IP Library Granted Patent US 9,186,307
Granted Patent B2
US 9,186,307 · App. 13/835,819 · Granted Nov 17, 2015

Treated silicas and metal silicates for improved cleaning in dentifrice

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Quick Facts
Patent No.
US 9,186,307
App. No.
13/835,819
Granted
Nov 17, 2015
Kind
B2
Abstract

Treated silica materials are disclosed, together with methods of making such materials and dentifrice compositions comprising the treated silica materials.

Claims (29)

1. A method for preparing a heat treated silica material, the method comprising heat treating a precipitated silica material comprising a metal, wherein the metal has a Mohs hardness value of at least about 5.5 in its oxide form, and wherein heat treating comprises heating the precipitated silica material at a temperature and for a period of time sufficient to produce the heat treated silica material, which is characterized by a loss on ignition at 900° C. of less than about 3 wt. %, and wherein:

an Einlehner abrasion value of the heat treated silica material is from about 90% to about 450% greater than an Einlehner abrasion value of the precipitated silica material.

2. The method of claim 1 , wherein heat treating comprises heating the precipitated silica material at a temperature of at least about 400° C. for at least about 8 hours.

3. The method of claim 1 , wherein heat treating comprises heating the precipitated silica material at a temperature of at least about 550° C. for at least about 8 hours.

4. The method of claim 1 , wherein the heat treated silica material has a metal concentration of from about 1 wt. % up to about 10 wt. %.

5. The method of claim 1 , wherein the precipitated silica material is prepared by contacting a silicate solution, an acidulating agent, and a soluble metal salt, wherein the soluble metal salt comprises a metal ion having a Mohs hardness value of at least 5.5 in its oxide form.

6. The method of claim 5 , wherein the metal ion comprises one or more of aluminum, tin, or a combination thereof.

7. The method of claim 5 , wherein the metal ion comprises aluminum.

8. The method of claim 5 , wherein the metal ion comprises tin.

9. A heat treated silica material prepared by the method of claim 1 .

10. A dentifrice composition comprising the heat treated silica material of claim 9 .

11. A method for preparing a dentifrice material, the method comprising heat treating a precipitated silica material comprising aluminum and/or tin at a temperature of from about 400° C. to about 900° C. to form a heat treated silica material, and then contacting the heat treated silica material with one or more dentifrice components to form the dentifrice material; wherein:

the heat treated silica material has a loss on ignition at 900° C. of less than about 3 wt. %, which wherein

an Einlehner abrasion value of the heat treated silica material is from about 90% to about 450% greater than an Einlehner abrasion value of the precipitated silica material.

12. The method of claim 11 , wherein heat treating comprises heating the precipitated silica material at a temperature of from about 400° C. to about 900° C. for at least about 8 hours.

13. The method of claim 11 , wherein heat treating comprises heating the precipitated silica material at a temperature of from about 550° C. to about 900° C. for at least about 8 hours.

14. A dentifrice material prepared by the method of claim 11 .

15. The method of claim 1 , wherein the precipitated silica material comprises silica particles.

16. The method of claim 1 , wherein the precipitated silica material comprises aluminosilicate particles.

17. The method of claim 1 , wherein the metal comprises aluminum, tin, or a combination thereof.

18. The method of claim 5 , wherein the metal salt comprises a sulfate, a nitrate, a phosphate, or a carbonate of aluminum or tin.

19. A precipitated silica material comprising from about 1 wt. % to about 10 wt. % of a metal having a Mohs hardness value of at least 5.5 in its oxide form, and wherein the precipitated silica material is characterized by:

a loss on ignition at 900° C. of less than about 3 wt. %; and

a pellicle cleaning ratio (PCR) at 20% loading of at least 90.

20. The silica material of claim 19 , wherein the metal comprises aluminum.

21. The silica material of claim 19 , wherein the metal comprises tin.

22. The silica material of claim 19 , wherein the precipitated silica material comprises aluminosilicate particles.

23. The silica material of claim 19 , wherein the precipitated silica material is further characterized by an Einlehner abrasion value in a range from 18 to 34.8 mg lost/100,000 revolutions.

24. A dentifrice composition comprising the silica material of claim 19 .

Assignments (4)
CHANGE OF NAME Recorded Dec 20, 2019
From: EVONIK DEGUSSA GMBH
To: EVONIK OPERATIONS GMBH
Reel/Frame 051382/0001 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Oct 25, 2017
From: J.M. HUBER CORPORATION
To: EVONIK DEGUSSA GMBH
Reel/Frame 043944/0334 →
RELEASE OF SECURITY INTEREST IN PATENTS Recorded Jun 27, 2014
From: WELLS FARGO BANK, NATIONAL ASSOCIATION
To: J.M. HUBER CORPORATION; CP KELCO U.S., INC.; HUBER ENGINEERED WOODS LLC
Reel/Frame 033247/0705 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jul 3, 2013
From: GALLIS, KARL W.; HAGAR, WILLIAM J.; MCGILL, PATRICK; NASSIVERA, TERRY W.
To: J.M. HUBER CORPORATION
Reel/Frame 030733/0216 →