IP Library Granted Patent US 10,619,031
Granted Patent B2
US 10,619,031 · App. 14/899,230 · Granted Apr 14, 2020

Crystallizable thermoplastic resin composition and molded article

Inventors: Takahiro Takano (Kanagawa, JP); Ryusuke Yamada (Kanagawa, JP)
Assignee: MITSUBISHI ENGINEERING-PLASTICS CORPORATION
C08K7/06C08G69/265C08J5/042C08K3/04C08K3/34C08K5/098C08K7/04C08L77/06C08J2377/00
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Quick Facts
Patent No.
US 10,619,031
App. No.
14/899,230
Granted
Apr 14, 2020
Kind
B2
Abstract

Provided is resin molded articles having large elastic modulus, and good appearance. A thermoplastic resin composition contains 80 to 120 parts by weight of a carbon fiber and 0.1 to 3.0 parts by weight of a black colorant, per 100 parts by weight of a (A) crystallizable thermoplastic resin which shows a semicrystallization time (ST (P)) of 20 to 500 seconds, wherein the semicrystallization time is measured by depolarization photometry, under conditions that a sample melting temperature is 20 to 40° C. higher than a melting point of the crystallizable thermoplastic resin, a sample melting time is 3 minutes, and an oil bath temperature for crystallization is 140° C.

Claims (16)

1. A thermoplastic resin composition comprising 80 to 120 parts by weight of a carbon fiber and 0.1 to 3.0 parts by weight of a black colorant, per 100 parts by weight of a (A) crystallizable thermoplastic resin which shows a semicrystallization time of 20 to 500 seconds, wherein the semicrystallization time is measured by depolarization photometry, under conditions that a sample melting temperature is 20 to 40° C. higher than a melting point of the crystallizable thermoplastic resin, a sample melting time is 3 minutes, and an oil bath temperature for crystallization is 140° C.,

wherein the carbon fiber comprises polyacrylonitrile-based carbon fiber,

wherein the (A) crystallizable thermoplastic resin is a xylylenediamine-based polyamide resin which comprises diamine constitutive units consisting essentially of 70 to 100% by mol of metaxylylenediamine and 30 to 0% by mol of paraxylylenediamine, and 70% by mol or more of a dicarboxylic acid constitutive unit being derived from adipic acid,

wherein the carbon fiber is about 43.7 to about 54.5% by weight of the thermoplastic resin composition,

wherein the total content of the crystallizable thermoplastic resin and the carbon fiber accounts for 90% by weight or more of the thermoplastic resin composition,

wherein the black colorant is carbon black,

wherein the carbon black has a DBP absorption of 30 to 300 cm 3 /100 g,

wherein the carbon black comprises furnace black, and

wherein the thermoplastic resin composition is free from a flame retarder.

2. The thermoplastic resin composition of claim 1 , wherein the polyamide resin contains an aromatic ring in a molecule thereof, and has a ratio of carbon atoms composing the aromatic ring, relative to the polyamide resin molecule, of 30% by mol or larger.

3. The thermoplastic resin composition of claim 1 , wherein 30% by weight or more of the carbon fiber, contained in the thermoplastic resin composition, is assignable to the polyacrylonitrile-based carbon fiber.

4. The thermoplastic resin composition of claim 1 , wherein a quantity of talc, contained in the thermoplastic resin composition, is 1% by weight or less relative to the thermoplastic resin composition.

5. The thermoplastic resin composition of claim 1 , wherein the carbon fiber shows a tensile strength of 5.0 GPa or smaller, when measured at 23° C. in accordance with JIS R7601.

6. A molded article obtained by molding the thermoplastic resin composition described in of claim 1 .

7. The thermoplastic resin composition of claim 2 , wherein a quantity of talc, contained in the thermoplastic resin composition, is 1% by weight or less relative to the thermoplastic resin composition.

8. The thermoplastic resin composition of claim 1 , the composition being free from dyes.

Assignments (2)
NUNC PRO TUNC ASSIGNMENT Recorded Jan 29, 2024
From: MITSUBISHI ENGINEERING-PLASTICS CORPORATION
To: GLOBAL POLYACETAL CO., LTD.
Reel/Frame 066278/0901 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Dec 18, 2015
From: TAKANO, TAKAHIRO; YAMADA, RYUSUKE
To: MITSUBISHI ENGINEERING-PLASTICS CORPORATION
Reel/Frame 037333/0916 →
Priority Claims (1)
JP 2013-130211 · Jun 21, 2013 · national
Continuity (1)
Related Publication 20160145419A1 · May 26, 2016