IP Library Granted Patent US 10,270,035
Granted Patent B2
US 10,270,035 · App. 15/252,427 · Granted Apr 23, 2019

Polymer, composition for organic electroluminescent element, organic electroluminescent element, organic EL display device, and organic EL lighting device

Inventors: Koichiro Iida (Kanagawa, JP); Yanjun Li (Kanagawa, JP); Tomokazu Umemoto (Kanagawa, JP); Qi Gao (Kanagawa, JP); Hideki Goromaru (Kanagawa, JP)
Assignee: Mitsubishi Chemical Corporation
H01L51/0039C07C13/66C07C25/02C07C25/22C07C39/17C07C211/45C07C309/00C07F5/04C08G73/02H01L51/0043C07C2602/06C07C2603/08C07C2603/50H01L51/0003H01L51/008H01L51/0058H01L51/0059H01L51/0067H01L51/0072H01L51/0081H01L51/0085H01L51/5056H01L51/5088
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Quick Facts
Patent No.
US 10,270,035
App. No.
15/252,427
Granted
Apr 23, 2019
Kind
B2
Abstract

The object of the present invention is to provide a polymer capable of being insolubilized at a low temperature in a short time, having a high hole injecting and transporting ability and a high durability, and a composition for organic electroluminescent element comprising the polymer. The polymer of the present invention comprises a specific crosslinkable group.

Claims (26)

1. A polymer having a crosslinkable group represented by the following formula (1):

wherein the 1,2-dihydrocyclobuta[a]naphthalene ring may have a substituent.

2. The polymer according to claim 1 , which comprises a repeating unit represented by the following formula (2):

wherein p represents an integer of 0 to 3,

Ar 1 and Ar 2 each independently represent a direct bond, an aromatic hydrocarbon group that may have a substituent, or an aromatic heterocyclic group that may have a substituent,

Ar 3 to Ar 5 each independently represent an aromatic hydrocarbon group that may have a substituent, or an aromatic heterocyclic group that may have a substituent, and

the Ar 1 and Ar 2 are not direct bonds at the same time.

3. The polymer according to claim 1 , which comprises a repeating unit represented by the following formula (3):

wherein q represents an integer of 0 to 3,

R 1 represents an alkyl group of 1 to 24 carbon atoms that may have a substituent, an aromatic hydrocarbon group that may have a substituent, or an aromatic heterocyclic group that may have a substituent,

Ar 6 and Ar 7 each independently represents a direct bond, an aromatic hydrocarbon group that may have a substituent, or an aromatic heterocyclic group that may have a substituent,

Ar 8 to Ar 12 each independently represents an aromatic hydrocarbon group that may have a substituent, or an aromatic heterocyclic group that may have a substituent, and

the Ar 6 and Ar 7 are not direct bonds at the same time.

4. The polymer according to claim 1 , which comprises a repeating unit represented by the following formula (4):

wherein r represents an integer of 0 to 3,

Ar 13 , Ar 14 , Ar 16 , and Ar 17 each independently represent an aromatic hydrocarbon group that may have a substituent, or an aromatic heterocyclic group that may have a substituent, and

Ar 15 represents a direct bond, an aromatic hydrocarbon group that may have a substituent, or an aromatic heterocyclic group that may have a substituent.

5. The polymer according to claim 1 , which has a weight-average molecular weight (Mw) of 20,000 or more, and a degree of dispersion (Mw/Mn) of 2.5 or less.

6. A composition for organic electroluminescent element, which comprises the polymer of claim 1 .

7. An organic electroluminescent element comprising a substrate, an anode and a cathode provided on the substrate, and an organic layer provided between the anode and the cathode, wherein the organic layer contains a layer formed by a wet film formation method using the composition for organic electroluminescent elements of claim 6 .

8. The organic electroluminescent element according to claim 7 , wherein the layer formed by a wet film formation method is at least one of a hole injection layer and a hole transport layer.

9. The organic electroluminescent element according to claim 7 , which comprises a hole injection layer, a hole transport layer and a light-emitting layer between the anode and the cathode, wherein the hole injection layer, the hole transport layer, and the light-emitting layer are all formed by a wet film formation method.

10. An organic EL display device comprising the organic electroluminescent element of claim 7 .

11. An organic EL lighting device comprising the organic electroluminescent element of claim 7 .

12. A compound represented by the following formula (5):

wherein X represents a halogen atom.

Assignments (3)
CHANGE OF NAME Recorded Sep 5, 2017
From: MITSUBISHI RAYON CO., LTD.
To: MITSUBISHI CHEMICAL CORPORATION
Reel/Frame 043750/0834 →
MERGER Recorded Sep 4, 2017
From: MITSUBISHI CHEMICAL CORPORATION
To: MITSUBISHI RAYON CO., LTD.
Reel/Frame 043750/0207 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Oct 26, 2016
From: IIDA, KOICHIRO; LI, YANJUN; UMEMOTO, TOMOKAZU; GAO, QI; GOROMARU, HIDEKI
To: MITSUBISHI CHEMICAL CORPORATION
Reel/Frame 040141/0809 →
Priority Claims (1)
JP 2014-040769 · Mar 3, 2014 · national
Continuity (2)
Continuation PCTJP2015056094 · Mar 2, 2015
Related Publication 20160372676A1 · Dec 22, 2016