IP Library Granted Patent US 10,246,658
Granted Patent B2
US 10,246,658 · App. 15/592,080 · Granted Apr 2, 2019

Biorenewable kerosene, jet fuel, jet fuel blendstock, and method of manufacturing

Inventors: Ramin Abhari (Bixby, OK); David A. Slade (Ames, IA); H. Lynn Tomlinson (Tulsa, OK); Erik Ashby (S. San Francisco, CA); Nate Green (Ames, IA); Caroline Golden (Baton Rouge, LA)
Assignee: REG SYNTHETIC FUELS, LLC
C10L1/08C10G3/50C10G3/54C10L1/04C10L5/361C10L5/365C10L11/04C10G2300/1011C10G2300/1014C10G2300/304C10G2400/04C10G2400/08C10L2200/0469C10L2230/06C10L2270/026C10L2270/04Y02E50/13Y02P30/20Y02T50/678
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Quick Facts
Patent No.
US 10,246,658
App. No.
15/592,080
Granted
Apr 2, 2019
Kind
B2
Abstract

The present technology provides compositions that include at least about 98 weight percent (wt. %) n-paraffins which, among other surprising features, may be suitable for use as a diesel fuel, an aviation fuel, a jet fuel blendstock, a blendstock to reduce the cloud point of a diesel fuel, a fuel for portable heaters, and/or as a charcoal lighter fluid. The composition includes at least 98 wt. % C 7 -C 12 n-paraffins, where at least 10 wt. % of composition includes n-decane, at least 20 wt. % of the composition includes n-dodecane, and at least 75 wt. % of the composition includes even carbon number paraffins. The composition also includes less than 0.1 wt. % oxygenates and less than 0.1 wt. % aromatics. The composition may be produced by a process that includes hydrotreating a biorenewable feedstock comprising at least one of palm kernel oil, coconut oil, babassu oil, microbial oil, or algal oil.

Claims (38)

1. A composition comprising

at least 98 wt % C 7 -C 12 n-paraffins, wherein at least 10 wt % of composition comprises n-decane, at least 20 wt % of the composition comprises n-dodecane, and at least 75 wt % of composition comprises even carbon number paraffins, and a weight ratio of C 12 paraffins to C 11 paraffins from 3.0:1 to 1.2:1;

less than 0.1 wt % oxygenates; and

less than 0.1 wt % aromatics.

2. The composition of claim 1 , wherein at least 75 wt % of composition comprises even carbon number n-paraffins.

3. The composition of claim 1 , wherein the composition comprises less than 0.01 wt % oxygenates.

4. The composition of claim 1 , wherein at least 20 wt % of the composition comprises n-octane.

5. The composition of claim 1 , wherein a weight ratio of C 12 paraffins to C 7 paraffins is 150:1 or greater.

6. The composition of claim 1 , wherein a weight ratio of C 12 paraffins to C 9 paraffins is 10:1 or greater.

7. The composition of claim 1 , wherein a weight ratio of C 10 paraffins to C 7 paraffins is 150:1 or greater.

8. The composition of claim 1 , wherein a weight ratio of C 10 paraffins to C 9 paraffins is 10:1 or greater.

9. The composition of claim 1 , wherein a weight ratio of C 10 paraffins to C 11 paraffins is from 2.0:1 to 0.5:1.

10. The composition of claim 1 , wherein a weight ratio of C 12 paraffins to C 10 paraffins is from 2.0:1 to 0.5:1.

11. The composition of claim 1 , wherein the composition is suitable as a diesel fuel, a diesel fuel additive, a diesel fuel blendstock, a turbine fuel, a turbine fuel additive, a turbine fuel blendstock, an aviation fuel, an aviation fuel additive, an aviation fuel blendstock, a fuel for portable heaters, a fuel for portable generators, a charcoal lighter fluid, or a combination of any two or more thereof.

12. A charcoal heating material comprising

a charcoal comprising

wood char;

a binder;

an exterior surface of the charcoal; and

optionally a plurality of pores within the charcoal; and

a composition of claim 1 disposed on at least the exterior surface of the charcoal.

13. A method of producing the composition of claim 1 , the method comprising

contacting a feed stream comprising a biorenewable feedstock with a hydrotreatment catalyst in a fixed bed hydrotreatment reactor to produce a hydrotreated product; and

fractionating the hydrotreated product to produce the composition;

wherein

the biorenewable feedstock comprises at least one of palm kernel oil, coconut oil, babassu oil, microbial oil, or algal oil;

the fixed bed hydrotreatment reactor

is at a temperature less than 750° F.; and

is at a pressure from 200 psig to 4,000 psig.

14. The method of claim 13 , wherein the liquid hourly space velocity of the biorenewable feedstock through the fixed bed hydrotreatment reactor is from 0.2 hr −1 to 10.0 hr −1 .

15. The method of claim 13 , wherein the method comprises fractionating the hydrotreated product to produce the composition and one or more C 14 -C 22 n-paraffin fractions comprising at least 90 wt % C 14 -C 22 n-paraffins.

16. The method of claim 15 , wherein the one or more C 14 -C 22 n-paraffin fractions comprises one or more of a fraction comprising at least 90 wt % n-hexadecane, a fraction comprising at least 90 wt % n-octadecane; a fraction comprising at least 90 wt % n-icosane, and a fraction comprising at least 90 wt % n-docosane.

17. A phase change material comprising a C 14 -C 22 n-paraffin fraction of claim 16 .

18. A blended fuel comprising

a composition of claim 1 ; and

a petroleum-based fuel and/or a synthetic fuel.

19. A method for producing a blended fuel, the method comprising combining a composition of claim 1 with a petroleum-based fuel and/or a synthetic fuel to produce the blended fuel.

20. The composition of claim 1 , wherein the composition is produced by hydrotreating a biorenewable feedstock comprising at least one of palm kernel oil, coconut oil, babassu oil, microbial oil, or algal oil.

Assignments (3)
RELEASE OF SECURITY INTEREST Recorded Jul 1, 2022
From: UMB BANK, N.A., AS COLLATERAL TRUSTEE
To: REG SYNTHETIC FUELS, LLC; RENEWABLE ENERGY GROUP, INC.; REG SENECA, LLC; REG BIOFUELS, LLC
Reel/Frame 060562/0428 →
PATENT SECURITY AGREEMENT Recorded Jun 19, 2021
From: REG SYNTHETIC FUELS, LLC
To: UMB BANK, N.A., AS COLLATERAL TRUSTEE
Reel/Frame 056628/0673 →
ASSIGNMENT OF ASSIGNOR'S INTEREST Recorded May 15, 2017
From: ABHARI, RAMIN; SLADE, DAVID A.; TOMLINSON, H. LYNN; ASHBY, ERIK; GREEN, NATE; GOLDEN, CAROLINE
To: REG SYNTHETIC FUELS, LLC
Reel/Frame 042375/0073 →
Continuity (2)
Provisional Application 62334968 · May 11, 2016
Related Publication 20170327757A1 · Nov 16, 2017
Cited By (3)
US 12,297,393 US 12,331,254 US 12,522,771