IP Library Granted Patent US 10,326,121
Granted Patent B2
US 10,326,121 · App. 15/483,311 · Granted Jun 18, 2019

Oxidation resistant separator for a battery

Inventors: Zhengming Zhang (Rock Hill, SC); Pankaj Arora (Chesterfield, VA)
Assignee: Celgard, LLC
H01M2/1686H01M2/145H01M2/1653H01M2/1673H01M4/628H01M10/058H01M10/0525
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Quick Facts
Patent No.
US 10,326,121
App. No.
15/483,311
Granted
Jun 18, 2019
Kind
B2
Abstract

A method for preventing oxidation of a polyolefin separator in a lithium ion secondary battery includes the steps of: providing a lithium ion secondary battery having a positive electrode and a polyolefin separator film; and positioning an antioxidative barrier coating between the positive electrode and the polyolefin separator film, the antioxidative barrier coating being made of a polymer having a resistance to oxidation greater than polyethylene.

Claims (28)

1. A method for preventing oxidation on a polyolefin separator in a lithium ion secondary battery comprising the steps of:

providing a lithium ion secondary battery having a positive electrode and a polyolefin separator film; and

positioning an antioxidative barrier coating between the positive electrode and the polyolefin separator film,

the antioxidative barrier coating comprises polyvinylidene fluoride and polypropylene;

wherein the antioxidative barrier coating has a weight of <0.15 mg/cm 2 .

2. The method of claim 1 wherein the antioxidative barrier coating is a discrete polymer coating formed onto the polyolefin separator film and/or the positive electrode by a coating method selected from the group consisting of brushing, spraying, applying via roller, and applying by immersion.

3. The method of claim 1 wherein the antioxidative barrier coating is formed on the polyolefin separator film.

4. The method of claim 1 wherein the antioxidative barrier coating is formed on the positive electrode.

5. The method of claim 1

wherein at least one of polyvinylidene fluoride and polypropylene is included in the polyolefin separator film.

6. The method of claim 1 wherein the polyolefin separator film is made of polyethylene, copolymers thereof and mixtures thereof.

7. The method of claim 6 wherein the polyolefin separator film is a single layered film.

8. The method of claim 6 wherein the polyolefin separator film is a multi-layered film.

9. A method for preventing oxidation on a polyolefin separator in a lithium ion secondary battery comprising the steps of:

providing a lithium ion secondary battery having a positive electrode and a polyolefin separator film;

adding an antioxidative barrier between the positive electrode and the separator film,

the antioxidative barrier including a polymer having a resistance to oxidation greater than polyethylene,

the polymer comprises polyvinylidene fluoride and polypropylene; and

positioning the antioxidative barrier toward the positive electrode;

wherein the antioxidative barrier has a weight of <0.15 mg/cm 2 .

10. The method of claim 9 wherein the antioxidative barrier is a discrete polymer coating formed on the polyolefin separator film.

11. A method for preventing oxidation on a polyolefin separator in a lithium ion secondary battery comprising the steps of:

providing a lithium ion secondary battery having a positive electrode and a polyolefin separator film;

positioning an antioxidative barrier coating between the positive electrode and the polyolefin separator film,

the antioxidative barrier coating is a discrete polymer coating formed on the polyolefin separator film and/or on the positive electrode,

the antioxidative barrier coating includes a polymer having a resistance to oxidation greater than polyethylene, and

the polymer comprises polyvinylidene fluoride and polypropylene; and

wherein the antioxidative barrier coating has a weight of <0.15 mg/cm 2 .

Continuity (3)
Division 11549273 · Oct 13, 2006
Division 10371461 · Feb 21, 2003
Related Publication 20170214023A1 · Jul 27, 2017