IP Library Granted Patent US 10,221,268
Granted Patent B2
US 10,221,268 · App. 15/120,261 · Granted Mar 5, 2019

Vinyl polymer powder, thermoplastic resin composition, and molded body thereof

Inventors: Masahiro Ueda (Otake, JP); Shinji Matsuoka (Otake, JP)
Assignee: Mitsubishi Chemical Corporation
C08F212/08C08F220/18C08J3/16C08L25/14C08L67/00C08L69/00C08L77/00C08L101/00C08J2325/14C08L33/06C08L77/02C08L77/06C08L77/10C08L2201/54
View Patent ↗
Loading inventors, assignments & file history…
Monitor This Case
Get email alerts when status or documents change.
Order Certified Copies
Most orders are placed with the USPTO same day — all within 24 business hours.
Order via The Patent Place →
Pre-filled with this patent's details
Quick Facts
Patent No.
US 10,221,268
App. No.
15/120,261
Granted
Mar 5, 2019
Kind
B2
Abstract

This vinyl polymer powder, which contains a vinyl polymer, has a glass transition temperature of at least 0° C. (where if there are a plurality of glass transition points, all of the glass transition temperatures are at least 0° C.), has no greater than 350 ppm of the total content of magnesium ions, calcium ions, aluminum ions, barium ions, and zinc ions, has no greater than 100 ppm of the content of ammonium ions, has an acid number of no greater than 2.5 mgKOH/g, and has a bulk density of 0.10-0.60 g/cm 3 .

Claims (41)

1. A thermoplastic resin composition comprising:

70 to 99.9% by mass of an engineering plastic; and

0.1 to 30% by mass of a vinyl polymer powder comprising a vinyl polymer,

wherein:

a glass transition temperature of the vinyl polymer is 0° C. or higher, provided that when there are a plurality of glass transition points, all of the glass transition temperatures are 0° C. or higher,

a total content of magnesium ions, calcium ions, aluminum ions, barium ions, and zinc ions is 350 ppm or less with respect to a total mass of the vinyl polymer powder,

a content of ammonium ions is 100 ppm or less with respect to a total mass of the vinyl polymer powder,

an acid value is 2.5 mgKOH/g or less, and

a bulk density is 0.10 to 0.60 g/cm 3 .

2. The thermoplastic resin composition according to claim 1 , wherein the engineering plastic is at least one resin selected from polyamide, polyester, and polycarbonate.

3. A molded body formed by molding the thermoplastic resin composition according to claim 1 .

4. A vinyl polymer powder comprising:

0.5 to 99.5% by mass of a (meth)acrylate ester unit which contains an alkyl group having 1 to 4 carbon atoms or an aromatic group in an ester moiety;

0.5 to 99.5% by mass of an aromatic vinyl monomer unit; and

a vinyl polymer having a glass transition temperature of 0° C. or higher, provided that, when there are a plurality of glass transition points, all of the glass transition temperatures are 0° C. or higher,

wherein:

the vinyl polymer powder satisfies the following Conditions [1] and [2];

Condition [1]:

a bulk density as measured according to JIS K6720 is 0.30 to 0.60 g/cm 3 ;

Condition [2]:

free flow property as measured by the following method is 20 g/10 sec or more;

[Measurement Method for Free Flow Property]

a measurement instrument, which includes a seat on which a tray is set, a funnel provided with a shutter at a cylindrical opening thereof which has an inner diameter of an upper part at 8 mm and an inner diameter of a lower part at 20 mm, a support holding the funnel above the seat, and a support rod to which the support is fixed, is placed in a horizontal site;

the shutter of the funnel is closed, and 120 cm 3 of powder is uniformly put into the funnel;

subsequently, the shutter is opened to drop the powder, and immediately, the tray is set on the seat;

at the same time of setting the tray, the counting of time starts by using a stopwatch, and after 10 seconds, the tray is removed from the measurement instrument;

the tray containing the powder is weighed to obtain the amount of the powder dropped for 10 seconds; and

the above measurement is carried out two times, and an average value of the amounts of the powder dropped for 10 seconds is obtained and this value is designated as the free flow property (g/10 sec).

5. The thermoplastic resin composition according to claim 1 , wherein free flow property as measured by the following method is 15 g/10 sec or more;

[Measurement Method for Free Flow Property]

a measurement instrument, which includes a seat on which a tray is set, a funnel provided with a shutter at a cylindrical opening thereof which has an inner diameter of an upper part at 8 mm and an inner diameter of a lower part at 20 mm, a support holding the funnel above the seat, and a support rod to which the support is fixed, is placed in a horizontal site;

the shutter of the funnel is closed, and 120 cm 3 of powder is uniformly put into the funnel;

subsequently, the shutter is opened to drop the powder, and immediately, the tray is set on the seat;

at the same time of setting the tray, the counting of time starts by using a stopwatch, and after 10 seconds, the tray is removed from the measurement instrument;

the tray containing the powder is weighed to obtain the amount of the powder dropped for 10 seconds; and

the above measurement is carried out two times, and an average value of the amounts of the powder dropped for 10 seconds is obtained and this value is designated as the free flow property (g/10 sec).

6. The thermoplastic resin composition according to claim 1 , wherein the total content of sodium ions and potassium ions is 100 ppm or less with respect to the total mass of the vinyl polymer powder.

7. The thermoplastic resin composition according to claim 1 , wherein the vinyl polymer contains a (meth)acrylate ester unit which contains an alkyl group having 1 to 4 carbon atoms or an aromatic group in an ester moiety.

8. The thermoplastic resin composition according to claim 1 , wherein 0.5 to 99.5% by mass of an aromatic vinyl monomer unit is contained in the total mass of the monomer unit that constitutes the vinyl polymer.

9. The thermoplastic resin composition according to claim 1 , wherein a mass average molecular weight of the vinyl polymer is 5,000 to 20,000,000.

10. The thermoplastic resin composition according to claim 1 , wherein a mass average molecular weight of the vinyl polymer is 5,000 to 200,000.

Assignments (2)
MERGER Recorded Jun 28, 2017
From: MITSUBISHI RAYON CO., LTD.
To: MITSUBISHI CHEMICAL CORPORATION
Reel/Frame 043029/0663 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Aug 19, 2016
From: UEDA, MASAHIRO; MATSUOKA, SHINJI
To: MITSUBISHI RAYON CO., LTD.
Reel/Frame 039484/0022 →
Priority Claims (1)
JP 2014-058378 · Mar 20, 2014 · national
Continuity (1)
Related Publication 20170066860A1 · Mar 9, 2017