IP Library Granted Patent US 10,485,856
Granted Patent B2
US 10,485,856 · App. 15/462,320 · Granted Nov 26, 2019

Carbon nanotube compositions and methods of use thereof

Inventors: Tarek M. Fahmy (New Haven, CT); Lisa D. Pfefferle (Branford, CT); Gary L. Haller (Hamden, CT); Tarek R. Fadel (Brookline, MA)
Assignee: Yale University
A61K39/00A61K9/20A61K35/17A61K38/2013A61K39/0011A61K39/385A61K39/39A61K2035/124A61K2039/5158A61K2039/55555A61K2039/6093B82Y5/00B82Y40/00Y02A50/412Y10S977/746Y10S977/75Y10S977/847Y10S977/918
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Quick Facts
Patent No.
US 10,485,856
App. No.
15/462,320
Granted
Nov 26, 2019
Kind
B2
Abstract

Carbon nanotube (CNT)-based compositions for activating cellular immune responses are provided. The CNTs function as high surface area scaffolds for the attachment of T cell ligands and/or antigens. The CNT compositions function as artificial antigen-presenting cells (aAPCs) or as modular vaccines. The disclosed CNT aAPCs are efficient at activating T cells and may be used to activate T cells ex vivo or in vivo for adoptive or active immunotherapy.

Claims (21)

1. A method for making a formulation for adoptive immunotherapy comprising

contacting regulatory T cells (Treg) isolated from a subject with carbon nanotube bundles comprising acid washed carbon nanotubes, the nanotubes having bound to or present on the surface one or more T cell receptor activators selected from the group consisting of antigens bound to MHC molecules and antibodies or fragments thereof that crosslink the T cell receptor/CD3 complex, one or more T cell costimulatory or T cell adhesion molecules, and polymeric nanoparticles comprising a cytokine encapsulated therein,

for an effective amount of time to activate, expand, or activate and expand the Treg cells.

2. The method of claim 1 , wherein the formulation is effective for treatment of a disease or disorder selected from the group consisting of allergic disease, autoimmune diseases or disorders, graft rejection or graft-versus-host disease.

3. The method of claim 1 , wherein the method further comprises separating the Treg cells from the nanotube bundles.

4. The method of claim 1 , wherein the Treg cells are CD4 + CD25 + T cells.

5. The method of claim 1 , wherein the nanotubes are single-walled carbon nanotubes.

6. The method of claim 1 , wherein the nanotubes are treated with acid prior to adsorption of the one or more T cell receptor activators, and further treated with lithium borohydride.

7. The method of claim 1 , wherein the one or more T cell receptor activators is MHC molecules bound to peptide antigens.

8. The method of claim 1 , wherein the one or more T cell receptor activators is a polyclonal T cell activator.

9. The method of claim 1 , wherein the one or more T cell receptor activators comprises an antibody or fragment thereof that crosslinks the T cell receptor/CD3 complex.

10. The method of claim 9 , wherein the antibody or fragments thereof that crosslinks the T cell receptor/CD3 complex is anti-CD3 or a fragment thereof.

11. The method of claim 1 , wherein the one or more T cell costimulatory or T cell adhesion molecules is an antibody that specifically binds to a co-stimulatory molecule present on a T cell.

12. The method of claim 11 , wherein the antibody is an anti-CD28 antibody.

13. The method of claim 1 , wherein the polymer of the nanoparticles is biodegradable.

14. The method of claim 13 , wherein the biodegradable polymer comprises polylactic acid, polyglycolic acid, or polylactide-co-glycolide.

15. The method of claim 1 , wherein the cytokine is IL-2.

16. The method of claim 1 , wherein the nanoparticle further comprises ferromagnetic and superparamagnetic materials.

17. The method of claim 1 , wherein the nanotube comprises a magnetic particle bound to or present thereon.

18. The method of claim 17 , wherein the magnetic particle is selected from the group consisting of ferromagnetic and superparamagnetic materials.

19. The method of claim 1 , wherein the Treg cells contacted with carbon nanotube bundles were positively selected, negatively selected, or positively and negatively selected from a population of T cells isolated from the subject.

Assignments (4)
CONFIRMATORY LICENSE Recorded May 10, 2023
From: YALE UNIVERSITY
To: NATIONAL SCIENCE FOUNDATION
Reel/Frame 063593/0708 →
CONFIRMATORY LICENSE Recorded Nov 16, 2020
From: YALE UNIVERSITY
To: NATIONAL SCIENCE FOUNDATION
Reel/Frame 054438/0825 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jan 24, 2018
From: FADEL, TAREK R.
To: YALE UNIVERSITY
Reel/Frame 044717/0571 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Mar 17, 2017
From: FAHMY, TAREK M.; PFEFFERLE, LISA D.; HALLER, GARY
To: YALE UNIVERSITY
Reel/Frame 041622/0158 →
Continuity (4)
Division 13842782 · Mar 15, 2013
Continuation In Part 12933223
Provisional Application 61037798 · Mar 19, 2008
Related Publication 20170209570A1 · Jul 27, 2017