IP Library Granted Patent US 9,938,609
Granted Patent B2
US 9,938,609 · App. 15/177,856 · Granted Apr 10, 2018

Acid and alkali resistant Ni—Cr—Mo—Cu alloys with critical contents of chromium and copper

Inventors: Paul Crook (Kokomo, IN); Vinay P. Deodeshmukh (Carmel, IN)
Assignee: Haynes International, Inc.
C22C19/055C22C19/053C22F1/10
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Quick Facts
Patent No.
US 9,938,609
App. No.
15/177,856
Granted
Apr 10, 2018
Kind
B2
Abstract

A nickel-chromium-molybdenum-copper alloy resistant to 70% sulfuric acid at 93° C. and 50% sodium hydroxide at 121° C. for acid and alkali neutralization in the field of waste management; the alloy contains, in weight percent, 27 to 33 chromium, 4.9 to 7.8 molybdenum, 3.1 to 6.0 wt. % copper (when chromium is between 30 and 33 wt. %) or 4.7 to 6.0 wt. % copper (when chromium is between 27 and 29.9 wt. %), up to 3.0 iron, 0.3 to 1.0 manganese, 0.1 to 0.5 aluminum, 0.1 to 0.8 silicon, 0.01 to 0.11 carbon, up to 0.13 nitrogen, up to 0.05 magnesium, up to 0.05 rare earth elements, with a balance of nickel and impurities. Titanium or another MC carbide former can be added to enhance thermal stability of the alloy.

Claims (57)

1. A nickel-chromium-molybdenum-copper alloy resistant to sulfuric acid, having a corrosion rate of less than 0.45 mm/y in 70% sulfuric acid at 93° C. and resistant to sodium hydroxide, having a maximum internal attack corresponding to corrosion rate of less than 0.45 mm/y in 50% sodium hydroxide at 121° C., consisting essentially of:

30 to 33 wt. % chromium

4.9 to 7.8 wt. % molybdenum

3.1 to 6.0 wt. % copper

up to 3.0 wt. % iron

0.3 to 1.0 wt. % manganese

0.1 to 0.5 wt. % aluminum

0.1 to 0.8 wt. % silicon

0.01 to 0.11 wt. % carbon

up to 0.13 wt. % nitrogen

up to 0.05 wt. % magnesium

up to 0.05 wt. % rare earth elements

up to 0.56 wt. % titanium

up to 1.12 wt. % niobium

up to 2.24 wt. % tantalum

up to 2.24 wt. % hafnium

with a balance of nickel and impurities.

2. The nickel-chromium-molybdenum-copper alloy of claim 1 , wherein the alloys are in wrought forms selected from the group consisting of sheets, plates, bars, wires, tubes, pipes, and forgings.

3. The nickel-chromium-molybdenum-copper alloy of claim 1 , wherein the alloy is in cast form.

4. The nickel-chromium-molybdenum-copper alloy of claim 1 , wherein the alloy is in powder metallurgy form.

5. The nickel-chromium-molybdenum-copper alloy of claim 1 , consisting essentially of:

30 to 33 wt. % chromium

5.0 to 6.2 wt. % molybdenum

3.5 to 4.0 wt. % copper

up to 1.5 wt. % iron

0.3 to 0.7 wt. % manganese

0.1 to 0.4 wt. % aluminum

0.1 to 0.6 wt. % silicon

0.02 to 0.10 wt. % carbon

with a balance of nickel and impurities.

6. The nickel-chromium-molybdenum-copper alloy of claim 1 , consisting essentially of:

31 wt. % chromium

5.6 wt. % molybdenum

3.8 wt. % copper

1.0 wt. % iron

0.5 wt. % manganese

0.4 wt. % silicon

0.3 wt. % aluminum

0.03 to 0.07 wt. % carbon

with a balance of nickel, nitrogen, impurities, and trace amounts of magnesium.

7. The nickel-chromium-molybdenum-copper alloy of claim 1 , consisting essentially of:

31 wt. % chromium

5.6 wt. % molybdenum

3.8 wt. % copper

1.0 wt. % iron

0.5 wt. % manganese

0.4 wt. % silicon

0.3 wt. % aluminum

0.03 to 0.07 wt. % carbon

with a balance of nickel, nitrogen, impurities, trace amounts of magnesium and trace amounts of the rare earth elements.

8. The nickel-chromium-molybdenum-copper alloy of claim 1 , wherein the alloy contains at least one MC carbide former.

9. The nickel-chromium-molybdenum-copper alloy of claim 8 , wherein the MC carbide former is selected from the group consisting of titanium, niobium, tantalum and hafnium.

10. The nickel-chromium-molybdenum-copper alloy of claim 1 , the alloy consisting essentially of 0.20 to 0.56 wt. % titanium.

11. The nickel-chromium-molybdenum-copper alloy of claim 1 , the alloy consisting essentially of 0.30 to 1.12 wt. % niobium.

12. The nickel-chromium-molybdenum-copper alloy of claim 1 , the alloy consisting essentially of 0.60 to 2.24 wt. % tantalum.

13. The nickel-chromium-molybdenum-copper alloy of claim 1 , the alloy consisting essentially of 0.60 to 2.24 wt. % hafnium.

14. The nickel-chromium-molybdenum-copper alloy of claim 1 , wherein the impurities are selected from the group consisting of cobalt, tungsten, sulfur, phosphorous, oxygen and calcium.

Assignments (3)
RELEASE OF SECURITY INTEREST Recorded Nov 21, 2024
From: JPMORGAN CHASE BANK, N.A., AS ADMINISTRATIVE AGENT
To: HAYNES INTERNATIONAL, INC.
Reel/Frame 069358/0006 →
SECURITY INTEREST Recorded Oct 19, 2020
From: HAYNES INTERNATIONAL, INC.
To: JPMORGAN CHASE BANK, N.A., AS ADMINISTRATIVE AGENT
Reel/Frame 054091/0935 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jun 22, 2016
From: CROOK, PAUL; DEODESHMUKH, VINAY
To: HAYNES INTERNATIONAL, INC.
Reel/Frame 038980/0956 →
Continuity (5)
Division 14055126 · Oct 16, 2013
Continuation In Part 13871405 · Apr 26, 2013
Continuation In Part 13719369 · Dec 19, 2012
Provisional Application 61640096 · Apr 30, 2012
Related Publication 20160289799A1 · Oct 6, 2016