IP Library Granted Patent US 8,324,309
Granted Patent B2
US 8,324,309 · App. 12/768,114 · Granted Dec 4, 2012

High melt flow block copolymers for non-woven adhesives

View Patent ↗
Loading inventors, assignments & file history…
Monitor This Case
Get email alerts when status or documents change.
Order Certified Copies
Most orders are placed with the USPTO same day — all within 24 business hours.
Order via The Patent Place →
Pre-filled with this patent's details
Quick Facts
Patent No.
US 8,324,309
App. No.
12/768,114
Granted
Dec 4, 2012
Kind
B2
Abstract

The present invention provides a low viscosity block copolymer for non-wovens construction adhesives of the formula [A−(A/B)]nX, wherein A represents an aromatic vinyl compound and (A/B) represents a polymer block obtained by random copolymerization of a mixture of a aromatic vinyl compound and butadiene in a weight ratio in the range of from 2:98 to 30:70, wherein n is an integer in the range of from 1 to 5, and wherein X is the remainder of the coupling agent.

Claims (24)

1. A non-woven assembly adhesive comprising:

from about 20 to about 30 wt. % of styrenic block copolymer,

from about 40 to about 70 wt. % of tackifier resin, and

from about 5 to about 40 wt. % of plasticizer, all based on 100 wt % of the non-woven assembly adhesive,

said styrenic block copolymer having the formula of (S−S/B) n X, wherein S represents a polymer block of styrene and S/B represents a polymer block obtained by random copolymerization of a mixture of styrene and butadiene in a weight ratio in the range of from 2:98 to 30:70, and said styrenic block copolymer has a total apparent molecular weight from 20,000 to 150,000 g/mol, wherein n is an integer in the range of from 1 to 5, wherein X is the remainder of the coupling agent; and said styrenic block copolymer has a melt flow rate ranging from 40 to about 60 g/min., at 200° C./5 kg;

said tackifier is selected from C5-C9 hydrocarbon resin; and

said plasticizer is an oil compatible with said styrenic block copolymer and said tackifier resin.

2. The non-woven assembly adhesive of claim 1 , wherein said styrenic block copolymer has a coupling efficiency of 70 to about 98%.

3. The non-woven assembly adhesive of claim 1 , wherein said S/B block has a vinyl content in the range of about 7 to about 15 wt. %.

4. The non-woven assembly adhesive of claim 1 , wherein said S/B has average homopolymer block lengths of less than 100 monomer units.

5. The non-woven assembly adhesive of claim 4 , wherein said S/B has average homopolymer block lengths of less than 20 monomer units.

6. The non-woven assembly adhesive of claim 1 , wherein said styrenic block copolymer comprises a polystyrene end-block content from about 30 to about 60 wt. %.

7. A non-woven assembly, comprising a non-woven layer and an adhesive secured thereto, said adhesive comprising

from about 20 to about 30 wt. % of styrenic block copolymer,

from about 40 to about 70 wt. % of tackifier resin, and

from about 5 to about 40 wt. % of plasticizer, all based on 100 wt % of the non-woven assembly adhesive,

said styrenic block copolymer having the formula of (S−S/B) n X, wherein S represents a polymer block of styrene and S/B represents a polymer block obtained by random copolymerization of a mixture of styrene and butadiene in a weight ratio in the range of from 2:98 to 30:70, and said styrenic block copolymer has a total apparent molecular weight from 20,000 to 150,000 g/mol, wherein n is an integer in the range of from 1 to 5, wherein X is the remainder of the coupling agent; and said styrenic block copolymer has a melt flow rate ranging from 40 to about 60 g/min., at 200° C./5 kg;

said tackifier is selected from C5-C9 hydrocarbon resin; and

said plasticizer is an oil compatible with said styrenic block copolymer and said tackifier resin.

8. The non-woven assembly of claim 7 , wherein said styrenic block copolymer has a coupling efficiency of 70 to about 98%.

9. The non-woven assembly of claim 7 , wherein said S/B block has a vinyl content in the range of about 7 to about 15 wt. %.

10. The non-woven assembly of claim 7 , wherein said assembly is a diaper, personal sanitary articles, or a bed pad.

11. The non-woven assembly of claim 7 , wherein said styrenic block copolymer comprises a polystyrene end-block content from about 30 to about 60 wt. %.

12. The non-woven assembly of claim 7 , wherein said S/B has average homopolymer block lengths of less than 100 monomer units.

Assignments (5)
CORRECTIVE ASSIGNMENT TO CORRECT THE PATENT NO. 8837224 TO PATENT NO. 7737224 PREVIOUSLY RECORDED AT REEL: 037448 FRAME: 0453. ASSIGNOR(S) HEREBY CONFIRMS THE ASSIGNMENT. Recorded Jun 11, 2022
From: KRATON POLYMERS U.S. LLC; ARIZONA CHEMICAL COMPANY, LLC
To: BANK OF AMERICA, N.A.
Reel/Frame 060344/0919 →
RELEASE OF SECURITY INTEREST Recorded Mar 15, 2022
From: CREDIT SUISSE AG, CAYMAN ISLANDS BRANCH, AS COLLATERAL AGENT
To: KRATON POLYMERS U.S. LLC
Reel/Frame 059366/0611 →
PATENT SECURITY AGREEMENT Recorded Jan 7, 2016
From: KRATON POLYMERS U.S. LLC
To: CREDIT SUISSE AG, CAYMAN ISLANDS BRANCH, AS COLLATERAL AGENT
Reel/Frame 037457/0843 →
CORRECTIVE ASSIGNMENT TO CORRECT THE PATENT NUMBER 8837224 TO PATENT NUMBER 7737224 PREVIOUSLY RECORDED AT REEL: 037448 FRAME: 0453. ASSIGNOR(S) HEREBY CONFIRMS THE SECURITY INTEREST. Recorded Jan 6, 2016
From: KRATON POLYMERS U.S. LLC; ARIZONA CHEMICAL COMPANY, LLC
To: BANK OF AMERICA, N.A.
Reel/Frame 037448/0453 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jun 30, 2010
From: DUBOIS, DONN
To: KRATON POLYMERS U.S. LLC
Reel/Frame 024618/0994 →