IP Library Granted Patent US 8,591,988
Granted Patent B1
US 8,591,988 · App. 13/652,936 · Granted Nov 26, 2013

Method of fabrication of anchored nanostructure materials

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Quick Facts
Patent No.
US 8,591,988
App. No.
13/652,936
Granted
Nov 26, 2013
Kind
B1
Abstract

Methods for fabricating anchored nanostructure materials are described. The methods include heating a nano-catalyst under a protective atmosphere to a temperature ranging from about 450° C. to about 1500° C. and contacting the heated nano-catalysts with an organic vapor to affix carbon nanostructures to the nano-catalysts and form the anchored nanostructure material.

Claims (18)

1. A method of producing an anchored nanostructure material comprising:

(a) etching a substrate with an etchant to produce metal ions adjacent the surface of the substrate;

(c) exposing the metal ions to hydrogen to reduce the metal ions and produce nano-catalysts;

(d) heating the nano-catalysts under a protective atmosphere to a temperature ranging from about 450° C. to about 1500° C.; and

(e) contacting the heated nano-catalysts with an organic vapor to affix carbon nanostructures to the nano-catalysts and form the anchored nanostructure material.

2. The method of claim 1 wherein step (e) comprises flowing the organic vapor proximal to the heated nano-catalysts at a rate ranging from about 100 cc/minute to about 10 L/minute.

3. The method of claim 1 wherein step (e) comprises exposing the heated nano-catalysts to the organic vapor at a process pressure of ranging from about 1 torr to about 1000 torr.

4. The method of claim 1 further comprising the steps:

(e) cooling the anchored nanostructure material under a protective atmosphere to a temperature at which the anchored nanostructure material does not significantly oxidize in an ambient atmosphere; and

(f) discontinuing the protective atmosphere and providing access to the anchored nanostructure material in the ambient atmosphere.

5. The method of claim 1 wherein step (a) further comprises drying the substrate in the presence of the etchant wherein nano-size deposits comprising the metal ions are deposited adjacent the surface of the substrate.

6. The method of claim 1 wherein step (d) further comprises exposing the heated nano-catalysts to hydrogen while contacting the heated nano-catalysts with the organic vapor.

7. The method of claim 1 wherein the substrate comprises nickel and wherein the etchant is selected from the group consisting of an aqueous solution of a chloride salt of aluminum, dilute hydrochloric acid, and combinations thereof.

8. The method of claim 1 wherein the substrate comprises nickel and wherein the etchant is selected from the group consisting of an aqueous solution of a nitrate salt of aluminum, dilute nitric acid, and combinations thereof.

9. The method of claim 1 wherein the substrate comprises nickel in the form of nickel aluminide and wherein the etchant is selected from the group consisting of an aqueous solution of a chloride salt of aluminum, dilute hydrochloric acid, and combinations thereof.

10. The method of claim 1 wherein the substrate comprises nickel in the form of nickel aluminide and wherein the etchant is selected from the group consisting of an aqueous solution of a nitrate salt of aluminum, dilute nitric acid, and combinations thereof.

11. The method of claim 1 further comprising disposing a coupling agent on the surface of the substrate to facilitate binding of the metal ions to the substrate.

12. The method of claim 1 further comprising disposing a chelating agent on the surface of the substrate to facilitate binding of the metal ions to the substrate.

Assignments (3)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Sep 17, 2014
From: BABCOCK & WILCOX TECHNICAL SERVICES Y-12, LLC
To: CONSOLIDATED NUCLEAR SECURITY, LLC
Reel/Frame 033756/0649 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Oct 16, 2013
From: SEALS, ROLAND D.; MENCHHOFER, PAUL A.; HOWE, JANE Y.; WANG, WEI
To: BABCOCK & WILCOX TECHNICAL SERVICES Y-12, LLC
Reel/Frame 031415/0328 →
CONFIRMATORY LICENSE Recorded Feb 13, 2013
From: SANDIA CORPORATION
To: U.S. DEPARTMENT OF ENERGY
Reel/Frame 029809/0413 →