IP Library Granted Patent US 8,920,520
Granted Patent B2
US 8,920,520 · App. 13/409,600 · Granted Dec 30, 2014

Methods of preparing polysaccharide sheets for esterification

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Quick Facts
Patent No.
US 8,920,520
App. No.
13/409,600
Granted
Dec 30, 2014
Kind
B2
Abstract

Processing of cellulose, and more particularly, fiber opening and downstream processing and chemistry are provided. A process includes moistening a cellulose sheet stock to a water content in a range from about 20% to about 50%, attriting the moistened cellulose sheet to a wet pulp, flash drying the wet pulp to a floccule of cellulose having a moisture content from about 4% to about 8%, and esterifying the floccule of cellulose to provide a cellulose ester product.

Claims (41)

1. A process comprising:

moistening a cellulose sheet stock to a water content in a range from about 20% to about 50%;

attriting the moistened cellulose sheet to a wet pulp;

flash drying said wet pulp to a floccule of cellulose having a moisture content from about 4% to about 8%, wherein flash drying is conducted in a flash dryer having an inlet temperature of about 105° C. to about 200° C. and an outlet temperature of about 60° C. to about 130° C.; and

esterifying said floccule of cellulose to provide a cellulose ester product.

2. The process of claim 1 , wherein moistening said cellulose sheet comprises treatment with demineralized water.

3. The process of claim 1 , wherein attriting comprises the steps of:

shredding said cellulose sheet stock into small fragments; and

attriting said small fragments into said wet pulp.

4. The process of claim 1 , wherein flash drying is conducted with a low pressure hot gas, wherein said low pressure is in a range from between about 2 to about 4 psig.

5. The process of claim 1 , wherein the flash drying step is conducted with air that is heated indirectly.

6. The process of claim 1 , further comprising separating said floccule of cellulose in a cyclone separator.

7. The process of claim 1 , wherein the esterification step comprises treatment with acetic anhydride, propionic anhydride, butyric anhydride, a mixed anhydride, and combinations thereof.

8. The process of claim 1 , wherein said process is used to produce a cellulose acetate having a degree of substitution from about 0.1 to about 3 acetate groups per monomer unit.

9. The process of claim 1 , wherein said process is used to produce cellulose diacetate, cellulose triacetate, fiber grade cellulose acetate, water-soluble cellulose acetate, or combinations thereof.

10. The process of claim 1 , further comprising forming a fiber tow from said cellulose ester product.

11. The process of claim 1 , further comprising incorporating said cellulose ester product in a composite matrix comprising one selected from the group consisting of a thermoplastic and a thermoset.

12. The process of claim 10 , further comprising incorporating said cellulose ester tow in a composite matrix comprising one selected from the group consisting of a thermoplastic and a thermoset.

13. A process comprising:

(a) moistening a cellulose sheet stock to a water content in a range from about 20% to about 50%;

(b) attriting the moistened cellulose sheet to a wet pulp;

(c) flash drying said wet pulp to a floccule of cellulose having a moisture content from about 5% to about 8%, wherein flash drying is conducted in a flash dryer having an inlet temperature of about 105° C. to about 200° C. and an outlet temperature of about 60° C. to about 130° C.;

(d) esterifying said floccule of cellulose to provide a cellulose ester product; and

(e) forming a fiber tow from said cellulose ester product.

14. The process of claim 13 , wherein moistening said cellulose sheet comprises treatment with demineralized water.

15. The process of claim 13 , wherein attriting comprises the steps of:

shredding said cellulose sheet stock into small fragments; and

attriting said small fragments into said wet pulp.

16. The process of claim 13 , wherein flash drying is conducted with a low pressure hot gas, wherein said low pressure is in a range from between about 2 to about 4 psig.

17. The process of claim 13 , wherein the flash drying step is conducted with air that is heated indirectly.

18. The process of claim 13 , further comprising separating said floccule of cellulose in a cyclone separator.

19. The process of claim 13 , wherein the esterification step comprises treatment with acetic anhydride, propionic anhydride, butyric anhydride, a mixed anhydride, and combinations thereof.

20. The process of claim 13 , wherein said process is used to produce a cellulose acetate having a degree of substitution from about 0.1 to about 3 acetate groups per monomer unit.

21. The process of claim 13 , wherein said process is used to produce cellulose diacetate, cellulose triacetate, fiber grade cellulose acetate, produce water-soluble cellulose acetate and combinations thereof.

22. The process of claim 13 , further comprising incorporating said cellulose ester tow thereof in a composite matrix comprising one selected from the group consisting of a thermoplastic and a thermoset.

23. A process comprising:

moistening a cellulose sheet stock to a water content of the cellulose sheet stock is about 20% to about 50%;

attriting the moistened cellulose sheet to a wet pulp, wherein a water content of the wet pulp is about 20% to about 50%;

delivering the wet pulp to a flash dryer;

flash drying said wet pulp to a floccule of cellulose, wherein a water content of the flocculate of cellulose is about 4% to about 8%, and wherein the flash dryer has an inlet temperature of about 105° C. to about 200° C. and an outlet temperature of about 60° C. to about 130° C.; and

esterifying said floccule of cellulose to provide a cellulose ester product.

Assignments (2)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Dec 14, 2017
From: CELANESE ACETATE LLC
To: ACETATE INTERNATIONAL LLC
Reel/Frame 044391/0796 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Mar 1, 2012
From: GARRETT, THOMAS S.; KIZER, LAWTON E.; STOGNER, HENRY P.
To: CELANESE ACETATE LLC
Reel/Frame 027790/0401 →