IP Library Granted Patent US 9,670,116
Granted Patent B2
US 9,670,116 · App. 15/137,805 · Granted Jun 6, 2017

Process and composition for inhibiting the polymerization of cyclopentadiene compounds

Inventors: Stefanie Rinker (Dorsten, DE); Bettina Ludwig (Marl, DE); Manfred Neumann (Marl, DE); Felix Nissen (Nottuln, DE); Oliver Erpeldinger (Wuelfrath, DE); Phillip R. James (Tenby, GB); Peter Watkins (West Berkshire, GB)
Assignee: Evonik Degussa GmbH
C07C7/20C09K15/08C09K15/20C07C2101/10C07C2103/68
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Quick Facts
Patent No.
US 9,670,116
App. No.
15/137,805
Granted
Jun 6, 2017
Kind
B2
Abstract

A process for inhibiting the polymerization of cyclopentadiene compounds (B) by contacting the cyclopentadiene compound with a quinone methide compound (A) of structure (I), Compositions (AB) comprising (A) and (B) are also provided.

Claims (13)

1. A process for inhibiting polymerization of a cyclopentadiene compound (B), the process comprising:

contacting the cyclopentadiene compound (B) with at least one compound (A); wherein

(A) is a compound of structure (I)

wherein

R 1 and R 2 are each tert-butyl; and

R 3 is —CN or —O—R 10 , where R 10 is methyl, ethyl, n-propyl, iso-propyl, n-butyl, n-pentyl, or n-hexyl.

2. The process according to claim 1 , wherein the cyclopentadiene compound (B) is at least one selected from the group consisting of cyclopentadiene, dicyclopentadiene, alkylated cyclopentadiene, and alkylated dicyclopentadiene.

3. The process according to claim 1 , wherein the cyclopentadiene compound (B) is at least one of cyclopentadiene and dicycloptentadiene.

4. The process according to claim 1 , wherein the at least one compound (A) forms a solution (AC) with at least one solvent (C), wherein the solvent (C) is at least one selected from the group consisting of benzene, a mono-alkylated aromatic compound, a polyalkylated aromatic compound, an alkane having a carbon number of 6 to 15, a cycloalkane having a carbon number of 6 to 15, a high-boiling hydrocarbon cut, an ether having a carbon number of 6 to 15, and an ester having a carbon number of 6 to 15.

5. The process according to claim 4 , wherein a ratio of a total weight of the at least one compound (A) in the solution (AC) to a total weight of the at least one solvent (C) in the solution (AC) is from 1:1000 to 100:1.

6. The process according to claim 1 , wherein a total concentration of the at least one compound (A) is between 10 ppb and 100,000 ppm, based on a total weight of all cyclopentadiene compounds.

7. The process according to claim 1 , wherein the cyclopentadiene compound (B) is a component of a process stream and a concentration of the cyclopentadien compound (B) is 0.0001 to 15 wt % based on the total weight of the process stream.

8. The process according to claim 1 , wherein R 3 is —CN.

Assignments (1)
CHANGE OF NAME Recorded Jan 31, 2020
From: EVONIK DEGUSSA GMBH
To: EVONIK OPERATIONS GMBH
Reel/Frame 051765/0166 →
Priority Claims (1)
DE 10 2013 204 950 · Mar 20, 2013 · national
Continuity (2)
Continuation 14217588 · Mar 18, 2014
Related Publication 20160237346A1 · Aug 18, 2016