IP Library Granted Patent US 10,537,856
Granted Patent B2
US 10,537,856 · App. 15/505,752 · Granted Jan 21, 2020

Hollow fiber membrane and hollow fiber membrane module

Inventors: Noritaka Shibata (Toyohashi, JP); Kenjiro Takayanagi (Tokyo, JP)
Assignee: Mitsubishi Chemical Corporation
B01D69/02B01D69/043C08L23/12C08L25/06C08L67/02C08L2207/04C08L2207/062
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Quick Facts
Patent No.
US 10,537,856
App. No.
15/505,752
Granted
Jan 21, 2020
Kind
B2
Abstract

The invention provides a hollow fiber membrane exhibiting a favorable gas permeation performance and an excellent heat resistance in which the generation of pinholes are suppressed, and a hollow fiber membrane module using the same. The hollow fiber membrane comprising a gas permeable nonporous layer; and a porous supporting layer to support the nonporous layer formed of a thermoplastic elastomer having a DSC melting peak temperature of 130° C. or higher and a rupture elongation prescribed in ISO 37 (2010) of 300% or more.

Claims (21)

1. A hollow fiber membrane comprising:

a gas permeable nonporous layer; and

a porous supporting layer to support the nonporous layer,

wherein:

the nonporous layer is formed of a thermoplastic elastomer having a DSC melting peak temperature of 130° C. or higher and a rupture elongation prescribed in ISO 37 (2010) of 300% or more,

the nonporous layer is formed of a composition containing a styrene-based thermoplastic elastomer (I) and a polyolefin (II), wherein the styrene-based thermoplastic elastomer (I) containing at least either of an ABA type styrene-based thermoplastic elastomer (α) having a polystyrene portion (A) and a poly-conjugated diene portion (B) or a hydrogenated product (αh) of the ABA type styrene-based thermoplastic elastomer (α), and

the composition contains the styrene-based thermoplastic elastomer (I) at 60% by mass or more and 90% by mass or less with respect to a total amount of the styrene-based thermoplastic elastomer (I) and the polyolefin (II), and

the polyolefin (II) is an unsaturated carboxylic acid-modified polypropylene.

2. The hollow fiber membrane according to claim 1 , wherein

the poly-conjugated diene portion (B) contains at least either of a 1,2-bonding unit or a 3,4-bonding unit, wherein

a total amount of the 1,2-bonding unit and the 3,4-bonding unit is 50% by mole or more with respect to a total amount of the entire units constituting the poly-conjugated diene portion (B).

3. The hollow fiber membrane according to claim 1 , wherein the poly-conjugated diene portion (B) contains at least either of butadiene or isoprene as a component.

4. The hollow fiber membrane according to claim 1 , wherein a thickness of the nonporous layer is 0.5 μm or more and 10 μm or less.

5. The hollow fiber membrane according to claim 1 , wherein the porous supporting layer is formed of polyethylene.

6. The hollow fiber membrane according to claim 5 , wherein polyethylene is high-density polyethylene.

7. A hollow fiber membrane module comprising the hollow fiber membrane according to claim 1 .

8. The hollow fiber membrane according to claim 2 , wherein the total amount of the 1,2-bonding unit and the 3,4-bonding unit is 60% by mole or more and 80% by mole or less with respect to a total amount of the entire units constituting the poly-conjugated diene portion (B).

9. The hollow fiber membrane according to claim 2 , wherein the total amount of the 1,2-bonding unit and the 3,4-bonding unit is 60% by mole or more and 70% by mole or less with respect to a total amount of the entire units constituting the poly-conjugated diene portion (B).

10. The hollow fiber membrane according to claim 1 , wherein the unsaturated carboxylic acid-modified polypropylene is a graft product of an unsaturated carboxylic acid selected from the group consisting of anhydrous maleic acid, acrylic acid, methacrylic acid, maleic acid, itaconic acid and fumaric acid.

11. The hollow fiber membrane according to claim 1 , wherein a mass average molecular weight (Mw) of each of the ABA type styrene-based thermoplastic elastomer (α) and the hydrogenated product (αH) is 5,000 or more and 150,000 or less.

12. The hollow fiber membrane according to claim 1 , wherein a mass average molecular weight (Mw) of each of the ABA type styrene-based thermoplastic elastomer (α) and the hydrogenated product (αH) is 7,000 or more and 130,000 or less.

Assignments (2)
MERGER Recorded Jun 28, 2017
From: MITSUBISHI RAYON CO., LTD.
To: MITSUBISHI CHEMICAL CORPORATION
Reel/Frame 043029/0663 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded Feb 22, 2017
From: SHIBATA, NORITAKA; TAKAYANAGI, KENJIRO
To: MITSUBISHI RAYON CO., LTD.
Reel/Frame 041341/0781 →
Priority Claims (1)
JP 2014-171904 · Aug 26, 2014 · national
Continuity (1)
Related Publication 20170266624A1 · Sep 21, 2017