IP Library Granted Patent US 9,676,986
Granted Patent B2
US 9,676,986 · App. 15/025,542 · Granted Jun 13, 2017

Adhesive composition for heat dissipating adhesive tape, and heat dissipating adhesive tape

Inventors: Ji-Hye Kim (Bucheon-si, KR); Byung-Ho Ra (Uijeongbu-si, KR); Jang-Soon Kim (Seongnam-si, KR)
Assignee: LG Chem, Ltd.
C09K5/08C09J7/02C09J9/00C09J133/06C09K5/14C08L2312/06C09J2201/602C09J2203/326C09J2400/20C09J2433/00
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Quick Facts
Patent No.
US 9,676,986
App. No.
15/025,542
Granted
Jun 13, 2017
Kind
B2
Abstract

Provided is an adhesive composition for a heat dissipating adhesive tape, the adhesive composition comprising a (meth)acrylic acid ester based photocurable resin, a thermal conductive filler, and a benzotriazole-based compound.

Claims (25)

1. An adhesive composition for a heat dissipating adhesive tape, the adhesive composition comprising:

a (meth)acrylic acid ester-based photocurable resin;

a thermal conductive filler;

a benzotriazole-based compound;

a photo initiator; and

a curing agent.

2. The adhesive composition of claim 1 , wherein the (meth)acrylic acid ester-based photocurable resin is a copolymer of a (meth)acrylic acid ester-based monomer and a functional group-containing cross-linking monomer.

3. The adhesive composition of claim 2 , wherein the functional group-containing cross-linking monomer is a hydroxyl group-containing cross-linking monomer.

4. The adhesive composition of claim 3 , wherein the hydroxyl group-containing cross-linking monomer comprises at least one selected from the group consisting of 2-hydroxyethyl (meth)acrylate, 2-hydroxypropyl (meth)acrylate, 4-hydroxybutyl (meth)acrylate, 6-hydroxyhexyl (meth)acrylate, 8-hydroxyoctyl (meth)acrylate, 2-hydroxyethylene glycol (meth)acrylate, 2-hydroxypropylene glycol (meth)acrylate, and a combination thereof.

5. The adhesive composition of claim 3 , wherein the hydroxyl group-containing cross-linking monomer is polymerized at an amount ratio in a range of about 0.1 wt % to about 50 wt % in monomer components that constitute the (meth)acrylic acid ester-based photocurable resin.

6. The adhesive composition of claim 3 , wherein the (meth)acrylic acid ester-based photocurable is free of a carboxylic group.

7. The adhesive composition of claim 1 , wherein the (meth)acrylic acid ester-based monomer comprises at least one selected from the group consisting of methyl(meth)acrylate, ethyl(meth)acrylate, n-propyl(meth)acrylate, isopropyl(meth)acrylate, n-butyl(meth)acrylate, t-butyl(meth)acrylate, sec-butyl(meth)acrylate, pentyl(meth)acrylate, 2-ethylhexyl(meth)acrylate, 2-ethylbutyl(meth)acrylate, n-octyl(meth)acrylate, isooctyl(meth)acrylate, isobornyl(meth)acrylate, isononyl(meth)acrylate, and a combination thereof.

8. The adhesive composition of claim 1 , wherein the benzotriazole-based compound comprises at least one selected from the group consisting of octyl 3-3(tert-butyl-4-hydroxy-5-(5-chloro-2H-benzotriazol-2-yl)phenyl)propionate, 2-ethylhexyl 3-[3-(5-chlorobenzotriazol-2-yl)-4-hydroxy-5-tert-butyl-phenyl]propanoate, 2-(2H-benzotriazol-2-yl)-6-(dodecyl)-4-methylphenol, 2-(2H-benzotriazol-2-yl)-p-cresol, 2-(2H-benzotriazol-2-yl)-4,6-ditertpentylphenol, 2-(2-hydroxyphenyl)-benzotriazol, 2-(2H-benzotriazol-2-yl)-4,6-bis(1-methyl-1-phenylethyl)phenol, 2-(2H-benzotriazol-2-yl)-6-(1-methyl-1-phenylethyl)-4-(1,1,3,3-tetramethylbutyl)-phenol, and a combination thereof.

9. The adhesive composition of claim 1 , wherein an amount of the benzotriazole-based compound is in a range of about 0.1 part to about 5.0 parts by weight based on 100 parts by weight of the (meth)acrylic acid ester-based photocurable resin.

10. The adhesive composition of claim 1 , wherein the thermal conductive filler is an inorganic filler comprising at least one selected from the group consisting of a metal oxide, a metal hydroxide, a metal nitride, a metal carbide, a metal boride, and a combination thereof.

11. The adhesive composition of claim 1 , wherein an amount of the thermal conductive filler is in a range of about 50 parts to about 300 parts by weight based on 100 parts by weight of the (meth)acrylic acid ester-based photocurable resin.

12. The adhesive composition of claim 1 , wherein a thermal conductivity of a adhesive tape prepared by using the adhesive composition is in a range of about 0.5 W/mK to about 1.0 W/mK.

13. The adhesive composition of claim 1 , wherein the photo initiator comprises at least one selected from the group consisting of a benzoin-based initiator, a hydroxy ketone-based initiator, an aminoketone-based initiator, a caprolactam-based initiator, and a combination thereof.

14. The adhesive composition of claim 1 further comprising an additive that comprises at least one selected from a filler, a surfactant, a tackifier, a coupling agent, an antistatic agent, a dye, a pigment, a sunscreen, an antioxidant, a working fluid, and a combination thereof.

15. A heat dissipating adhesive tape prepared by using an adhesive composition, wherein the adhesive composition comprising:

a (meth)acrylic acid ester-based photocurable resin;

a thermal conductive filler;

a benzotriazole-based compound;

a photo initiator; and

a curing agent.

Assignments (2)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Dec 22, 2016
From: LG HAUSYS, LTD.
To: LG CHEM, LTD.
Reel/Frame 040747/0138 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Mar 28, 2016
From: KIM, JI-HYE; RA, BYUNG-HO; KIM, JANG-SOON
To: LG HAUSYS, LTD.
Reel/Frame 038117/0208 →
Priority Claims (1)
KR 10-2014-0034687 · Mar 25, 2014 · national
Continuity (1)
Related Publication 20160215195A1 · Jul 28, 2016