IP Library Granted Patent US 9,862,648
Granted Patent B2
US 9,862,648 · App. 15/301,597 · Granted Jan 9, 2018

Transparent metal fluoride ceramic

Inventors: Michel Mortier (Paris, FR); Pierre Aballea (Alfortville, FR); Patrick Gredin (Aulnay Sous Bois, FR); Akiko Suganuma (Paris, FR)
Assignees: PARIS SCIENCES ET LETTRES—QUARTIER LATIN; CENTRE NATIONAL DE LA RECHERCHE SCIENTIFIQUE (CNRS); UNIVERSITY PIERRE ET MARIE CURIE (PARIS 6)
C04B35/553C04B35/6263C04B35/6264C04B35/6266C04B35/62615C04B35/62655C04B35/64C04B2235/3201C04B2235/3206C04B2235/3208C04B2235/3213C04B2235/3215C04B2235/3224C04B2235/3225C04B2235/3227C04B2235/3241C04B2235/3279C04B2235/5454C04B2235/5481C04B2235/658C04B2235/6562C04B2235/6565C04B2235/6567C04B2235/668C04B2235/77C04B2235/781C04B2235/784C04B2235/785C04B2235/9653
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Quick Facts
Patent No.
US 9,862,648
App. No.
15/301,597
Granted
Jan 9, 2018
Kind
B2
Abstract

A method for producing a metal fluoride ceramic, comprising: providing a sedimented compound comprising metal fluoride particles having an average particle size lower than 30 nm and a solvent, partially drying the sedimented compound at a temperature lower than 65° C. until the partially dried compound comprises from 5 wt % to 45 wt % of the solvent, and sintering, for example in air, the partially dried and sedimented compound.

Claims (19)

1. A method for producing a metal fluoride ceramic, comprising:

providing a sedimented compound comprising metal fluoride particles having an average particle size lower than 30 nm and a solvent;

partially drying the sedimented compound at a temperature lower than 65° C. until the partially dried compound comprises from 5 wt % to 45 wt % of the solvent; and

sintering the partially dried and sedimented compound.

2. The method according to claim 1 , wherein providing a sedimented compound comprises:

centrifuging the metal fluoride particles in the solvent, and removing the supernate.

3. The method according to claim 1 , wherein the sintering is performed under air and under atmospheric pressure.

4. The method according to claim 1 , wherein the sedimented compound comprises about 60 wt % of solvent or less.

5. The method according to claim 1 , wherein the metal fluoride particles have a standard deviation of the particle size lower than 25 nm.

6. The method according to claim 1 , wherein the metal fluoride particles are selected from the group comprising MF2, AMF3, ABF4 and AB3F10, and a solid solution MF2-M′F2, wherein A is an alkali metal, B is a rare earth metal and M and M′ are an alkaline earth metal.

7. The method according to claim 6 , wherein A is selected from the group consisting of potassium, sodium, cesium and rubidium, B is selected from the group consisting of yttrium and lanthanides, and M and M′ are selected from the group comprising calcium, magnesium, barium and strontium.

8. The method according to claim 7 , wherein M is calcium.

9. The method according to claim 1 , wherein the metal fluoride particles further comprise at least one dopant.

10. The method according to claim 9 , wherein the dopant is selected from the group consisting of transition metals and rare earth metals.

11. The method according to claim 1 , wherein the metal fluoride particles are ytterbium (III) doped calcium fluoride particles.

12. The method according claim 1 , wherein the sintering is performed at a temperature ranging between 500° C. to 750° C.

13. The method according to claim 1 , wherein providing a sedimented compound comprises:

providing a mixture of a solvent and of metal fluoride particles, and

centrifuging the mixture for about 40 min or more, and removing the supernate.

Assignments (2)
CHANGE OF NAME Recorded Jan 19, 2022
From: PARIS SCIENCES ET LETTRES - QUARTIER LATIN
To: PARIS SCIENCES ET LETTRES
Reel/Frame 058772/0593 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jan 3, 2017
From: MORTIER, MICHEL; ABALLEA, PIERRE; GREDIN, PATRICK; SUGANUMA, AKIKO
To: PARIS SCIENCES ET LETTRES - QUARTIER LATIN; CENTRE NATIONAL DE LA RECHERCHE SCIENTIFIQUE - CNRS; UNIVERSITE PIERRE ET MARIE CURIE (PARIS 6)
Reel/Frame 040826/0516 →
Priority Claims (1)
EP 14305495 · Apr 4, 2014 · regional
Continuity (1)
Related Publication 20170015591A1 · Jan 19, 2017