IP Library Granted Patent US 10,532,972
Granted Patent B2
US 10,532,972 · App. 15/499,967 · Granted Jan 14, 2020

Dibasic esters and the use thereof in plasticizer compositions

Inventors: Tessa Pals (Woodridge, IL); Steven A. Cohen (Woodridge, IL); Thomas E. Snead (Woodridge, IL); Allyson Beuhler (Woodridge, IL); Paul A. Bertin (Woodridge, IL)
Assignee: Elevance Renewable Sciences, Inc.
C07C69/67C07C69/34C08K5/06C08K5/11
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Quick Facts
Patent No.
US 10,532,972
App. No.
15/499,967
Granted
Jan 14, 2020
Kind
B2
Abstract

Dibasic esters (diesters) and their use in plasticizer compositions are generally disclosed. In some embodiments, the diesters are branched-chain esters of long-chain alkanedioic acids, such as octadecanedioic acid. In some embodiments, such plasticizer compositions are used to increase the plasticity of a polymer resin, such as a vinyl chloride resin or poly vinyl butyral. In some other embodiments, such plasticizer compositions are used to lower the glass transition temperature of a polymer resin. In some embodiments, at least a portion of the plasticizer is derived from a renewable source, such as a natural oil.

Claims (16)

1. A compound of formula (I):

wherein:

X 1 is —(CH 2 ) 16 —, —(CH 2 ) 18 —, —(CH 2 ) 20 —, or —(CH 2 ) 22 —;

R 1 is —(CH 2 —CH 2 —O) 3-12 —(C 1-6 unbranched alkyl); and

R 2 is —(CH 2 —CH 2 —O) 3-12 —(C 1-6 unbranched alkyl).

2. The compound of claim 1 , wherein X 1 is —(CH 2 ) 16 —.

3. The compound of claim 1 , wherein R 1 is —(CH 2 —CH 2 —O) 3 —CH 3 , —(CH 2 —CH 2 —O) 4 —CH 3 , —(CH 2 —CH 2 —O) 5 —CH 3 , —(CH 2 —CH 2 —O) 6 —CH 3 , —(CH 2 —CH 2 —O) 7 —CH 3 , —(CH 2 —CH 2 —O) 8 —CH 3 , —(CH 2 —CH 2 —O) 9 —CH 3 , —(CH 2 —CH 2 —O) 10 —CH 3 , —(CH 2 —CH 2 —O) 11 —CH 3 , or —(CH 2 —CH 2 —O) 12 —CH 3 .

4. The compound of claim 1 , wherein R 2 is —(CH 2 —CH 2 —O) 3 —CH 3 , —(CH 2 —CH 2 —O) 4 —CH 3 , —(CH 2 —CH 2 —O) 5 —CH 3 , —(CH 2 —CH 2 —O) 6 —CH 3 , —(CH 2 —CH 2 —O) 7 —CH 3 , —(CH 2 —CH 2 —O) 8 —CH 3 , —(CH 2 —CH 2 —O) 9 —CH 3 , —(CH 2 —CH 2 —O) 10 —CH 3 , —(CH 2 —CH 2 —O) 11 —CH 3 , or —(CH 2 —CH 2 —O) 12 —CH 3 .

5. The compound of claim 1 , wherein R 1 and R 2 are the same.

6. The compound of claim 1 , wherein R 1 and R 2 are not the same.

7. A plasticizer composition, comprising a compound of claim 1 .

8. The plasticizer composition of claim 7 , further comprising one or more additional plasticizers.

9. The plasticizer composition of claim 8 , wherein the one or more additional plasticizers are phthalates, adipates, trimellitic esters, phosphate esters, sebacates, azelates, sulphonates, epoxidized fatty acid esters, or a combination thereof.

10. The plasticizer composition of claim 7 , further comprising one or more additives.

11. The plasticizer composition of claim 10 , wherein the one or more additives are: metal oxides; antioxidants; colorants; color modifiers; diluents; or any combinations thereof.

12. The plasticizer composition of claim 9 , wherein the one or more additional plasticizers are benzenedicarboxylic esters, citraconic esters, 2-hydroxy-1,2,3-propanetricarboxylic esters, malonic esters, succinates, vegetable and animal oils, benzoic esters, triethylene glycol dihexanoate, tetraethylene glycol diheptanoate, linear alkylbenzenes (LABs), branched alkylbenzenes (BABs), polyethylene glycols, polyethylene glycol ethers, polypropylene glycols, polypropylene glycol ethers, or any combinations thereof.

Assignments (3)
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Jun 15, 2020
From: ELEVANCE RENEWABLE SCIENCES, INC.
To: WILMAR TRADING PTE LTD
Reel/Frame 052942/0933 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded May 14, 2019
From: COHEN, STEVEN A.; SNEAD, THOMAS E.; BEUHLER, ALLYSON; BERTIN, PAUL A.
To: ELEVANCE RENEWABLE SCIENCES, INC.
Reel/Frame 049177/0180 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded May 14, 2019
From: PALS, TESSA
To: ELEVANCE RENEWABLE SCIENCES, INC.
Reel/Frame 049177/0223 →