IP Library Granted Patent US 9,233,986
Granted Patent B2
US 9,233,986 · App. 14/233,085 · Granted Jan 12, 2016

Method for producing hydrophobic, heat-insulating mouldings

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Quick Facts
Patent No.
US 9,233,986
App. No.
14/233,085
Granted
Jan 12, 2016
Kind
B2
Abstract

Process for hydrophobizing a microporous thermal insulation molding comprising hydrophilic silica, in which the molding is treated with at least one organosilane and in which one or more organosilanes which are gaseous under the reaction conditions are introduced into a chamber containing the microporous thermal insulation molding comprising hydrophilic silica until the pressure difference Δp is ≧20 mbar.

Claims (30)

1. A process for hydrophobizing a molding, the method comprising:

perforating a microporous thermal insulation molding comprising hydrophilic silica, to obtain a perforated, microporous molding; and

treating the perforated, microporous molding with at least one organosilane in a chamber, thereby obtaining a hydrophobized molding,

wherein:

the at least one organosilane is gaseous under said treating and is introduced into the chamber until a pressure difference Δp is ≧20 mbar, wherein Δp=p2−p1, where p1=pressure in the chamber before introduction of the organosilane, p2=pressure in the chamber at which the introduction of the organosilane is stopped.

2. The process of claim 1 , wherein pressure p1 is less than atmospheric pressure.

3. The process of claim 1 , wherein pressure p1 is atmospheric pressure or above.

4. The process of claim 1 , wherein the molding comprises at least one of a pyrogenic silica and a silicon dioxide aerogel as the hydrophilic silica.

5. The process of claim 1 , wherein the at least one organosilane is selected from the group consisting of R n —Si—X 4-n , R 3 Si—Y—SiR 3 , R n Si n O n , (CH 3 ) 3 —Si—(O—Si(CH 3 ) 2 ) n —OH, and HO—Si(CH 3 ) 2 —(O—Si(CH 3 ) 2 ) n —OH,

where

n is a number of from 1 to 8;

R is —H, —CH 3 , or —C 2 H 5 ;

X is —Cl, —Br; —OCH 3 , —OC 2 H 5 , or —OC 3 H 8 ; and

Y is NH, or O.

6. The process of claim 1 , wherein the at least one organosilane is introduced in liquid or vapor form into the chamber.

7. The process of claim 1 , wherein at least one of water, an alcohol, and a hydrogen halide is introduced simultaneously with or subsequently to the at least one organosilane.

8. The process of claim 1 , wherein the molding further comprises at least one of an opacifier, a fiber, and a finely divided inorganic additive.

9. The process of claim 8 , wherein the molding comprises:

45-95% by weight of at least one of pyrogenic silicon dioxide and silicon dioxide aerogel,

5-20% by weight of the opacifier,

5-35% by weight of the finely divided inorganic additive, and

0-12% by weight of the fiber.

10. The process of claim 1 , wherein said treating occurs at a temperature of from 20 to 300° C.

11. The process of claim 1 , wherein the molding is left in the chamber for from 1 minute to 1 hour before introducing the at least one organosilane.

12. The process of claim 1 , wherein the perforation is carried out by needling.

13. the process of claim 12 , wherein the needling is carried out with needle grippers during actual pressing of the thermal insulation molding.

14. The process of claim 1 , wherein the hole depth of the perforations is about 2/3 of the thickness of the thermal insulation molding comprising hydrophilic silica.

15. The process of claim 1 , wherein the perforations are in the form of a channel having a diameter in the range of 0.1 mm to 3.0 mm.

16. The process of claim 1 , wherein the pressure difference Δp is greater than or equal to 100 mbar and less than or equal to 500 mbar.

17. The process of claim 1 , wherein the pressure difference Δp is greater than or equal to 200 mbar and less than or equal to 400 mbar.

Assignments (3)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Aug 1, 2023
From: EVONIK OPERATIONS GMBH
To: KINGSPAN INSULATION LIMITED
Reel/Frame 064447/0565 →
CHANGE OF NAME Recorded Jan 31, 2020
From: EVONIK DEGUSSA GMBH
To: EVONIK OPERATIONS GMBH
Reel/Frame 051765/0166 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jan 15, 2014
From: KRATEL, GUENTER; BORCHERT, GERD; MENZEL, FRANK
To: EVONIK DEGUSSA GMBH
Reel/Frame 031977/0752 →