water;

at least one wax;

a dispersant; and

an additive comprising an organic zirconium compound and/or an organic titanium compound having a chemical formula:

wherein R 1 may be a straight or branched chain, substituted or unsubstituted, alkyl, alkenyl, aralkyl, aralkenyl group of from about 5 to about 30 carbon atoms, wherein the group has from zero to or about 10 oxygen atoms; R 2 may be the same or different than R 1 ; m and n are integers and each is at least 1 and no greater than 4.

2. The wax emulsion according to claim 1 , wherein the at least one wax comprises one or more of montan wax, paraffin wax, carnauba wax, a Fischer-Tropsch wax, and derivatives and blends thereof.

3. The wax emulsion according to claim 2 , wherein the at least one wax is a blend of paraffin wax with montan wax.

4. The wax emulsion according to claim 1 , comprising a paraffinic hydrocarbon.

5. The wax emulsion according to claim 1 , further comprising at least one stabilizer.

6. The wax emulsion according to claim 5 , wherein the at least one stabilizer comprises polyvinyl alcohol.

7. The wax emulsion according to claim 6 , wherein the polyvinyl alcohol is about 97% to about 100% hydrolyzed polyvinyl alcohol.

8. The wax emulsion according to claim 1 , further comprising a saponifying agent.

9. The wax emulsion according to claim 8 , wherein the saponifying agent is an alkali metal hydroxide.

10. A mixture useful for gypsum-based building products, comprising:

water;

a dispersant or blend of dispersants; and

an additive comprising an organic zirconium compound and/or an organic titanium compound having a chemical formula:

wherein R 1 may be a straight or branched chain, substituted or unsubstituted, alkyl, alkenyl, aralkyl, aralkenyl group of from about 5 to about 30 carbon atoms, wherein the group has from zero to or about 10 oxygen atoms; R 2 may be the same or different than R 1 ; m and n are integers and each is at least 1 and no greater than 4.

11. The mixture according to claim 10 , wherein the dispersant comprises a sulfonate or a sulfonate-containing group.

12. The mixture according to claim 10 , wherein the dispersant is lignosulfonic acid, naphthalene sulfonic acid, and combinations and salts thereof.

13. The mixture according to claim 10 , comprising: about 70 percent by weight to about 99.9 percent by weight of the water; about 0.01 percent by weight to about 10 percent by weight of the dispersant; about 0.001 percent by weight to about 10 percent by weight of the additive; and 0 to about 30 percent by weight of at least one stabilizer.

14. The mixture according to claim 13 , comprising: about 80 percent by weight to about 99.9 percent by weight of the water; about 0.01 percent by weight to about 8 percent by weight of the dispersant; about 0.1 percent by weight to about 2.0 percent by weight of the additive; and about 0 percent by weight to about 10 percent by weight of the at least one stabilizer.

15. The mixture according to claim 10 , wherein the additive is selected from the group consisting of titanium IV 2,2(bis-2-propenolatomethyl)butanolato, tris-neodecanato-O; titanium IV 2,2(bis-2-propenolatomethyl)butanolato, tris(dodecyl)benezenesulfanato-O; titanium IV 2,2(bis-2-propenolatomethyl)butanolato, tris(dioctyl)pyrophosphate-O; titanium IV 2-propenolatomethyl, tris-isooctadecanoato-O; sodium zirconium lactate; triethanolamine titanium complex; titanium phosphate complex; alkanolamine titanate; and titanium chelate.

16. The mixture according to claim 10 , wherein R 1 is a branched chain alkenyloxy group of about 5 to about 12 carbon atoms and R 2 is different from R 1 and is a straight chain alkyl group of about 10 to about 15 carbon atoms; m is 1 and n is 3.

17. The mixture according to claim 10 , wherein the additive has a chemical formula:

18. A method for reducing energy use in the manufacture of a building product, wherein the building product is gypsum wallboard, comprising,

adding to a formulation for forming the building product a mixture comprising:

water;

a dispersant; and

an additive comprising an organic zirconium compound and/or an organic titanium compound having the chemical formula:

wherein R 1 may be a straight or branched chain, substituted or unsubstituted, alkyl, alkenyl, aralkyl, aralkenyl group of from about 5 to about 30 carbon atoms, wherein the group has from zero to or about 10 oxygen atoms; R 2 may the same or different than R 1 ; m and n are integers and each is at least 1 and no greater than 4.

19. The method according to claim 18 , wherein the building product is a water-resistant building product and the mixture is a wax emulsion, and wherein the wax emulsion comprises at least one wax.

Assignments (19)
RELEASE OF SECURITY INTEREST IN PATENTS RECORDED AT R/F 39943/0408 Recorded Sep 2, 2021
From: ROYAL BANK OF CANADA, AS AGENT
To: HENRY COMPANY LLC
Reel/Frame 057397/0108 →
INTELLECTUAL PROPERTY RELEASE OF SECURITY INTEREST RECORDED AT R/F 028456/0618 Recorded Oct 6, 2016
From: ANTARES CAPITAL LP, AS SUCCESSOR IN INTEREST TO GENERAL ELECTRIC CAPITAL CORPORATION
To: HENRY COMPANY LLC
Reel/Frame 040241/0956 →
INTELLECTUAL PROPERTY RELEASE OF SECURITY INTEREST RECORDED AT R/F 028456/0633 Recorded Oct 6, 2016
From: GUGGENHEIM CORPORATE FUNDING, LLC
To: HENRY COMPANY LLC
Reel/Frame 040242/0020 →
INTELLECTUAL PROPERTY RELEASE OF SECURITY INTEREST RECORDED AT R/F 033886/0659 Recorded Oct 6, 2016
From: ANTARES CAPITAL LP, AS SUCCESSOR IN INTEREST TO GENERAL ELECTRIC CAPITAL CORPORATION
To: HENRY COMPANY LLC
Reel/Frame 040242/0045 →
INTELLECTUAL PROPERTY RELEASE OF SECURITY INTEREST RECORDED AT R/F 033886/0779 Recorded Oct 6, 2016
From: GUGGENHEIM CORPORATE FUNDING, LLC
To: HENRY COMPANY LLC
Reel/Frame 040242/0495 →
SECURITY INTEREST Recorded Oct 5, 2016
From: HENRY COMPANY LLC
To: ROYAL BANK OF CANADA, AS COLLATERAL AGENT
Reel/Frame 039943/0408 →
CERTIFICATE OF CONVERSION Recorded Jul 19, 2016
From: HENRY COMPANY
To: HENRY COMPANY LLC
Reel/Frame 039389/0808 →
ASSIGNMENT OF INTELLECTUAL PROPERTY SECURITY AGREEMENT Recorded Sep 25, 2015
From: GENERAL ELECTRIC CAPITAL CORPORATION
To: ANTARES CAPITAL LP
Reel/Frame 036687/0869 →
SECURITY INTEREST Recorded Oct 2, 2014
From: HENRY COMPANY LLC
To: GUGGENHEIM CORPORATE FUNDING, LLC, AS ADMINISTRATIVE AGENT
Reel/Frame 033886/0779 →
RELEASE OF SECURITY INTEREST Recorded Jun 27, 2012
From: GENERAL ELECTRIC CAPITAL CORPORATION
To: HENRY COMPANY LLC
Reel/Frame 028455/0086 →
RELEASE OF SECURITY INTEREST Recorded Jun 27, 2012
From: GUGGENHEIM CORPORATE FUNDING, LLC
To: HENRY COMPANY LLC
Reel/Frame 028455/0106 →
FIRST LIEN PATENT SECURITY AGREEMENT Recorded Jun 27, 2012
From: HENRY COMPANY LLC
To: GENERAL ELECTRIC CAPITAL CORPORATION
Reel/Frame 028456/0618 →
SECOND LIEN PATENT SECURITY AGREEMENT Recorded Jun 27, 2012
From: HENRY COMPANY LLC
To: GUGGENHEIM CORPORATE FUNDING, LLC
Reel/Frame 028456/0633 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Apr 22, 2011
From: HENRY COMPANY
To: HENRY COMPANY LLC
Reel/Frame 026171/0567 →
SECURITY AGREEMENT Recorded Dec 31, 2010
From: HENRY COMPANY LLC, A CALIFORNIA LIMITED LIABILITY COMPANY
To: GUGGENHEIM CORPORATE FUNDING, LLC, AS AGENT
Reel/Frame 025573/0733 →
SECURITY AGREEMENT Recorded Dec 29, 2010
From: HENRY COMPANY LLC, A CALIFORNIA LIMITED LIABILITY COMPANY
To: GENERAL ELECTRIC CAPITAL CORPORATION, AS AGENT
Reel/Frame 025570/0566 →
RELEASE OF SECURITY INTEREST Recorded Dec 27, 2010
From: GENERAL ELECTRIC CAPITAL CORPORATION, AS AGENT
To: HENRY COMPANY LLC
Reel/Frame 025537/0694 →
SECURITY AGREEMENT Recorded Mar 23, 2010
From: HENRY COMPANY
To: GENERAL ELECTRIC CAPITAL CORPORATION, AS AGENT
Reel/Frame 024120/0671 →
NUNC PRO TUNC ASSIGNMENT Recorded Mar 1, 2010
From: MAHONEY, DENNIS MICHAEL; STUART, JONATHAN; BURNS, JOHN H.
To: HENRY COMPANY
Reel/Frame 024004/0443 →