IP Library Granted Patent US 8,309,644
Granted Patent B1
US 8,309,644 · App. 13/220,506 · Granted Nov 13, 2012

Methods of treating carbon fibers, fiber-reinforced resins, and methods of making the fiber-reinforced resins

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Quick Facts
Patent No.
US 8,309,644
App. No.
13/220,506
Granted
Nov 13, 2012
Kind
B1
Abstract

A method of treating carbon fibers includes introducing a functional group to a carbon fiber surface, and reacting the functional group with a silane to incorporate a silanol moiety to the carbon fiber surface. The functional group is chosen from amine groups, carboxyl groups, hydroxyl groups, and/or carbonyl groups. Also disclosed herein are a fiber-reinforced resin and a method of making the same.

Claims (14)

1. A method for treating carbon fibers, comprising:

introducing a functional group to a carbon fiber surface, the functional group being chosen from the group consisting of amine groups, carboxyl groups, hydroxyl groups, carbonyls, and combinations thereof; and

reacting the functional group with a silane to incorporate a silanol moiety to the carbon fiber surface, the silane having an isocyanate group capable of chemically reacting with the functional group introduced to the carbon fiber surface.

2. The method as defined in claim 1 wherein the introducing of the functional group to the carbon fiber surface is accomplished via a chemical, electrochemical, or physical treatment process.

3. The method as defined in claim 1 wherein the silane is chosen from the group consisting of 3-(triethoxysilyl)propyl isocyanate, (trimethoxysilyl)propyl isocyanate, (triethoxysilyl)butyl isocyanate, (triethoxysilyl)ethyl isocyanate, and (triethoxysilyl)methyl isocyanate.

4. A method of making a fiber-reinforced resin, comprising:

treating respective surfaces of carbon fibers by incorporating a silanol moiety to the surfaces by:

introducing a functional group to a carbon fiber surface, the functional group being chosen from the group consisting of amine groups, groups containing oxygen, and combinations thereof; and

reacting the functional group with a silane to incorporate the silanol moiety to the carbon fiber surface, the silane having an isocyanate group capable of chemically reacting with the functional group introduced to the carbon fiber surface;

reacting the treated carbon fibers with a coupling agent to the form a resin-reinforcing material; and

incorporating the resin-reinforcing material into a resin.

5. The method as defined in claim 4 wherein the groups containing oxygen are chosen from the group consisting of carboxyl groups, hydroxyl groups, and carbonyl groups.

6. The method as defined in claim 4 wherein the introducing of the functional group to the carbon fiber surface is accomplished via a chemical, electrochemical, or physical treatment process.

7. The method as defined in claim 4 wherein the coupling agent is chosen from the group consisting of N-β(aminoethyl)-γ-aminopropyl-methyldimethoxy silane, N-β(aminoethyl)-γ-aminopropyl-trimethoxy silane, γ-aminopropyl-triethoxy silane, γ-glycidopropyl-trimethoxy silane, vinyltrimethoxy silane, vinyltriethoxy silane, N-propyl-trimethoxy silane, aminoalkyl silane, γ-methacryloxy-propyl trimethoxy silane, γ-mercaptopropyl trimethoxy silane, and methyltrimethoxy silane.

Assignments (3)
RELEASE OF SECURITY INTEREST Recorded Nov 7, 2014
From: WILMINGTON TRUST COMPANY
To: GM GLOBAL TECHNOLOGY OPERATIONS LLC
Reel/Frame 034186/0776 →
SECURITY AGREEMENT Recorded Jun 28, 2012
From: GM GLOBAL TECHNOLOGY OPERATIONS LLC
To: WILMINGTON TRUST COMPANY
Reel/Frame 028458/0184 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Aug 31, 2011
From: HUANG, XIAOSONG
To: GM GLOBAL TECHNOLOGY OPERATIONS LLC
Reel/Frame 026835/0704 →