IP Library Granted Patent US 9,902,694
Granted Patent B2
US 9,902,694 · App. 15/111,068 · Granted Feb 27, 2018

Crystalline forms

Inventors: Istvan Kaldor (Research Triangle Park, NC); Dalin Tang (Shanghai, CN)
Assignee: GlaxoSmithKline Intellectual Property (No 2) Limited
C07D209/42C07B2200/13
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Quick Facts
Patent No.
US 9,902,694
App. No.
15/111,068
Granted
Feb 27, 2018
Kind
B2
Abstract

This invention relates to crystalline forms of (R)-1-(1-(methylsulfonyl)propan-2-yl)-4-(trifluoromethyl)indoline-5-carbonitrile, a modulator of the androgen receptor, and methods for the use in treatment.

Claims (27)

1. A crystalline form of:

that is characterized by an X-ray powder diffraction (XRPD) pattern that has the representative peaks:

Position [°2Theta]

d-spacing [Å]

 7.4 ± 0.1

11.9

12.7 ± 0.1

7.0

17.5 ± 0.1

5.1

19.5 ± 0.1

4.6

21.9 ± 0.1

4.1

22.5 ± 0.1

3.9

23.9 ± 0.1

3.7

26.5 ± 0.1

3.4.

2. The crystalline form of claim 1 that is further characterized by an XRPD pattern substantially in accordance with FIG. 2 .

3. The crystalline form of claim 1 that is further characterized by an 19 F SSNMR spectrum comprising isotropic chemical shifts at −55.5±0.2 and −56.3±0.2 ppm, wherein the 19 F SSNMR spectrum is obtained on a spectrometer operating at a frequency of 470.40 MHz for 19 F observation using a cross-polarization pulse sequence with a Bruker 4-mm triple resonance magic-angle spinning probe at a rotor frequency of 12.5 kHz.

4. The crystalline form of claim 1 that is further characterized by an 19 F SSNMR spectrum substantially in accordance with FIG. 6 .

5. The crystalline form of claim 1 that is further characterized by an 13 C SSNMR (solid state nuclear magnetic resonance) spectrum comprising isotropic chemical shifts at 138.4±0.2, 127.4±0.2, 125.5±0.2, 124.3±0.2, 123.3±0.2 116.5±0.2, 114.1±0.2, 104.7±0.2, 97.4±0.2, 61.8±0.2, 60.9±0.2, 59.2±0.2, 48.2±0.2, 47.6±0.2, 46.3±0.2, 44.4±0.2, 42.3±0.2 , and 26.1±0.2 ppm, wherein the 13 C SSNMR spectrum is obtained on a spectrometer operating at a frequency of 125.73 MHz for 13 C observation using a cross-polarization pulse sequence with a Bruker 4-mm triple resonance magic-angle spinning probe at a rotor frequency of 8kHz.

6. The crystalline form of claim 1 that is further characterized by an 13 C SSNMR spectrum substantially in accordance with FIG. 5 .

7. A method of treating a disorder selected from muscle wasting associated with chronic obstructive pulmonary disease (COPD), muscle wasting associated with chronic kidney disease (CKD), muscle wasting associated with chronic heart failure (CHF), and urinary incontinence, wherein said method comprises administering a compound according to claim 1 to a human subject.

8. A method of accelerating hip fracture repair and healing, wherein said method comprises administering a compound according to claim 1 to a human subject.

Assignments (1)
CHANGE OF ADDRESS Recorded Apr 16, 2025
From: GLAXOSMITHKLINE INTELLECTUAL PROPERTY (NO.2) LIMITED
To: GLAXOSMITHKLINE INTELLECTUAL PROPERTY (NO.2) LIMITED
Reel/Frame 070854/0469 →
Continuity (2)
Provisional Application 61929814 · Jan 21, 2014
Related Publication 20160332967A1 · Nov 17, 2016