IP Library Granted Patent US 10,100,602
Granted Patent B2
US 10,100,602 · App. 15/348,491 · Granted Oct 16, 2018

Self-pressurizing soluble alkali silicate for use in sealing subterranean spaces

View Patent ↗
Loading inventors, assignments & file history…
Monitor This Case
Get email alerts when status or documents change.
Order Certified Copies
Most orders are placed with the USPTO same day — all within 24 business hours.
Order via The Patent Place →
Pre-filled with this patent's details
Quick Facts
Patent No.
US 10,100,602
App. No.
15/348,491
Granted
Oct 16, 2018
Kind
B2
Abstract

Compositions and methods are disclosed for sealing subterranean spaces such as natural or induced fractures, vugs or annular spaces. The composition is composed of a base fluid consisting of a soluble alkali silicate, a gas generating additive, water, solids, and a setting agent. The gas generating additive may be coated or uncoated. The gas generating additive may also be in the form of a slurry. In the case of coated additives, the coating may act as a retarder or an accelerator to the expansion and setting agent of the soluble alkali silica. Similarly, the choice of carrier fluid in a slurry may retard or accelerate the expansion and setting of the alkali silicate-based plug.

Claims (10)

1. A method for sealing subterranean spaces comprising the step of introducing into a downhole a base fluid containing a soluble alkali silicate, a gas generating additive, a setting agent, water, and solids, whereby the soluble alkali silicate promotes a gas generating reaction wherein the gas generating additive reacts with water to produce a gas, causing the soluble alkali silicate to expand and self-pressurize in a subterranean space, thereby sealing the subterranean space.

2. The method of claim 1 wherein said gas generating additive is one of a metal and a metal salt, wherein the soluble alkali silicate promotes an oxidation reaction of the one of a metal and a metal salt with water.

3. A method for sealing a subterranean space comprising the steps of:

a. introducing into a downhole a base fluid containing a soluble alkali silicate, a gas generating additive, water, solids, and a setting agent; and

b. said soluble alkali silicate promoting a gas generating reaction of said gas generating additive with water to produce a gas;

wherein said gas produced by said reaction causes said alkali silicate to expand and self-pressurize in said downhole, thereby sealing the subterranean space.

4. The method of claim 3 further comprising the step

(c) said setting agent causing said expanded alkali silicate to set in said downhole.

5. The method of claim 4 wherein said gas generating additive is one of a metal and a metal salt, wherein the soluble alkali silicate promotes an oxidation reaction of the one of a metal and a metal salt with water.

6. The method of claim 5 wherein said setting agent is one of a metal and a metal salt.

Assignments (9)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Oct 20, 2022
From: BYK USA INC.
To: BYK-CHEMIE GMBH
Reel/Frame 061478/0199 →
CHANGE OF NAME Recorded Dec 2, 2021
From: PQ CORPORATION
To: PQ LLC
Reel/Frame 058295/0836 →
PARTIAL RELEASE OF SECURITY INTEREST IN PATENTS RECORDED AT R/F 056539/0903 Recorded Aug 5, 2021
From: CREDIT SUISSE AG, CAYMAN ISLANDS BRANCH, AS ADMINISTRATIVE AGENT
To: PQ CORPORATION
Reel/Frame 057089/0255 →
TERM LOAN PATENT SECURITY AGREEMENT Recorded Jun 10, 2021
From: PQ CORPORATION
To: CREDIT SUISSE AG, CAYMAN ISLANDS BRANCH, AS AGENT
Reel/Frame 056539/0903 →
RELEASE OF SECURITY INTEREST IN PATENTS AT R/F 053281/0474 Recorded Jun 10, 2021
From: CREDIT SUISSE AG, CAYMAN ISLANDS BRANCH, AS COLLATERAL AGENT
To: PQ CORPORATION
Reel/Frame 056539/0782 →
SECURITY INTEREST Recorded Jul 22, 2020
From: PQ CORPORATION
To: CREDIT SUISSE AG, CAYMAN ISLANDS BRANCH, AS COLLATERAL AGENT
Reel/Frame 053281/0474 →
MERGER Recorded May 19, 2017
From: BYK ADDITIVES INC.
To: BYK USA INC.
Reel/Frame 042436/0509 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Nov 11, 2016
From: MCDONALD, MICHAEL JAMES; LI, XIANGLIAN; SHORT, KELLY PAUL, JR.
To: PQ CORPORATION
Reel/Frame 040290/0869 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Nov 11, 2016
From: CRAMER, BRETT HOWARD
To: BYK ADDITIVES, INC.
Reel/Frame 040605/0933 →