IP Library Granted Patent US 9,318,274
Granted Patent B2
US 9,318,274 · App. 14/117,097 · Granted Apr 19, 2016

Fabrication of nano-structure electrodes for ultra-capacitor

Inventor: Qingkang Wang (Shanghai, CN)
Assignee: EMPIRE TECHNOLOGY DEVELOPMENT LLC
H01G11/36B82Y10/00B82Y40/00H01G11/24H01G11/26H01G11/30H01G11/86H01L28/87H01L28/91H01L29/0673H01L29/92Y02E60/13Y10T29/417
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Quick Facts
Patent No.
US 9,318,274
App. No.
14/117,097
Granted
Apr 19, 2016
Kind
B2
Abstract

Techniques described herein generally relate to the fabrication of ultra-capacitor. In one or more embodiments of the present disclosure, methods for fabricating an ultra-capacitor are described that may include preparing a substrate surface of a silicon wafer. The methods may further include etching one or more nano-structures on the substrate surface of the silicon wafer with a galvanic displacement process, and constructing electrodes for the ultra-capacitor from the silicon wafer with the one or more nano-structures.

Claims (34)

1. A method for constructing an electric double-layer ultra-capacitor, comprising:

preparing a substrate surface of a silicon wafer;

etching one or more nano-structures on the substrate surface of the silicon wafer with a galvanic displacement process, wherein the one or more nano-structures contain silicon nano-wires with a height-to-diameter ratio that is above a first predetermined threshold of about 100:1; and

constructing the double-layer ultra-capacitor using two wafer segments from the silicon wafer as two electrodes, wherein each of the wafer segments contain a respective subset of silicon nano-wires, the constructing comprising:

positioning the two wafer segments having their respective subset of nano-wires facing each other, wherein a distance between the two respective subsets of nano-wires is smaller than a second predetermined threshold of about 0.5 μm; and

configuring the two wafer segments as the two electrodes for the double-layer ultra-capacitor.

2. The method as recited in claim 1 , wherein the preparing the substrate surface of the silicon wafer comprises:

cleaning the surface of the silicon wafer with one or more of H 2 SO 4 /H 2 O 2 , acetone, ethanol, and/or de-ionized water; and

drying the silicon wafer.

3. The method as recited in claim 1 , wherein the silicon wafer is a mono-crystalline silicon wafer having an effective sheet resistance in a range from approximately 5 Ω/□ to approximately 10 Ω/□.

4. The method as recited in claim 1 , wherein the silicon wafer is a P-type highly doped wafer with an effective sheet resistance that is less than approximately 10 Ω/□.

5. The method as recited in claim 1 , wherein the galvanic displacement process comprises:

preparing an etchant for the galvanic displacement process, wherein the etchant has a mixing ratio of about 35 mM/L of silver nitrate (AgNO 3 ) and about 20% of hydrofluoric acid (HF).

6. The method as recited in claim 5 , wherein the etching with the galvanic displacement process further comprises:

placing the etchant inside a container;

immersing the silicon wafer in the container with the etchant; and

sealing the container.

7. The method as recited in claim 6 , wherein the etching with the galvanic displacement process further comprises:

maintaining the silicon wafer in the sealed container for an elapsed time of about 15 minutes or more.

8. The method as recited in claim 7 , wherein the etching with the galvanic displacement process further comprises:

removing the silicon wafer from the container;

cleaning the silicon wafer to provide a cleaned silicon wafer; and

removing residual etchant from the cleaned silicon wafer.

9. The method as recited in claim 5 , wherein etching with the galvanic displacement process further comprises:

immersing the silicon wafer in the etchant for an elapsed time of at least 15 minutes.

10. An electric double-layer ultra-capacitor, comprising:

a first electrode and a second electrode configured in cooperative operation, wherein

each of the first electrode and the second electrode have a respective nano-structure that contains a plurality of nano-wires with a height-to-diameter ratio that is above a first predetermined threshold of about 100:1,

the first electrode's nano-structure and the second electrode's nano-structure are configured to face each other, and

a distance between the first electrode's nano-structure and the second electrode's nano-structure is smaller than a second predetermined threshold of about 0.5 μm.

11. The electric double-layer ultra-capacitor as recited in claim 10 , wherein the first electrode's nano-structure and the second electrode's nano-structure are constructed based on a highly-doped silicon wafer with a sheet resistance that is less than about 10 Ω/□.

12. The electric double-layer ultra-capacitor as recited in claim 10 , wherein the plurality of nano-wires are silicon-based.

13. The electric double-layer ultra-capacitor as recited in claim 10 , wherein the first electrode's nano-structure and the second electrode's nano-structure are constructed using a galvanic displacement process.

14. The electric double-layer ultra-capacitor as recited in claim 13 , wherein the first electrode's nano-structure and the second electrode's nano-structure are etched from silicon substrates by the galvanic displacement process.

Assignments (4)
RELEASE OF SECURITY INTEREST IN PATENTS, RECORDED ON JANUARY 29, 2019 AT REEL 048373 FRAME 0217 Recorded Sep 22, 2025
From: CRESTLINE DIRECT FINANCE, L.P., AS COLLATERAL AGENT
To: EMPIRE TECHNOLOGY DEVELOPMENT LLC
Reel/Frame 072936/0464 →
SECURITY INTEREST Recorded Jan 29, 2019
From: EMPIRE TECHNOLOGY DEVELOPMENT LLC
To: CRESTLINE DIRECT FINANCE, L.P.
Reel/Frame 048373/0217 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Nov 12, 2013
From: WANG, QINGKANG
To: SHANGHAI JIAO TONG UNIVERSITY
Reel/Frame 031582/0603 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Nov 12, 2013
From: SHANGHAI JIAO TONG UNIVERSITY
To: EMPIRE TECHNOLOGY DEVELOPMENT LLC
Reel/Frame 031582/0675 →
Continuity (1)
Related Publication 20140347786A1 · Nov 27, 2014