IP Library Granted Patent US 9,496,560
Granted Patent B2
US 9,496,560 · App. 13/272,704 · Granted Nov 15, 2016

Fuel cell production method

Inventor: Shigeki Hasegawa (Gotemba, JP)
Assignee: TOYOTA JIDOSHA KABUSHIKI KAISHA
H01M4/9083B82Y30/00H01M4/8814H01M4/8892H01M4/926H01M8/1004H01M2008/1095Y02E60/521Y02P70/56
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Quick Facts
Patent No.
US 9,496,560
App. No.
13/272,704
Granted
Nov 15, 2016
Kind
B2
Abstract

A method of producing a fuel cell includes: preparing a plurality of carbon nanotubes that are aligned substantially vertically to a plane of a substrate; supporting an electrode catalyst on the carbon nanotubes; forming an electrode layer by disposing an ionomer formed of a first solid polymer electrolyte on a surface of the carbon nanotubes on which the electrode catalyst is supported; and placing the electrode layer to face an electrolyte membrane formed of a second solid polymer electrolyte, which has a glass-transition temperature lower than that of the first solid polymer electrolyte, and bonding the electrolyte membrane to the electrode layer by applying a pressure higher than 5 MPa between the electrolyte membrane and electrode layer at a temperature that is higher than the glass-transition temperature of the second solid polymer electrolyte and that is lower than the glass-transition temperature of the first solid polymer electrolyte.

Claims (10)

1. A method of producing a fuel cell, comprising:

preparing a plurality of carbon nanotubes that are aligned vertically to a plane of a substrate;

supporting an electrode catalyst on the carbon nanotubes;

forming an electrode layer by disposing an ionomer formed of a first solid polymer electrolyte having a glass-transition temperature of at least 150° C. on a surface of the carbon nanotubes on which the electrode catalyst is supported;

placing the electrode layer to face an electrolyte membrane formed of a second solid polymer electrolyte, which has a glass-transition temperature of 100° C. to 120° C., and bonding the electrolyte membrane to the electrode layer such that the ionomer on the surface of the carbon nanotubes is not softened and a portion of the carbon nanotubes is embedded in the semi-melted electrolyte membrane, by applying a pressure of 10 MPa to 15 MPa between the electrolyte membrane and electrode layer at a temperature that is higher than or equal to 120° C. and that is lower than 150° C.; and

stopping heating, performing cooling and removing a substrate layer after the electrolyte membrane and electrode layer have been bonded to each other,

wherein the first polymer electrolyte has a weight ratio, with regard to the carbon nanotube grown on the substrate layer, of 1.6 to 2.0.

2. The method of producing a fuel cell according to claim 1 , wherein a shape in a tube length direction of the carbon nanotubes grown on the substrate layer is not a straight shape.

3. The method of producing a fuel cell according to claim 1 , wherein a shape in a tube length direction of the carbon nanotubes grown on the substrate layer is a helical shape.

4. The method of producing a fuel cell according to claim 1 , wherein the glass-transition temperature of the first polymer electrolyte is 30° C. to 50° C. higher than the glass-transition temperature of the second polymer electrolyte.

Assignments (1)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Oct 13, 2011
From: HASEGAWA, SHIGEKI
To: TOYOTA JIDOSHA KABUSHIKI KAISHA
Reel/Frame 027075/0165 →
Priority Claims (1)
JP 2010-235600 · Oct 20, 2010 · national
Continuity (1)
Related Publication 20120100463A1 · Apr 26, 2012