IP Library Granted Patent US 9,528,033
Granted Patent B2
US 9,528,033 · App. 14/541,112 · Granted Dec 27, 2016

Electrolyte material composition and method

Inventors: Theodore F. Cyman, Jr. (Grand Island, NY); Kevin J. Hook (Grand Island, NY); Pamela Geddes (Alden, NY); Alan R. Murzynowski (Grand Island, NY); James W. Blease (Avon, NY); Daniel E. Kanfoush (Grand Island, NY)
Assignee: R.R. Donnelley & Sons Company
C09J133/14B05B1/02B05B15/06B32B37/1284C08K5/01C09D11/10C09D11/106C09D11/324C09D11/36C09D11/38C09D11/52C09J5/00C09J5/06C09J131/04H01B3/00H01B3/306H01B3/421H01B3/441H01B3/447H01M2/145H01M4/0402H01M4/0404H01M4/0411H01M4/0414H01M4/0419H01M4/0435H01M4/08H01M4/12H01M4/131H01M4/133H01M4/134H01M4/1395H01M4/364H01M4/382H01M4/622H01M4/625H01M6/181H01M6/188H01M6/40H01M10/0436H01M10/0525H01M10/0565H01M4/1391H01M4/505H01M10/0454H01M10/052H01M10/0583H01M2004/027H01M2300/0082Y02E60/122Y02P70/54Y10T156/10
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Quick Facts
Patent No.
US 9,528,033
App. No.
14/541,112
Granted
Dec 27, 2016
Kind
B2
Abstract

The electrolyte material includes a polymer, a salt, and a solvent. The electrolyte material has a viscosity in the range from about 3.0 cP to about 20.0 cP such that the electrolyte material can be applied to a substrate using an ink jet print head.

Claims (32)

1. An electrolyte material comprising a polymer, a salt, and a solvent, wherein the electrolyte material has a viscosity in the range from about 3.0 to 8.0 cP such that the electrolyte material can be applied to a surface in a layer using an ink jet print head, wherein the polymer is present in an amount ranging from about 0.5% to about 2.5% by weight, and wherein the solvent is present in the amount ranging from about 95.0% to about 98.0% by weight.

2. The electrolyte material of claim 1 , wherein the polymer comprises a polyimide.

3. The electrolyte material of claim 1 , wherein the salt comprises lithium.

4. The electrolyte material of claim 1 , further comprising a surface tension modifier.

5. The electrolyte material of claim 1 , further comprising a co-solvent.

6. The electrolyte material of claim 1 , further comprising a device for use in an ink jet print operation comprising:

a housing;

a series of ejection nozzles mounted within the housing, each ejection nozzle capable of ejecting a drop on demand; and

a source of the electrolyte material communicating with the nozzles.

7. The electrolyte material of claim 1 , wherein the polymer is present in an amount ranging from about 1% to about 1.5% by weight.

8. The electrolyte material of claim 1 , wherein the solvent is selected from the group consisting of gamma butyrolactone, n-methyl-pyrrolidone, n-gamma valerolactone, N-methyl-2-pyrrolidinone, 3-methyl-oxazolidinone, tetramethylurea, dimethylsulfoxide, dimethylformamide, dimethylacetamide, methylethylketone, methyl isobutyl ketone, ethylene carbonate, propylene carbonate, dimethylcarbonate, ethylmethylcarbonate, diethylcarbonate, dimethoxyethane, dimethoxymethane, diethoxyethane, tetrahydrofuran, 2-methyl-tetrahydrofuran, 1,3-dioxolane, 4-methyl-1,3-dioxolane, 2-methyl-1,3-dioxolane, acetonitrile, methylacetate, ethylacetate, methyl butyrate, ethyl butyrate or any polar aprotic solvent and mixtures thereof.

9. The electrolyte material of claim 8 , wherein the solvent comprises gamma butyrolactone.

10. The electrolyte material of claim 1 , wherein the layer has a thickness in the range of from about 10 micrometers to about 30 micrometers.

11. The electrolyte material of claim 10 , wherein the layer has a thickness in the range of from about 16 micrometers to about 22 micrometers.

12. The electrolyte material of claim 1 , wherein the surface comprises one of a substrate and an intermediate layer disposed atop the substrate.

13. The electrolyte material of claim 12 , wherein the intermediate layer comprises one of an adhesive material, a cathode material, an anode material, or an insulating material.

14. An electrolyte adapted to be applied using an ink jet print head, comprising:

from about 0.5% to about 2.5% by weight of a polymer;

a lithium salt; and

from about 95.0% to about 98.0% by weight of a solvent;

wherein the electrolyte has a viscosity in the range from about 3.0 to 8.0 cP such that the electrolyte can be jetted by the ink jet print head.

15. The electrolyte of claim 14 , wherein the electrolyte has a dynamic surface tension in the range from about 30 dynes/cm to about 50 dynes/cm.

16. The electrolyte of claim 14 , wherein the polymer is present in an amount ranging from about 1% to about 1.5% by weight.

17. A method of manufacturing a battery using an ink jet print head comprising the steps of:

jetting an electrolyte material onto a substrate, wherein the electrolyte material comprises a polymer, a salt, and a solvent, wherein the electrolyte material has a viscosity in the range from about 3.0 to 8.0 cP such that the electrolyte material can be applied to a surface in a layer using an ink jet print head, wherein the polymer is present in an amount ranging from about 0.5% to about 2.5% by weight, and wherein the solvent is present in the amount ranging from about 95.0% to about 98.0% by weight; and

vaporizing a portion of the solvent.

18. The method of claim 17 , wherein the substrate is heated to promote vaporization of the solvent.

19. The method of claim 17 , wherein the electrolyte material forms a layer having a thickness in the range of from about 10 micrometers to about 30 micrometers.

20. The method of claim 19 , wherein the thickness is in the range of from about 18 micrometers to about 22 micrometers.

21. The method of claim 17 , wherein the electrolyte material is jetted from an ink jet print head, and the method further comprises relative movement of the ink jet print head over the substrate more than once to form a layer thereon.

22. The method of claim 21 , wherein the relative movement includes up to 50 passes.

23. The method of claim 22 , wherein the relative movement includes between 20 and 30 passes.

Assignments (19)
INTELLECTUAL PROPERTY ASSIGNMENT AGREEMENT Recorded Apr 22, 2025
From: WELLS FARGO BANK, NATIONAL ASSOCIATION
To: BANK OF AMERICA, N.A.
Reel/Frame 070919/0394 →
PATENT SECURITY AGREEMENT Recorded Aug 9, 2024
From: R. R. DONNELLEY & SONS COMPANY; CONSOLIDATED GRAPHICS, INC.; VALASSIS COMMUNICATIONS, INC.; VALASSIS DIGITAL CORP.; VALASSIS DIRECT MAIL, INC.
To: U.S. BANK TRUST COMPANY, NATIONAL ASSOCIATION
Reel/Frame 068534/0447 →
PATENT SECURITY AGREEMENT Recorded Aug 9, 2024
From: R. R. DONNELLEY & SONS COMPANY; CONSOLIDATED GRAPHICS, INC.; VALASSIS COMMUNICATIONS, INC.; VALASSIS DIGITAL CORP.; VALASSIS DIRECT MAIL, INC.
To: U.S. BANK TRUST COMPANY, NATIONAL ASSOCIATION
Reel/Frame 068534/0366 →
TERMINATION AND RELEASE OF SECURITY INTEREST IN PATENT RIGHTS (R/F 064463/0597) Recorded Aug 9, 2024
From: U.S. BANK TRUST COMPANY, NATIONAL ASSOCIATION
To: R. R. DONNELLEY & SONS COMPANY; CONSOLIDATED GRAPHICS, INC.
Reel/Frame 068534/0330 →
TERMINATION AND RELEASE OF SECURITY INTEREST IN PATENT RIGHTS (R/F 064462/0445) Recorded Aug 9, 2024
From: U.S. BANK TRUST COMPANY, NATIONAL ASSOCIATION
To: R. R. DONNELLEY & SONS COMPANY; CONSOLIDATED GRAPHICS, INC.
Reel/Frame 068534/0306 →
PATENT SECURITY AGREEMENT Recorded Aug 9, 2024
From: R. R. DONNELLEY & SONS COMPANY; CONSOLIDATED GRAPHICS, INC.; VALASSIS DIGITAL CORP.; VALASSIS DIRECT MAIL, INC.; VALASSIS COMMUNICATIONS, INC.
To: APOLLO ADMINISTRATIVE AGENCY LLC
Reel/Frame 068533/0812 →
RELEASE OF SECURITY INTEREST Recorded Jul 22, 2024
From: APOLLO ADMINISTRATIVE AGENCY LLC, AS ADMINISTRATIVE AGENT
To: R.R. DONNELLEY & SONS COMPANY; CONSOLIDATED GRAPHICS, INC.
Reel/Frame 068467/0314 →
RELEASE OF SECURITY INTEREST RECORDED AT RF 056122/0839; ASSIGNED VIA RF 059203/0333 TO JEFFERIES AND RF 063487/0449 TO APOLLO Recorded Apr 17, 2024
From: APOLLO ADMINISTRATIVE AGENCY LLC
To: R.R. DONNELLEY & SONS COMPANY
Reel/Frame 067131/0845 →
SECURITY INTEREST Recorded Apr 3, 2024
From: R. R. DONNELLEY & SONS COMPANY; CONSOLIDATED GRAPHICS, INC.
To: APOLLO ADMINISTRATIVE AGENCY LLC, AS ADMINISTRATIVE AGENT
Reel/Frame 067000/0669 →
PATENT SECURITY AGREEMENT Recorded Aug 1, 2023
From: R.R. DONNELLEY & SONS COMPANY; CONSOLIDATED GRAPHICS, INC.
To: U.S. BANK TRUST COMPANY, NATIONAL ASSOCIATION, AS 2028 NOTES COLLATERAL AGENT
Reel/Frame 064463/0597 →
PATENT SECURITY AGREEMENT Recorded Aug 1, 2023
From: R.R. DONNELLEY & SONS COMPANY; CONSOLIDATED GRAPHICS, INC.
To: U.S. BANK TRUST COMPANY, NATIONAL ASSOCIATION, AS NOTES COLLATERAL AGENT
Reel/Frame 064462/0445 →
TERMINATION AND RELEASE OF SECURITY INTEREST IN PATENTS, PREVIOUSLY RECORDED AT REEL 056079, FRAME 0534 Recorded Jul 31, 2023
From: U.S. BANK NATIONAL ASSOCIATION, AS COLLATERAL AGENT
To: R. R. DONNELLEY & SONS COMPANY; CONSOLIDATED GRAPHICS, INC.
Reel/Frame 064441/0646 →
ASSIGNMENT OF SECURITY INTEREST IN INTELLECTUAL PROPERTY COLLATERAL RECORDED AT REEL/FRAME 056122/0839 AND 059203/0333 Recorded Apr 28, 2023
From: JEFFERIES FINANCE LLC
To: APOLLO ADMINISTRATIVE AGENCY LLC
Reel/Frame 063487/0449 →
INTELLECTUAL PROPERTY ASSIGNMENT AGREEMENT Recorded Feb 10, 2023
From: BANK OF AMERICA, N.A.
To: WELLS FARGO BANK, NATIONAL ASSOCIATION
Reel/Frame 062702/0648 →
ASSIGNMENT OF SECURITY INTEREST IN INTELLECTUAL PROPERTY COLLATERAL RECORDED AT R/F 056122/0839 Recorded Feb 25, 2022
From: BANK OF AMERICA, N.A.
To: JEFFERIES FINANCE LLC
Reel/Frame 059203/0333 →
SECURITY INTEREST Recorded May 3, 2021
From: R. R. DONNELLEY & SONS COMPANY
To: BANK OF AMERICA, N.A.
Reel/Frame 056122/0810 →
SECURITY INTEREST Recorded May 3, 2021
From: R. R. DONNELLEY & SONS COMPANY
To: BANK OF AMERICA, N.A.
Reel/Frame 056122/0839 →
SECURITY INTEREST Recorded Apr 28, 2021
From: R. R. DONNELLEY & SONS COMPANY; CONSOLIDATED GRAPHICS, INC.
To: U.S. BANK NATIONAL ASSOCIATION
Reel/Frame 056079/0534 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jan 28, 2016
From: CYMAN, THEODORE F., JR.; HOOK, KEVIN J.; GEDDES, PAMELA; MURZYNOWSKI, ALAN R.; BLEASE, JAMES W.; KANFOUSH, DANIEL
To: R.R. DONNELLEY & SONS COMPANY
Reel/Frame 037612/0853 →
Continuity (7)
Provisional Application 61903816 · Nov 13, 2013
Provisional Application 61903829 · Nov 13, 2013
Provisional Application 61903819 · Nov 13, 2013
Provisional Application 61905697 · Nov 18, 2013
Provisional Application 61903846 · Nov 13, 2013
Provisional Application 61903859 · Nov 13, 2013
Related Publication 20150140442A1 · May 21, 2015