IP Library Granted Patent US 9,346,735
Granted Patent B2
US 9,346,735 · App. 14/356,168 · Granted May 24, 2016

Method for producing

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Quick Facts
Patent No.
US 9,346,735
App. No.
14/356,168
Granted
May 24, 2016
Kind
B2
Abstract

A method for efficiently producing t-butanol as a raw material of a methacrylic resin from isobutanol is described, including a step (1) of dehydrating isobutanol to obtain butenes, and a step (2) of hydrating the butenes to obtain t-butanol. A method for producing methacrolein and methacrylic acid is also described, which further includes a step (3) of dehydrating and oxidizing the obtained t-butanol to obtain methacrolein and methacrylic acid. An apparatus for performing the steps (1) to (3) is also described.

Claims (15)

1. A method for producing methacrolein and methacrylic acid, the method comprising:

a step (1) of dehydrating isobutanol derived from biomass to obtain butenes containing more than 55 mass % of isobutylene;

a step (2) of hydrating the butenes obtained from the step (1) to obtain t-butanol; and

a step (3) of dehydrating and oxidizing the t-butanol obtained from the step (2) to obtain methacrolein and methacrylic acid.

2. The method according to claim 1 , wherein an acid catalyst is used as a dehydration catalyst in the step (1).

3. The method according to claim 2 , wherein the acid catalyst includes alumina, silica alumina, solid phosphate, titania, or zirconia.

4. The method according to claim 1 , wherein an acid catalyst is used as a hydration catalyst in the step (2).

5. The method according to claim 4 , wherein the acid catalyst includes an ion exchange resin or heteropolyacid.

6. The method according to claim 1 , wherein an oxide including at least molybdenum, bismuth, and iron is used as an oxidation catalyst in the step (3).

7. An apparatus for producing methacrolein and methacrylic acid, comprising:

a device (A) for dehydrating isobutanol derived from biomass to obtain butenes containing more than 55 mass % of isobutylene;

a device (B) for hydrating the butenes obtained by the device (A), using an ion exchange resin as a hydration catalyst, to obtain t-butanol; and

a device (C) for dehydrating and oxidizing t-butanol obtained by the device (B) to obtain methacrolein and methacrylic acid.

8. A method for synthesizing methyl methacrylate, comprising:

obtaining methacrylic acid by the method according to claim 1 , and reacting the obtained methacrylic acid with methanol.

Assignments (2)
CHANGE OF NAME Recorded Sep 5, 2017
From: MITSUBISHI RAYON CO., LTD.
To: MITSUBISHI CHEMICAL CORPORATION
Reel/Frame 043750/0834 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded May 6, 2014
From: OOYACHI, KEN; YASUKAWA, TOSHIYA; AKIHARA, SHUJI
To: MITSUBISHI RAYON CO., LTD.
Reel/Frame 032835/0061 →