IP Library Granted Patent US 8,845,882
Granted Patent B2
US 8,845,882 · App. 13/578,384 · Granted Sep 30, 2014

High light olefins FCC catalyst compositions

Inventors: Yuying Shu (Ellicott City, MD); Richard F. Wormsbecher (Dayton, MD); Wu-Cheng Cheng (Ellicott City, MD)
Assignee: W. R. Grace & Co.-Conn.
C10G11/18C10G2400/02B01J29/088C10G2400/20C10G2300/70B01J2229/18
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Quick Facts
Patent No.
US 8,845,882
App. No.
13/578,384
Granted
Sep 30, 2014
Kind
B2
Abstract

Catalytic cracking catalyst compositions and processes for cracking hydrocarbons to maximize light olefins production are disclosed. Catalyst compositions comprise at least one zeolite having catalytic cracking activity under catalytic cracking conditions, preferably Y-type zeolite, which zeolite has low amounts of yttrium in specified ratios to rare earth metals exchanged on the zeolite. Catalyst and processes of the invention provide increased yields of light olefins and gasoline olefins during a FCC process as compared to conventional lanthanum containing Y-type zeolite FCC catalysts.

Claims (18)

1. A catalyst composition for catalytically cracking hydrocarbons to maximize light olefins production, which composition comprises a zeolite having catalytic cracking activity under catalytic cracking conditions, said zeolite being exchanged with yttrium and at least one rare earth metal, wherein the amount of yttrium exchanged on the zeolite ranges from about 1.75 wt % to about 0.175 wt % of the zeolite, and the ratio of yttrium to rare earth metal exchanged on the zeolite ranges from about 3 to about 50.

2. The catalyst of claim 1 wherein the zeolite is a faujasite zeolite.

3. The catalyst of claim 2 wherein the zeolite is a Y-type zeolite.

4. The catalyst of claim 1 wherein the rare earth metal is a metal selected from group consisting of lanthanum, a metal of the Lanthanide Series of the Periodic Table having an atomic number from 58 to 71, and combinations thereof.

5. The catalyst of claim 1 wherein the amount of zeolite present in the catalyst ranges from about 10 wt % to about 60 wt % of the catalyst composition.

6. The catalyst of claim 5 wherein the amount of zeolite present in the catalyst ranges from about 20 wt % to about 50 wt % of the catalyst composition.

7. The catalyst of claim 1 wherein the ratio of yttrium to rare earth exchanged on the zeolite is 3.5 to 20.

8. The catalyst of claim 1 wherein the catalyst further comprises clay.

9. The catalyst of claim 1 wherein the catalyst further comprises at least one ZSM-5 light olefins additive.

10. The catalyst of claim 9 wherein the ZSM-5 light olefins additive comprises a phosphorus stabilized ZSM-5 additive.

11. A process of catalytically cracking a hydrocarbon feedstock into lower molecular weight components to maximize light olefins production, said method comprising contacting a hydrocarbon feedstock with a cracking catalyst at elevated temperature whereby lower molecular weight hydrocarbon components are formed, said cracking catalyst comprising a zeolite having catalytic cracking activity under catalytic cracking conditions, said zeolite being exchanged with yttrium and at least one rare earth metal, wherein the amount of yttrium exchanged on the zeolite ranges from about 1.75 wt % to about 0.175 wt % of the zeolite, and the ratio of yttrium to rare earth metal exchanged on the zeolite ranges from about 3 to about 50.

12. The process of claim 11 wherein the cracking catalyst further comprises faujasite zeolite.

13. The process of claim 12 wherein the zeolite is a Y type zeolite.

14. The process of claim 11 further comprising recovering the cracking catalyst from said contacting step and treating the used catalyst in a regeneration zone to regenerate said catalyst.

15. The process of claim 11 wherein the hydrocarbon feedstock is contacted with the cracking catalyst under fluid catalytic cracking conditions.

16. The process of claim 11 wherein the zeolite is a Y-type zeolite.

17. The process of claim 11 wherein the ratio of yttrium to rare earth exchanged on the zeolite is 3.5 to 20.

18. The process of claim 11 wherein the catalyst further comprises at least one ZSM-5 light olefins additive.

Assignments (10)
NOTES SECURITY INTEREST Recorded Jan 29, 2026
From: W. R. GRACE & CO.-CONN.; ADVANCED REFINING TECHNOLOGIES LLC
To: WILMINGTON TRUST, NATIONAL ASSOCIATION, AS NOTES COLLATERAL AGENT
Reel/Frame 074532/0229 →
SECURITY AGREEMENT (NOTES) Recorded Aug 19, 2025
From: W. R. GRACE & CO.-CONN.
To: WILMINGTON TRUST, NATIONAL ASSOCIATION, AS NOTES COLLATERAL AGENT
Reel/Frame 072520/0653 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Mar 9, 2023
From: SHU, YUYING; WORMSBECHER, RICHARD FRANKLIN; CHENG, WU-CHENG
To: W.R. GRACE & CO.-CONN.
Reel/Frame 062938/0460 →
SECURITY INTEREST Recorded Feb 17, 2023
From: W.R. GRACE & CO.-CONN.
To: WILMINGTON TRUST, NATIONAL ASSOCIATION
Reel/Frame 062792/0510 →
RELEASE OF SECURITY INTEREST Recorded Sep 23, 2021
From: GOLDMAN SACHS BANK USA
To: W. R. GRACE & CO.-CONN.
Reel/Frame 057594/0026 →
NOTES SECURITY AGREEMENT Recorded Sep 23, 2021
From: W. R. GRACE & CO.-CONN.
To: WILMINGTON TRUST, NATIONAL ASSOCIATION
Reel/Frame 057594/0156 →
TERM LOAN SECURITY AGREEMENT Recorded Sep 23, 2021
From: W. R. GRACE & CO.-CONN.
To: JPMORGAN CHASE BANK, N.A.
Reel/Frame 057594/0104 →
SECURITY INTEREST Recorded Apr 3, 2018
From: W. R. GRACE & CO.-CONN.
To: GOLDMAN SACHS BANK USA, AS COLLATERAL AGENT
Reel/Frame 045828/0683 →
RELEASE OF SECURITY AGREEMENT RECORDED AT REEL/FRAME NO.: 032159/0384 Recorded Apr 3, 2018
From: GOLDMAN SACHS BANK USA, AS THE COLLATERAL AGENT
To: W.R. GRACE & CO.-CONN.
Reel/Frame 045832/0887 →
SECURITY AGREEMENT Recorded Feb 4, 2014
From: W.R. GRACE & CO.-CONN.
To: GOLDMAN SACHS BANK USA, AS THE COLLATERAL AGENT
Reel/Frame 032159/0384 →
Continuity (2)
Provisional Application 61315317 · Mar 18, 2010
Related Publication 20130001134A1 · Jan 3, 2013