IP Library Granted Patent US 9,782,542
Granted Patent B2
US 9,782,542 · App. 13/968,974 · Granted Oct 10, 2017

Self-lubricating pharmaceutical syringe stoppers

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Quick Facts
Patent No.
US 9,782,542
App. No.
13/968,974
Granted
Oct 10, 2017
Kind
B2
Abstract

In one aspect, a self-lubricating component is provided for a pharmaceutical packaging assembly. The self-lubricating component comprises a polymer composition and an effective amount of a lubricating additive such as, for example, boron nitride. In another aspect, a pharmaceutical packaging assembly may be provided having a surface thereof coated with a lubricating composition comprising boron nitride. The pharmaceutical packaging composition may be, for example, a pre-filled syringe comprising a body (barrel) and a plunger assembly.

Claims (23)

1. A self-lubricating component for a pharmaceutical packaging assembly comprising a polymer composition comprising:

a lubricating additive, wherein the lubricating additive comprises one or more of: boron nitride, graphite, molybdenum disulfide, talc, mica, colloidal silica, fumed silica, high molecular weight silicone gum, Reimer's salt, siloxane particles, vinylfluoro silicones, a salt, ester, or amide of a fatty acid, or any combination of two or more thereof;

wherein the polymer composition has a compression set of less than 20%.

2. The component of claim 1 in the form of a plunger, piston, diaphragm, or valve disc for medical equipment.

3. The component of claim 1 , wherein the lubricating additive is present in an amount of from about 0.1 to about 50% by weight of the polymer composition.

4. The component of claim 1 , wherein the lubricating additive is present in an amount of from about 5 to about 20% by weight of the polymer composition.

5. The component of claim 1 , wherein the lubricating additive is present in an amount of from about 10 to about 15% by weight of the polymer composition.

6. The component of claim 1 further comprising a reinforcing additive.

7. The component of claim 6 , wherein the reinforcing additive is chosen from carbon fiber, glass fiber, aramid fiber, a fibrous minerals, a vitreous fiber, a fumed metal oxide, or a combination of two or more thereof.

8. The component of claim 6 , comprising the reinforcing additive in an amount of from about 0.1 to about 20% by weight of the polymer composition.

9. The component of claim 1 , wherein the lubricating additive comprises hexagonal boron nitride.

10. The component of claim 6 , wherein the reinforcing additive is a high aspect filler having an aspect ratio of from about 10 to about 300.

11. The component of claim 10 , wherein the high aspect filler is chosen from a clay, an exfoliated clay, a graphite, an exfoliated graphite, graphene, exfoliated boron nitride, boron nitride nanosheets, a layered silicate, an aluminate, or a combination of two or more thereof.

12. The component of claim 10 , wherein the polymer composition comprises the high aspect filler in an amount of from about 1 vol % to about 70 vol %.

13. The component of claim 1 comprising a clay.

14. The component of claim 1 comprising a clay in an amount of from about .05 wt. % to about 10 wt. %.

15. The component of claim 1 wherein the polymer composition further comprises a hard filler.

16. The component of claim 15 wherein the hard filler is chosen from alumina, silica, titania, magnesia, zinc oxide, silicon carbide, silicon nitride, tungsten carbide, cubic boron nitride, aluminum nitride, or a combination of two or more thereof.

17. A self-lubricating component for a pharmaceutical packaging assembly wherein the self-lubricating component is formed by a polymer composition comprising:

a lubricating additive, wherein the lubricating additive comprises one or more of: boron nitride, graphite, molybdenum disulfide, talc, mica, colloidal silica, fumed silica, high molecular weight silicone gum, Reimer's salt, siloxane particles, vinylfluoro silicones, a salt, ester, or amide of a fatty acid, or any combination of two or more thereof;

wherein the polymer composition has a permeability of less than 500 barrers.

18. The component of claim 17 wherein the polymer composition further comprises a hard filler.

19. The component of claim 18 wherein the hard filler is chosen from alumina, silica, titania, magnesia, zinc oxide, silicon carbide, silicon nitride, tungsten carbide, cubic boron nitride, aluminum nitride, or a combination of two or more thereof.

Assignments (18)
PATENT SECURITY AGREEMENT Recorded May 23, 2025
From: MOMENTIVE PERFORMANCE MATERIALS QUARTZ, INC.
To: STANDARD CHARTERED BANK, AS COLLATERAL AGENT AND ADMINISTRATIVE AGENT
Reel/Frame 071368/0854 →
TERMINATION AND RELEASE OF SECURITY INTEREST IN PATENTS Recorded Mar 31, 2023
From: BNP PARIBAS
To: MOMENTIVE PERFORMANCE MATERIALS INC.
Reel/Frame 063259/0133 →
RELEASE OF SECURITY INTEREST Recorded Mar 30, 2023
From: KOOKMIN BANK NEW YORK
To: MOMENTIVE PERFORMANCE MATERIALS INC.
Reel/Frame 063197/0373 →
NUNC PRO TUNC ASSIGNMENT Recorded Feb 4, 2021
From: MOMENTIVE PERFORMANCE MATERIALS INC.
To: MOMENTIVE PERFORMANCE MATERIALS QUARTZ, INC.
Reel/Frame 055222/0140 →
RELEASE OF SECURITY INTEREST Recorded Nov 11, 2020
From: JPMORGAN CHASE BANK, N.A., AS COLLATERAL AGENT
To: MOMENTIVE PERFORMANCE MATERIALS INC.
Reel/Frame 054336/0023 →
ABL PATENT AGREEMENT Recorded Jun 5, 2019
From: MOMENTIVE PERFORMANCE MATERIALS INC.; MOMENTIVE PERFORMANCE MATERIALS GMBH
To: CITIBANK, N.A., AS ADMINISTRATIVE AGENT
Reel/Frame 049388/0252 →
SECOND LIEN TERM LOAN PATENT AGREEMENT Recorded Jun 5, 2019
From: MOMENTIVE PERFORMANCE MATERIALS INC.
To: KOOKMIN BANK, NEW YORK BRANCH, AS ADMINISTRATIVE AGENT
Reel/Frame 049388/0220 →
FIRST LIEN TERM LOAN PATENT AGREEMENT Recorded Jun 5, 2019
From: MOMENTIVE PERFORMANCE MATERIALS INC.
To: BNP PARIBAS, AS ADMINISTRATIVE AGENT
Reel/Frame 049387/0782 →
RELEASE OF SECURITY INTEREST Recorded May 15, 2019
From: BOKF, NA
To: MOMENTIVE PERFORMANCE MATERIALS INC.
Reel/Frame 049194/0085 →
RELEASE OF SECURITY INTEREST Recorded May 15, 2019
From: BOKF, NA
To: MOMENTIVE PERFORMANCE MATERIALS INC.
Reel/Frame 049249/0271 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded May 10, 2017
From: CONZONE, SAMUEL; RUSINKO, DAVID M.; RAMAN, CHANDRASHEKAR; RAMAKRISHNAN, INDUMATHI; DHANABALAN, ANANTHARAMAN; DUBEY, MAYANK KUMAR; BLEY, MARKUS; WINKELBACH, HANS RAFAEL
To: MOMENTIVE PERFORMANCE MATERIALS INC.
Reel/Frame 042318/0391 →
NOTICE OF CHANGE OF COLLATERAL AGENT - ASSIGNMENT OF SECURITY INTEREST IN INTELLECTUAL PROPERTY - SECOND LIEN Recorded Mar 6, 2015
From: THE BANK OF NEW YORK MELLON TRUST COMPANY, N.A. AS COLLATERAL AGENT
To: BOKF, NA, AS SUCCESSOR COLLATERAL AGENT
Reel/Frame 035137/0263 →
NOTICE OF CHANGE OF COLLATERAL AGENT - ASSIGNMENT OF SECURITY INTEREST IN INTELLECTUAL PROPERTY Recorded Mar 6, 2015
From: THE BANK OF NEW YORK MELLON TRUST COMPANY, N.A. AS COLLATERAL AGENT
To: BOKF, NA, AS SUCCESSOR COLLATERAL AGENT
Reel/Frame 035136/0457 →
TERMINATION AND RELEASE OF SECURITY INTEREST IN PATENT RIGHTS Recorded Nov 20, 2014
From: JPMORGAN CHASE BANK, N.A.
To: MOMENTIVE PERFORMANCE MATERIALS INC.
Reel/Frame 034410/0607 →
SECURITY INTEREST Recorded Oct 27, 2014
From: MOMENTIVE PERFORMANCE MATERIALS INC.
To: THE BANK OF NEW YORK MELLON TRUST COMPANY, N.A., AS COLLATERAL AGENT
Reel/Frame 034066/0570 →
SECURITY INTEREST Recorded Oct 27, 2014
From: MOMENTIVE PERFORMANCE MATERIALS INC.
To: THE BANK OF NEW YORK MELLON TRUST COMPANY, N.A., AS COLLATERAL AGENT
Reel/Frame 034066/0662 →
SECURITY INTEREST Recorded Apr 22, 2014
From: MOMENTIVE PERFORMANCE MATERIALS INC.
To: JPMORGAN CHASE BANK, N.A., AS COLLATERAL AGENT
Reel/Frame 032754/0774 →
SECURITY INTEREST Recorded Apr 22, 2014
From: MOMENTIVE PERFORMANCE MATERIALS INC.
To: JPMORGAN CHASE BANK, N.A., AS COLLATERAL AGENT
Reel/Frame 032736/0552 →