IP Library Granted Patent US 9,517,937
Granted Patent B2
US 9,517,937 · App. 14/660,702 · Granted Dec 13, 2016

Method to synthesize metal chalcogenide monolayer nanomaterials

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Quick Facts
Patent No.
US 9,517,937
App. No.
14/660,702
Granted
Dec 13, 2016
Kind
B2
Abstract

Metal chalcogenide monolayer nanomaterials can be synthesized from metal alkoxide precursors by solution precipitation or solvothermal processing. The synthesis routes are more scalable, less complex and easier to implement than other synthesis routes.

Claims (17)

1. A method to synthesize a metal chalcogenide nanomaterial according to the reaction:

wherein M is an alkaline earth metal or a transition metal and X is the oxidation state of the metal.

2. The method of claim 1 , wherein the transition metal comprises tungsten or molybdenum.

3. The method of claim 2 , wherein M(OR) x comprises W(OEt) 5 .

4. The method of claim 1 , wherein the alkaline earth metal comprises calcium, strontium, or barium.

5. The method of claim 4 , wherein M(OR) x comprises Ca(OAr) 2 .

6. The method of claim 4 , wherein M(OR) x comprises A E (ONep) 2 and A E comprises strontium or barium and wherein ONep is neopentoxide.

7. A method to synthesize a metal chalcogenide nanomaterial according to the reaction:

wherein M is an alkaline earth metal or a transition metal and TOP=E is trioctylphoshine selenide or telluride and X is the oxidation state of the metal.

8. The method of claim 7 , wherein the alkaline earth metal comprises calcium, strontium, or barium.

9. The method of claim 8 , wherein M(OR) x comprises Ca(OAr) 2 .

10. The method of claim 8 , wherein M(OR) x comprises A E (ONep) 2 and A E comprises strontium or barium and wherein ONep is neopentoxide.

11. The method of claim 7 , wherein the transition metal comprises cadmium.

12. The method of claim 11 , wherein M(OR)x comprises Cd(OAr) 2 or Cd(ONep) 2 .

13. The method of claim 7 , wherein the transition metal comprises tungsten or molybdenum.

14. The method of claim 13 , wherein the nanomaterial comprises a layered structure.

15. The method of claim 2 , wherein the nanomaterial comprises a layered structure.

Assignments (3)
CHANGE OF NAME Recorded May 25, 2018
From: SANDIA CORPORATION
To: NATIONAL TECHNOLOGY & ENGINEERING SOLUTIONS OF SANDIA, LLC
Reel/Frame 047052/0538 →
CONFIRMATORY LICENSE Recorded Dec 29, 2015
From: SANDIA CORPORATION
To: U.S. DEPARTMENT OF ENERGY
Reel/Frame 037395/0156 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Apr 9, 2015
From: HERNANDEZ-SANCHEZ, BERNADETTE A.; BOYLE, TIMOTHY J.
To: SANDIA CORPORATION
Reel/Frame 035367/0537 →