IP Library Granted Patent US 9,464,219
Granted Patent B2
US 9,464,219 · App. 14/351,701 · Granted Oct 11, 2016

Method for increasing the reactivity of lignin

Inventors: Suvi Pietarinen (Lappeenranta, FI); Okko Ringena (Neusass, DE); Kati Eskelinen (Imatra, FI); Sanna Valkonen (Augsburg, DE)
Assignee: UPM-Kymmene Corporation
C09J197/005C08G8/20C08G8/24C08H6/00C08L97/005C08L97/02C09J161/12C07G1/00
View Patent ↗
Loading inventors, assignments & file history…
Monitor This Case
Get email alerts when status or documents change.
Order Certified Copies
Most orders are placed with the USPTO same day — all within 24 business hours.
Order via The Patent Place →
Pre-filled with this patent's details
Quick Facts
Patent No.
US 9,464,219
App. No.
14/351,701
Granted
Oct 11, 2016
Kind
B2
Abstract

The present invention relates to a method for increasing the reactivity of lignin, wherein the method comprises the following steps: a) forming, under heating at a temperature of 30-70° C., an aqueous dispersion comprising alkali and lignin, wherein the alkali comprises a hydroxide of an alkali metal; and b) heating the dispersion formed in step a) at a temperature of 50-95° C. for producing alkalated lignin.

Claims (20)

1. A method for increasing the reactivity of lignin, wherein the method comprises the following steps:

a) forming, under heating at a temperature of 30-70° C., an aqueous dispersion consisting of alkali and lignin and water, wherein the alkali comprises a hydroxide of an alkali metal, and wherein the concentration of the lignin is 10-50 weight-% based on the total weight of the aqueous dispersion in step a); and

b) heating the aqueous dispersion formed in step a) at a temperature of 50-95° C. thereby producing alkalated lignin, wherein the alkalated lignin has increased reactivity relative to the lignin.

2. The method of claim 1 , wherein the concentration of alkali is 5-50 weight-% based on the total weight of the aqueous dispersion in step a).

3. The method of claim 1 , wherein the concentration of the lignin is 20-50 weight-%, based on the total weight of the aqueous dispersion in step a).

4. The method of claim 1 , wherein the temperature in step a) is 50-65° C.

5. The method of claim 1 , wherein the temperature in step b) is 60-75° C.

6. The method of claim 1 , wherein step b) is carried out for 15 minutes-24 hours.

7. The method of claim 1 , wherein the method comprises, before step a), a step i) of reacting the lignin with a compound selected from the class of phenols.

8. The method of claim 7 , wherein step i) is carried out at a temperature of 100-140° C. for 1-3 hours in the presence of a catalyst.

9. The method of claim 1 , wherein the method comprises, after step b), a step ii) of adding an aldehyde to the aqueous dispersion formed in step b).

10. The method of claim 9 , wherein the weight ratio of the aldehyde to the lignin in the aqueous dispersion from step b) is 0.2-0.7.

11. The method of claim 9 , wherein the aldehyde is formaldehyde.

12. The method of claim 1 , wherein the concentration of alkali is 10-25 weight-% based on the total weight of the aqueous dispersion in step a).

13. The method of claim 1 , wherein the concentration of the lignin is 20-45-weight-% based on the total weight of the aqueous dispersion in step a).

14. The method of claim 1 , wherein step b) is carried out for no longer than 5 hours.

15. The method of claim 1 , wherein step b) is carried out for 0.5-1.5 hours.

16. The method of claim 9 , wherein the weight ratio of the aldehyde to the lignin in the aqeuous dispersion from step b) is 0.3-0.6.

17. The method of claim 1 , wherein the alkalated lignin is a product, and the alkalated lignin product is added to a subsequent reaction process.

18. The method of claim 17 , wherein the subsequent reaction process comprises binder production.

Assignments (1)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Oct 23, 2014
From: PIETARINEN, SUVI; RINGENA, OKKO; ESKELINEN, KATI; VALKONEN, SANNA
To: UPM-KYMMENE CORPORATION
Reel/Frame 034020/0558 →
Priority Claims (1)
FI 20125358 · Mar 29, 2012 · national
Continuity (1)
Related Publication 20140249271A1 · Sep 4, 2014