IP Library Granted Patent US 9,663,708
Granted Patent B2
US 9,663,708 · App. 13/952,110 · Granted May 30, 2017

Synthetic proppants and monodispersed proppants and methods of making the same

Inventors: Robert D. Skala (Houston, TX); Christopher Y. Fang (Houston, TX); Christopher E. Coker (Houston, TX)
Assignee: Halliburton Energy Services, Inc.
C09K8/80C04B35/01C04B35/117C04B35/1115C04B35/14C04B35/16C04B35/18C04B35/185C04B35/19C04B35/195C04B35/26C04B35/443C04B35/515C04B35/56C04B35/58C04B35/62655C04B38/009C04B2235/3201C04B2235/3203C04B2235/3206C04B2235/3208C04B2235/3232C04B2235/3272C04B2235/3472C04B2235/36C04B2235/42C04B2235/528C04B2235/5296C04B2235/5436C04B2235/5445C04B2235/5481C04B2235/77C04B2235/784
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Quick Facts
Patent No.
US 9,663,708
App. No.
13/952,110
Granted
May 30, 2017
Kind
B2
Abstract

Synthetic ceramic proppants are described. Proppants having a monodispersity of 3-sigma distribution or lower are also described, including methods to make these proppants and methods of using these proppants.

Claims (21)

1. A proppant comprising a core and a shell on the core, wherein the proppant has a core strength to shell strength ratio of 0.8 to 1, wherein a plurality of micron particles are sintered together to form the core, the shell, or both the core and the shell, wherein the micron particles have a unimodal particle distribution, wherein total distribution of the micron particles has a width that is 5% or less than mean particle size of the micron particle, wherein the micron particles have a d 50 of 0.5 micron to 3.5 microns; wherein the proppant has a plurality of pores having a pore volume, wherein a majority of the pore volume results from interstitial gaps formed between the micron particles; wherein the proppant comprises:

a glassy phase present in an amount of at least 10% by weight of the proppant; and

ceramic whiskers having an average length from 1 micron to 3.5 microns, an average width from 0.1 to 0.3 and a whisker length distribution of about 8 or less.

2. The proppant of claim 1 , wherein the proppant is spherical and have a Krumbein sphericity of at least about 0.9 and/or a roundness of at least about 0.9.

3. The proppant of claim 1 , wherein the pore volume is from about 1% to 30% based upon the total volume of said proppant.

4. The proppant of claim 1 , wherein the pore volume is from about 5% to 20% based upon the total volume of said proppant.

5. The proppant of claim 1 , wherein said proppant has a specific gravity of from 0.8 to 4.

6. The proppant of claim 1 , wherein said proppant has a specific gravity of from about 1 to 3.5.

7. The proppant of claim 1 , wherein said proppant has a d 10 that is within 100% of the d 50 .

8. The proppant of claim 1 , wherein said proppant has a d 10 that is within 50% of the d 50 .

9. The proppant of claim 1 , wherein said proppant has a d 90 that is within 100% of the d 50 .

10. The proppant of claim 1 , wherein said proppant has a d 90 that is within 50% of the d 50 .

11. The proppant of claim 1 , wherein said proppant has a d 10 that is within 100% of the d 50 and has a d 90 that is within 100% of the d 50 .

12. The proppant of claim 1 , wherein said core comprises said plurality of micron particles that are sintered together.

13. The proppant of claim 1 , wherein said shell comprises a plurality of micron particles that are sintered together.

14. The proppant of claim 1 , wherein said proppant is in the absence of a binder.

15. The proppant of claim 1 , wherein said proppant is in the absence of a polymer.

16. The proppant of claim 1 , wherein the core comprises a plurality of micron particles that are sintered together, wherein said micron particles have a bimodal particle distribution with a modal A particle distribution and a modal B particle distribution.

17. The proppant of claim 16 , wherein said micron particles of each modal have a d 50 of 0.5 micron to 3.5 microns, and modal A has a d 50 that is at least 10% different from the d 50 of modal B.

18. The proppant of claim 16 , wherein said micron particles of each modal have a d 50 of 0.5 micron to 3.5 microns, and modal A has a d 50 that is at least 20% different from the d 50 of modal B.

19. The proppant of claim 16 , wherein said micron particles of each modal have a d 50 of 0.5 micron to 3.5 microns, and modal A has a d 50 that is from 10% to 100% different from the d 50 of modal B.

Assignments (4)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jul 23, 2015
From: OXANE MATERIALS, INC.
To: HALLIBURTON ENERGY SERVICES, INC.
Reel/Frame 036174/0785 →
RELEASE OF SECURITY INTEREST Recorded Jul 9, 2015
From: DELTA CENTAURI LLC
To: OXANE MATERIALS, INC.
Reel/Frame 036043/0665 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jun 4, 2015
From: SKALA, ROBERT D.; FANG, CHRISTOPHER Y.; COKER, CHRISTOPHER E.
To: OXANE MATERIALS, INC.
Reel/Frame 035783/0266 →
SECURITY INTEREST Recorded Dec 10, 2014
From: OXANE MATERIALS, INC.
To: DELTA CENTAURI LLC
Reel/Frame 034468/0045 →
Continuity (2)
Provisional Application 61678318 · Aug 1, 2012
Related Publication 20140038860A1 · Feb 6, 2014