IP Library Granted Patent US 9,266,825
Granted Patent B2
US 9,266,825 · App. 14/616,715 · Granted Feb 23, 2016

Copolymers of isocyanatoalkyltrialkoxysilanes and urethanediols

View Patent ↗
Loading inventors, assignments & file history…
Monitor This Case
Get email alerts when status or documents change.
Order Certified Copies
Most orders are placed with the USPTO same day — all within 24 business hours.
Order via The Patent Place →
Pre-filled with this patent's details
Quick Facts
Patent No.
US 9,266,825
App. No.
14/616,715
Granted
Feb 23, 2016
Kind
B2
Abstract

The present invention relates to a copolymer of the formula where A, B, and D are independently of one another an aliphatic (cyclo)alkylene radical, R is a C 1 -C 10 alkyl radical, and 3≦x≦10. The present invention also relates to a process for preparing the copolymer, to its use and also to a coating composition and a coating formulation containing the copolymer.

Claims (33)

1. A copolymer of formula

where

A, B, D are independently an aliphatic (cyclo)alkylene radical,

R is a C 1 -C 10 alkyl radical, and

3≦x≦10.

2. The copolymer according to claim 1 , wherein each A is independently a linear C 1 -C 10 alkylene radical.

3. The copolymer according to claim 1 , wherein each R is independently a methyl, ethyl or isopropyl radical.

4. The copolymer according to claim 1 , wherein each B is independently a linear, branched or cyclic C 1 -C 12 alkylene radical.

5. The copolymer according to claim 1 , wherein each D is independently a (cyclo)aliphatic C 6 -C 15 alkylene radical.

6. The copolymer according to claim 5 , wherein each D independently has a structural formula selected from the group consisting of

7. A process for preparing the copolymer according to claim 1 , the process comprising:

reacting at least one diol with at least one diisocyanate to give a urethane intermediate, and

subsequently reacting the urethane intermediate with at least one isocyanatoalkyltrialkoxysilane.

8. A coating composition or a constituent of a coating composition, comprising:

the copolymer according to claim 1 .

9. A coating composition, comprising:

A) at least one copolymer according to claim 1 ,

B) a binder component,

C) optionally up to 4 wt % of a catalyst,

D) optionally an auxiliary and an additive, and

E) optionally an organic solvent.

10. The coating composition according to claim 9 , wherein component B) is selected from the group consisting of a hydroxyl-comprising polyester, a polyether, a poly(meth)acrylate, a polycarbonate and a polyurethane having an OH number of from 20 to 500 mg KOH/g and an average molar mass of from 250 to 6000 g/mol.

11. The coating composition according to claim 9 , wherein component C) is at least one catalyst selected from the group consisting of: C1) an organic carboxylic acid having a melting point above 60° C. and C2) a tetraalkylammonium carboxylate.

12. The coating composition according to claim 11 , wherein component C2) is at least one selected from the group consisting of tetramethylammonium formate, tetramethylammonium acetate, tetramethylammonium propionate, tetramethylammonium butyrate, tetramethylammonium benzoate, tetraethylammonium formate, tetraethylammonium acetate, tetraethylammonium propionate, tetraethylammonium butyrate, tetraethylammonium benzoate, tetrapropylammonium formate, tetrapropylammonium acetate, tetrapropylammonium propionate, tetrapropylammonium butyrate, tetrapropylammonium benzoate, tetrabutylammonium formate, tetrabutylammonium acetate, tetrabutylammonium propionate, tetrabutylammonium butyrate and tetrabutylammonium benzoate.

13. A coating composition, comprising:

I) at least one copolymer according to claim 1 ,

II) optionally an adduct of at least one Isocyanatosilane and at least one hydroxy-functional compound,

III) a tin-comprising compound and

IV) an aminosilane.

14. A coating formulation for metal, glass, plastic, paper, textile or wood, the coating formulation comprising:

at least one copolymer according to claim 1 .

15. A coating formulation for metal, glass, plastic, paper, textile or wood, the coating formulation comprising:

at least one coating composition according to claim 9 .

Assignments (3)
CHANGE OF NAME Recorded Jan 31, 2020
From: EVONIK DEGUSSA GMBH
To: EVONIK OPERATIONS GMBH
Reel/Frame 051765/0166 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Dec 1, 2015
From: EVONIK INDUSTRIES AG
To: EVONIK DEGUSSA GMBH
Reel/Frame 037174/0982 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Feb 10, 2015
From: LOMOELDER, RAINER; GOERLITZER, HANS; UNKELHAEUSSER, TOBIAS; HALLACK, MARKUS; STACHE, WIEBKE
To: EVONIK INDUSTRIES AG
Reel/Frame 034931/0678 →