IP Library Granted Patent US 11,027,249
Granted Patent B2
US 11,027,249 · App. 15/355,907 · Granted Jun 8, 2021

Azeotrope-like compositions of 1,1,1,2-tetrafluoropropene and 1,1,1,2-tetrafluoroethane

Inventors: Christopher J. Seeton (East Amherst, NY); Hang T. Pham (Amherst, NY); Rajiv R. Singh (Getzville, NY); Ryan Hulse (Getzville, NY); Mark W. Spatz (East Amherst, NY); David P. Wilson (Amherst, NY); Samuel F. Yana Motta (East Amherst, NY)
Assignee: Honeywell International Inc.
B01F17/0085A61K8/046A61K8/70A61K9/124A61Q5/06A61Q15/00A61Q19/00B01F17/0035C08J9/146C09K3/00C09K3/30C09K5/045C11D7/505A61K2800/244C08J2203/164C08J2371/10C08J2375/04C09K2205/122C09K2205/126C09K2205/22C09K2205/32C09K2205/40
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Quick Facts
Patent No.
US 11,027,249
App. No.
15/355,907
Granted
Jun 8, 2021
Kind
B2
Abstract

Provided are azeotrope-like compositions consisting essentially of 1,1,1,2-tetrafluoropropene and 1,1,1,2-tetrafluoroethane and uses thereof, including use in refrigerant compositions, refrigeration systems, blowing agent compositions, and aerosol propellants.

Claims (20)

1. An azeotrope-like composition consisting essentially of from about 43.38 percent by weight to about 65.16 percent by weight of 1,1,1,2-tetrafluoropropene and from about 34.84 percent by weight to about 56.62 percent by weight of 1,1,1,2-tetrafluoroethane to form a non-flammable composition, said composition being azeotropic at least one concentration of the components within said range of component concentrations, said non-flammable composition having a boiling point that is below the boiling point of said 1,1,1,2-tetrafluoropropene and said 1,1,1,2-tetrafluoroethane and that is from about −29.16° C. to about −29.92° C. at a pressure of about 14.3 psia.

2. A method for modifying a refrigeration apparatus which refrigeration apparatus comprises a refrigerant and a lubricant, which refrigerant comprises a chlorofluorocarbon, a hydrofluorocarbon, a hydrochlorofluorocarbon, or combinations thereof, and the lubricant comprises a mineral oil, alkybenezene, polyalphaolefin, polyol ester, polyakylene glycol, polyvinyl ether, synthetic naphthalene, fluorolubricant or combinations thereof, the method comprising removing or leaking at least a portion of the refrigerant from the refrigeration apparatus and leaving a residue comprising the lubricant, and adding to said residue the azeotrope-like composition of claim 1 .

3. The azeotrope-like composition of claim 1 having a boiling point of from about −29.4° C. to about −29.9° C. at a pressure of about 14.3 psia.

4. The azeotrope-like composition of claim 1 which consists essentially of from about 39.32 percent by weight to about 52.9 weight percent 1,1,1,2-tetrafluoroethane and from about 47.1 to about 60.68 weight percent of 1,1,1,2-tetrafluoropropene.

5. A refrigerant composition comprising the azeotrope-like composition of claim 4 .

6. A method for cooling an article which comprises condensing a refrigerant composition of claim 5 and thereafter evaporating said refrigerant composition in the vicinity of the article to be cooled.

7. A method for heating an article which comprises condensing a refrigerant composition of claim 5 in the vicinity of the article to be heated and thereafter evaporating said refrigerant composition.

8. The azeotrope-like composition of claim 1 which consists essentially of from about 43.73 percent by weight to about 47.29 weight percent 1,1,1,2-tetrafluoroethane and from about 52.71 to about 56.27 weight percent of 1,1,1,2-tetrafluoropropene.

9. A refrigerant composition comprising the azeotrope-like composition of claim 8 .

10. A method for cooling an article which comprises condensing a refrigerant composition of claim 9 and thereafter evaporating said refrigerant composition in the vicinity of the article to be cooled.

11. A method for heating an article which comprises condensing a refrigerant composition of claim 9 in the vicinity of the article to be heated and thereafter evaporating said refrigerant composition.

12. The azeotrope-like composition of claim 1 which consists essentially of about 43.73 weight percent 1,1,1,2-tetrafluoroethane and about 56.27 weight percent of 1,1,1,2-tetrafluoropropene.

13. A refrigerant composition comprising the azeotrope-like composition of claim 12 .

14. A method for cooling an article which comprises condensing a refrigerant composition of claim 13 and thereafter evaporating said refrigerant composition in the vicinity of the article to be cooled.

15. A method for heating an article which comprises condensing a refrigerant composition of claim 13 in the vicinity of the article to be heated and thereafter evaporating said refrigerant composition.

16. The azeotrope-like composition of claim 1 having a boiling point of from about −30.0° C. to about −29.0° C. at a pressure of about 14.3 psia.

17. A refrigerant composition comprising the azeotrope-like composition of claim 1 .

18. A method for cooling an article which comprises condensing a refrigerant composition of claim 17 and thereafter evaporating said refrigerant composition in the vicinity of the article to be cooled.

19. A method for heating an article which comprises condensing a refrigerant composition of claim 17 in the vicinity of the article to be heated and thereafter evaporating said refrigerant composition.

20. A method of recharging a refrigerant system that contains a refrigerant to be replaced and a lubricant comprising the steps of: (a) removing the refrigerant to be replaced from the refrigeration system while retaining a substantial portion of the lubricant in said system; and (b) introducing to the system a refrigerant composition of claim 17 .

Assignments (2)
SECURITY INTEREST Recorded Jan 12, 2026
From: SOLSTICE ADVANCED MATERIALS US, INC.
To: JPMORGAN CHASE BANK, N.A., AS ADMINISTRATIVE AGENT
Reel/Frame 074569/0260 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Mar 30, 2017
From: SEETON, CHRISTOPHER J.; PHAM, HANG T.; SINGH, RAJIV R.; HULSE, RYAN; SPATZ, MARK W.; WILSON, DAVID P.; YANA MOTTA, SAMUEL F.
To: HONEYWELL INTERNATIONAL INC.
Reel/Frame 042114/0727 →
Continuity (3)
Division 12542185 · Aug 17, 2009
Provisional Application 61089986 · Aug 19, 2008
Related Publication 20170065953A1 · Mar 9, 2017