IP Library Granted Patent US 9,663,481
Granted Patent B2
US 9,663,481 · App. 14/016,442 · Granted May 30, 2017

Phenoxy acetic acids and phenyl propionic acids as PPARδ agonists

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Quick Facts
Patent No.
US 9,663,481
App. No.
14/016,442
Granted
May 30, 2017
Kind
B2
Abstract

Phenoxy acetic acids and phenyl propionic acids and their use in treating type I diabetes, type II diabetes, impaired glucose tolerance, insulin resistance, or obesity are provided herein. The present compounds are activators of PPARδ and may be useful for treating conditions mediated by the same.

Claims (44)

1. A method of arresting development of a disease-state, slowing development of a disease state, causing regression of a disease-state, or causing regression of a symptom of a disease-state, wherein the disease-state is type I diabetes, type II diabetes, impaired glucose tolerance, insulin resistance, or obesity, the method comprising administering to a subject in need thereof an effective amount of a compound according to formula (I) or a pharmaceutically acceptable salt thereof:

wherein is a double bond, with either E or Z substitution;

X 1 is C 1-6 -alkyl substituted with morpholino;

X 2 is phenylene;

X 3 is phenyl substituted with one or more halogens;

Ar is phenylene optionally substituted with methyl;

Y 1 is O;

Y 2 is O;

Z is CH 2 ;

R 1 is H; and

R 2 is H.

2. The method of claim 1 , wherein X 1 is morpholin-4-ylmethyl.

3. A method of arresting development of a disease-state, slowing development of a disease state, causing regression of a disease-state, or causing regression of a symptom of a disease-state, wherein the disease-state is type I diabetes, type II diabetes, impaired glucose tolerance, insulin resistance, or obesity, the method comprising administering to a subject in need thereof an effective amount of a compound selected from the group consisting of:

(E)-[4-[3-(4-Fluorophenyl)-3-[4-[3-(morpholin-4-yl)propynyl]phenyl]allyloxy]-2-methyl-phenoxy]acetic acid; and

(Z)-[4-[3-(4-Fluorophenyl)-3-[4-[3-(morpholin-4-yl)propynyl]phenyl]allyloxy]-2-methyl-phenoxy]acetic acid; or

a pharmaceutically acceptable salt thereof.

4. The method of claim 3 , wherein the compound is (E)-[4-[3-(4-Fluorophenyl)-3-[4-[3-(morpholin-4-yl)propynyl]phenyl]allyloxy]-2-methyl-phenoxy]acetic acid or a pharmaceutically acceptable salt thereof.

5. The method of claim 3 , wherein the compound is (Z)-[4-[3-(4-Fluorophenyl)-3-[4-[3-(morpholin-4-yl)propynyl]phenyl]allyloxy]-2-methyl-phenoxy]acetic acid or a pharmaceutically acceptable salt thereof.

6. A method of arresting development of a disease-state, slowing development of a disease state, causing regression of a disease-state, or causing regression of a symptom of a disease-state, wherein the disease-state is type I diabetes, type II diabetes, impaired glucose tolerance, insulin resistance, or obesity, the method comprising administering to a subject in need thereof an effective amount of a compound of formula (I) or a pharmaceutically acceptable salt thereof:

wherein is a double bond, with either E or Z substitution;

X 1 is C 1-6 alkyl substituted with morpholino;

X 2 is phenylene;

X 3 is phenyl substituted with one or more halogens;

Ar is phenylene optionally substituted with methyl;

Y 1 is O or S;

Y 2 is CH 2 ;

Z is —CH 2 —;

R 1 is hydrogen; and

R 2 is hydrogen.

7. The method of claim 6 , wherein X 1 is morpholin-4-ylmethyl.

8. The method of claim 6 , wherein the compound is (E)-[4-[3-(4-Chlorophenyl)-3-[4-[3-(morpholin-4-yl)propynyl]phenyl]allyloxy]-2-methylphenyl]-propionic acid or a pharmaceutically acceptable salt thereof.

9. The method of claim 6 , wherein the compound is (Z)-[4-[3-(4-Chlorophenyl)-3-[4-[3-(morpholin-4-yl)propynyl]phenyl]allyloxy]-2-methylphenyl]-propionic acid or a pharmaceutically acceptable salt thereof.

10. A method of arresting development of a disease-state, slowing development of a disease state, causing regression of a disease-state, or causing regression of a symptom of a disease-state, wherein the disease-state is type I diabetes, type II diabetes, impaired glucose tolerance, insulin resistance, or obesity, the method comprising administering to a subject in need thereof an effective amount of a compound of selected from the group consisting of:

(Z)-[2-Methyl-4-[3-(4-methylphenyl)-3-[4-[3-(morpholin-4-yl)propynyl]phenyl]allyloxy]-phenoxy]acetic acid;

(E)-[2-Methyl-4-[3-[4-[3-(pyrazol-1-yl)prop-1-ynyl]phenyl]-3-(4-trifluoromethylphenyl)-allyloxy]phenoxy]acetic acid;

(E)-[2-Methyl-4-[3-[4-[3-(morpholin-4-yl)propynyl]phenyl]-3-(4-trifluoromethylphenyl) allyloxy]-phenoxy]acetic acid;

(E)-[2-Methyl-4-[3-(4-methylphenyl)-3-[4-[3-(morpholin-4-yl)propynyl]phenyl]allyloxy]-phenoxy]acetic acid; and

(Z)-[2-Methyl-4-[3-[4-[3-(morpholin-4-yl)propynyl]phenyl]-3-(4-trifluoromethylphenyl) allyloxy]-phenoxy]acetic acid;

or a pharmaceutically acceptable salt thereof.

11. The method of claim 10 , wherein the compound is (Z)-[2-Methyl-4-[3-(4-methylphenyl)-3-[4-[3-(morpholin-4-yl)propynyl]phenyl]allyloxy]-phenoxy]acetic acid or a pharmaceutically acceptable salt thereof.

12. The method of claim 10 , wherein the compound is (E)-[2-Methyl-4-[3-[4-[3-(pyrazol-1-yl)prop-1-ynyl]phenyl]-3-(4-trifluoromethylphenyl)-allyloxy]phenoxy]acetic acid or a pharmaceutically acceptable salt thereof.

13. The method of claim 10 , wherein the compound is (E)-[2-Methyl-4-[3-[4-[3-(morpholin-4-yl)propynyl]phenyl]-3-(4-trifluoromethylphenyl)allyloxy]-phenoxy]acetic acid or a pharmaceutically acceptable salt thereof.

14. The method of claim 10 , wherein the compound is (E)-[2-Methyl-4-[3-(4-methylphenyl)-3-[4-[3-(morpholin-4-yl)propynyl]phenyl]allyloxy]-phenoxy]acetic acid or a pharmaceutically acceptable salt thereof.

15. The method of claim 10 , wherein the compound is (Z)-[2-Methyl-4-[3-[4-[3-(morpholin-4-yl)propynyl]phenyl]-3-(4-trifluoromethylphenyl) allyloxy]-phenoxy]acetic acid or a pharmaceutically acceptable salt thereof.

Assignments (9)
CORRECTIVE ASSIGNMENT TO CORRECT THE RECEIVING PARTY DATA PREVIOUSLY RECORDED AT REEL: 036254 FRAME: 0792. ASSIGNOR(S) HEREBY CONFIRMS THE ASSIGNMENT. Recorded Sep 24, 2015
From: M&F TTP HOLDINGS LLC, AS COLLATERAL AGENT
To: VTVX HOLDINGS II LLC
Reel/Frame 036675/0399 →
RELEASE OF SECURITY INTEREST Recorded Aug 3, 2015
From: M&F TTP HOLDINGS LLC, AS COLLATERAL AGENT
To: VTVX HOLDINGS I LLC
Reel/Frame 036254/0792 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jul 31, 2015
From: VTVX HOLDINGS II LLC
To: VTV THERAPEUTICS LLC
Reel/Frame 036242/0362 →
CHANGE OF NAME Recorded Jul 30, 2015
From: HIGH POINT PHARMACEUTICALS, LLC
To: VTVX HOLDINGS II LLC
Reel/Frame 036236/0159 →
SECURITY INTEREST Recorded Feb 26, 2015
From: HIGH POINT PHARMACEUTICALS, LLC
To: M&F TTP HOLDINGS LLC, AS COLLATERAL AGENT
Reel/Frame 035103/0029 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Sep 13, 2013
From: SAUERBERG, PER; PIHERA, PAVEL; POLIVKA, ZDENEK; HAVRANEK, MIROSLAV; PETTERSSON, INGRID; MOGENSEN, JOHN PATRICK
To: TRANSTECH PHARMA, INC.
Reel/Frame 031198/0548 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Sep 13, 2013
From: TRANSTECH PHARMA, INC.
To: HIGH POINT PHARMACEUTICALS, LLC
Reel/Frame 031198/0634 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Sep 13, 2013
From: NOVO NORDISK A/S
To: TRANSTECH PHARMA, INC.
Reel/Frame 031198/0865 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Sep 13, 2013
From: TRANSTECH PHARMA, INC.
To: HIGH POINT PHARMACEUTICALS, LLC
Reel/Frame 031199/0163 →