IP Library Granted Patent US 9,108,858
Granted Patent B2
US 9,108,858 · App. 14/546,170 · Granted Aug 18, 2015

Nanofilaments of catalytic materials for chemical process improvements

Inventors: John McDonald (West Monroe, LA); Chester Wilson (Ruston, LA); Joshua Brown (West Monroe, LA)
Assignee: Louisiana Tech University Research Foundation; a Division of Louisiana Tech University Foundation
C01C1/0411B01J12/007B01J19/006B01J19/24B01J19/249B01J23/462B01J23/745B01J23/75B01J35/006B01J37/341B01J37/348C07C1/0455C10G2/33C10G2/332C25D5/18C25D11/045C25D11/20B01J2219/0009B01J2219/00063B01J2219/00162B01J2219/00777B01J2219/248B01J2219/2479C25D3/12C25D5/006C25D11/08C25D11/12H01M10/052H01M12/08
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Quick Facts
Patent No.
US 9,108,858
App. No.
14/546,170
Granted
Aug 18, 2015
Kind
B2
Abstract

A Haber-Bosch process including the steps of providing a reactor having a substrate with catalyst filaments formed thereon. The catalyst filaments are formed of a metal including iron. A nitrogen compound and hydrogen are injected into the reactor such that at least a portion of the nitrogen compound and hydrogen contact the catalyst filaments. The nitrogen compound and hydrogen are reacted with the catalyst filaments at a temperature of less than about 600° F. and a pressure of less than about 2000 psig.

Claims (13)

1. A Haber-Bosch process comprising the steps of:

(a) providing a reactor including substrate elements having catalyst filaments formed on the substrates elements, the catalyst filaments comprising (i) a diameter of about 10 nm to about 500 nm; (ii) a length of about 30 nm to about 5000 nm; (iii) a packing density of between 5 mg/cm2 and about 200 mg/cm2; and (iv) being formed of a metal including iron;

(b) injecting a nitrogen compound and hydrogen into the reactor such that at least a portion of the nitrogen compound and hydrogen contact the catalyst filaments;

(c) reacting the nitrogen compound and hydrogen with the catalyst filaments at a temperature of less than about 600° F. and a pressure of less than about 2000 psig.

2. The process according to claim 1 , wherein the nitrogen compound is N2.

3. The process according to claim 1 , wherein the catalyst filaments comprise either iron or iron with osmium layers.

4. The process according to claim 1 , wherein the reaction pressure is less than about 1250 psig.

5. The process according to claim 1 , wherein the reaction pressure is less than about 1000 psig and the reaction temperature is between about 250° F. and about 450° F.

6. The process according to claim 1 , wherein the substrate elements are substantially nonporous.

7. The process according to claim 1 , wherein the filaments packing density is at least about 20 mg/cm2.

8. The process according to claim 1 , wherein the substrate elements are formed of a conductive material.

9. The process according to claim 1 , wherein the substrate elements are a nonconductive material with a layer of conductive material applied thereto.

10. The process according to claim 1 , wherein the catalyst filaments have a diameter between about 10 nm to about 200 nm.

Assignments (2)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Feb 3, 2016
From: LOUISIANA TECH UNIVERSITY RESEARCH FOUNDATION, A DIVISION OF LOUISIANA TECH UNIVERSITY FOUNDATION, INC.
To: LOUISIANA TECH RESEARCH CORPORATION
Reel/Frame 037653/0323 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded May 8, 2015
From: WILSON, CHESTER; MCDONALD, JOHN; BROWN, JOSHUA
To: LOUISIANA TECH UNIVERSITY RESEARCH FOUNDATION; A DIVISION OF LOUISIANA TECH UNIVERSITY FOUNDATION, INC.
Reel/Frame 035592/0564 →
Continuity (5)
Continuation 14151560 · Jan 9, 2014
Continuation 13722613 · Dec 20, 2012
Continuation In Part 12726106 · Mar 17, 2010
Provisional Application 61160949 · Mar 17, 2009
Related Publication 20150071843A1 · Mar 12, 2015