IP Library Granted Patent US 8,809,595
Granted Patent B2
US 8,809,595 · App. 13/517,252 · Granted Aug 19, 2014

Process for recovering monoalkylbenzene

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Quick Facts
Patent No.
US 8,809,595
App. No.
13/517,252
Granted
Aug 19, 2014
Kind
B2
Abstract

The invention relates to a process for recovering monoalkylbenzene from a gas stream comprising oxygen and monoalkylbenzene, —wherein the gas stream comprising oxygen and monoalkylbenzene is contacted with a liquid stream comprising polyalkylbenzene, a compound comprising two phenyl groups connected to each other via a C 1 -C 3 alkylene bridge or a mixture thereof. Further, the present invention relates to a process for preparing alkyl phenyl hydroperoxide incorporating said monoalkylbenzene recovery.

Claims (14)

1. A process for recovering monoalkylbenzene from a gas stream comprising oxygen and monoalkylbenzene, wherein the gas stream comprising oxygen and monoalkylbenzene is contacted with a liquid stream comprising polyalkylbenzene, a compound comprising two phenyl groups connected to each other via a C 1 -C 3 alkylene bridge or a mixture thereof.

2. The process according to claim 1 , wherein the monoalkylbenzene is a benzene which is substituted with an alkyl substituent which is a linear or branched C 1 -C 4 alkyl group, including ethyl, iso-propyl and sec-butyl.

3. The process according to claim 2 , wherein the monoalkylbenzene is ethylbenzene and the liquid stream comprises a mixture comprising triethylbenzene, tetraethylbenzene and 1,2-diphenylethane.

4. The process according to claim 3 , wherein the liquid stream originates from a process for preparing ethylbenzene from ethylene and benzene.

5. The process according to claim 1 , wherein the gas stream and the liquid stream are contacted counter-currently.

6. The process according to claim 5 , wherein the gas stream is fed to the bottom of a vertical column and the liquid stream is fed to the top of said column.

7. The process according to claim 1 , resulting in a liquid stream comprising monoalkylbenzene originating from the gas stream and polyalkylbenzene, a compound comprising two phenyl groups connected to each other via a C 1 -C 3 alkylene bridge or a mixture thereof and a gas stream comprising oxygen, wherein said liquid stream is separated into a fraction comprising monoalkylbenzene and a fraction comprising polyalkylbenzene, a compound comprising two phenyl groups connected to each other via a C 1 -C 3 alkylene bridge or a mixture thereof.

8. A process for preparing alkyl phenyl hydroperoxide comprising:

(i) reacting monoalkylbenzene into alkyl phenyl hydroperoxide using an oxygen containing gas as the oxidant;

(ii) separating the reaction mixture into a liquid stream comprising alkyl phenyl hydroperoxide and monoalkylbenzene and a gas stream comprising oxygen and monoalkylbenzene; and

(iii) contacting the gas stream comprising oxygen and monoalkylbenzene with a liquid stream comprising polyalkylbenzene, a compound comprising two phenyl groups connected to each other via a C 1 -C 3 alkylene bridge or a mixture thereof, resulting in a liquid stream comprising monoalkylbenzene originating from the gas stream and polyalkylbenzene, a compound comprising two phenyl groups connected to each other via a C 1 -C 3 alkylene bridge or a mixture thereof and a gas stream comprising oxygen.

9. The process according to claim 8 , wherein the liquid stream obtained in step (iii) is separated into a fraction comprising monoalkylbenzene and a fraction comprising polyalkylbenzene, a compound comprising two phenyl groups connected to each other via a C 1 -C 3 alkylene bridge or a mixture thereof.

10. The process according to claim 9 , wherein the fraction comprising monoalkylbenzene is recycled to step (i).

11. The process according to claim 9 , wherein the fraction comprising polyalkylbenzene, a compound comprising two phenyl groups connected to each other via a C 1 -C 3 alkylene bridge or a mixture thereof is recycled to step (iii).

Assignments (2)
CHANGE OF NAME Recorded Mar 7, 2022
From: SHELL OIL COMPANY
To: SHELL USA, INC.
Reel/Frame 059694/0819 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jan 10, 2013
From: HAWTON, MALCOLM JOHN
To: SHELL OIL COMPANY
Reel/Frame 029602/0138 →