IP Library Granted Patent US 9,816,027
Granted Patent B2
US 9,816,027 · App. 14/110,916 · Granted Nov 14, 2017

Method for producing a film having luminescent particles

Inventors: Michael Labrot (Aachen, DE); Monique Elmer (Emsdetten, DE); Jean Sablayrolles (Crouy en Thelle, FR); Frederic Clabau (Paris, FR)
Assignee: SEKISUI CHEMICAL CO., LTD.
C09K11/06B29C47/786B29C47/802B29C47/827B32B17/10669B32B17/10779C09K9/02G02B27/0101B32B2457/20B32B2551/00C09K2211/1007C09K2211/1014G02B2027/0112Y10T428/31616
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Quick Facts
Patent No.
US 9,816,027
App. No.
14/110,916
Granted
Nov 14, 2017
Kind
B2
Abstract

A method for producing a film having luminescent particles is described. The method has steps a) mixing a thermoplastic and a luminescent pigment containing a hydroxyalkyl terephthalate of the formulate: R 1 —COO—P(OH)x-COO—R 2 and obtaining a thermoplastic mixture; and b) homogenizing the thermoplastic mixture to 150° C. to 200° C. in an extruder, by way of an extrusion nozzle, and obtaining a thermoplastic film.

Claims (13)

1. A method for producing a film having luminescent particles, comprising:

a. mixing a thermoplastic and a luminescent pigment containing a hydroxyalkyl terephthalate of the formula R 1 —COO—P(OH)x-COO—R 2 , thereby obtaining a thermoplastic mixture without a solvent, wherein the thermoplastic mixture contains 0.5 g to 8 g of luminescent pigment per kg of the thermoplastic,

wherein R 1 , R 2 is an alkyl, aryl, or allyl radical having 1 C to 10 C atoms, P is a phenyl ring, OH is a hydroxyl group bound to the phenyl ring, and x is an integer from 1 to 4, and

b. homogenizing the thermoplastic mixture in an extruder at 150° C. to 200° C., and obtaining a thermoplastic film via an extrusion nozzle of the extruder,

wherein the extruder is heated in an extruder intake comprising a first 20% of the length of the extruder screw to a temperature of 135° C. to 150° C., wherein the extruder is heated in an extruder middle to temperature of 150° C. to 170° C.,

wherein the extruder is heated in an extruder discharge comprising a last 20% of the length of the extruder screw to a temperature of 160° C. to 180° C., and

wherein the thermoplastic film is conveyed with an extrusion rate of 10 mm/s to 20 mm/s.

2. The method according to claim 1 , wherein the luminescent pigment contains diethyl 2,5-dihydroxyterephtalate.

3. The method according to claim 1 , wherein the luminescent pigment has an excitation maximum in a range from 380 nm to 420 nm and/or an emission maximum in a range from 430 nm to 500 nm.

4. The method according to claim 1 , wherein the luminescent pigment comprises benzopyranes, naphthopyranes, 2H-naphthopyranes, 3H-naphthopyranes, 2H-phenanthropyranes, 3H-phenanthropyranes, photochromic resins, coumarins, xanthines, naphthalinic acid derivatives, oxazoles, stilbenes, styryls, perylenes, lanthanides, preferably Y 2 O 3 :Eu, YVO 4 :Tm, Y 2 O 2 S:Pr, Gd 2 O 2 S:Tb, and/or mixtures thereof.

5. The method according to claim 1 , wherein the thermoplastic film is conveyed in the extruder via a single extruder screw.

6. The method according to claim 1 , wherein the thermoplastic film is conveyed in a thickness of 0.3 mm to 1 mm.

7. The method according to claim 6 , wherein the thickness is 0.76 mm.

Assignments (2)
SAINT-GOBAIN GLASS FRANCE TRANSFERS 100 PERCENT OF ITS RIGHTS TO SEKISUI CHEMICAL CO., LTD. Recorded Apr 3, 2017
From: SAINT-GOBAIN GLASS FRANCE
To: SEKISUI CHEMICAL CO., LTD.
Reel/Frame 041861/0378 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Dec 11, 2013
From: LABROT, MICHAEL; ELMER, MONIQUE; SABLAYROLLES, JEAN; CLABAU, FREDERIC
To: SAINT-GOBAIN GLASS FRANCE
Reel/Frame 031763/0086 →
Priority Claims (1)
EP 11162567 · Apr 15, 2011 · regional
Continuity (1)
Related Publication 20140218803A1 · Aug 7, 2014